{"id":"https://openalex.org/W7225397397","doi":"https://doi.org/10.1002/adfm.79529","title":"Molecular Polarization Engineering Homogenizes Interfacial Potential for Long\u2010Life Wide\u2010Temperature Solid\u2010State Lithium Metal Batteries","display_name":"Molecular Polarization Engineering Homogenizes Interfacial Potential for Long\u2010Life Wide\u2010Temperature Solid\u2010State Lithium Metal Batteries","publication_year":2026,"publication_date":"2026-11-06","ids":{"openalex":"https://openalex.org/W7225397397","doi":"https://doi.org/10.1002/adfm.79529"},"language":"en","primary_location":{"id":"doi:10.1002/adfm.79529","doi":"https://doi.org/10.1002/adfm.79529","is_oa":false,"landing_page_url":"https://doi.org/10.1002/adfm.79529","pdf_url":null,"source":{"id":"https://openalex.org/S135204980","display_name":"Advanced Functional Materials","issn_l":"1616-301X","issn":["1616-301X","1616-3028"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-3","ki-jl-3","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320595","host_organization_name":"Wiley","host_organization_lineage":["https://openalex.org/P4310320595"],"host_organization_lineage_names":["Wiley"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Advanced Functional Materials","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5048823268","display_name":"Dajiang Tang","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I150229711","display_name":"University of Electronic Science and Technology of China","ror":"https://ror.org/04qr3zq92","country_code":"CN","type":"education","lineage":["https://openalex.org/I150229711"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Dajiang Tang","raw_affiliation_strings":["School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China","institution_ids":["https://openalex.org/I150229711"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5100430668","display_name":"Yiwen Zhang","orcid":"https://orcid.org/0000-0002-8620-1166","observed_orcids":["https://orcid.org/0000-0002-8620-1166"]},"institutions":[{"id":"https://openalex.org/I150229711","display_name":"University of Electronic Science and Technology of China","ror":"https://ror.org/04qr3zq92","country_code":"CN","type":"education","lineage":["https://openalex.org/I150229711"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Yiwen Zhang","raw_affiliation_strings":["School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China","institution_ids":["https://openalex.org/I150229711"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5062211829","display_name":"Xiaoyang Du","orcid":"https://orcid.org/0000-0002-1021-1819","observed_orcids":["https://orcid.org/0000-0002-1021-1819"]},"institutions":[{"id":"https://openalex.org/I150229711","display_name":"University of Electronic Science and Technology of China","ror":"https://ror.org/04qr3zq92","country_code":"CN","type":"education","lineage":["https://openalex.org/I150229711"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Xiaoyang Du","raw_affiliation_strings":["School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China","institution_ids":["https://openalex.org/I150229711"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5022944715","display_name":"Caijun Zheng","orcid":"https://orcid.org/0000-0002-4157-4313","observed_orcids":["https://orcid.org/0000-0002-4157-4313"]},"institutions":[{"id":"https://openalex.org/I150229711","display_name":"University of Electronic Science and Technology of China","ror":"https://ror.org/04qr3zq92","country_code":"CN","type":"education","lineage":["https://openalex.org/I150229711"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Cai\u2010jun Zheng","raw_affiliation_strings":["School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China"],"raw_orcid":"https://orcid.org/0000-0002-4157-4313","affiliations":[{"raw_affiliation_string":"School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China","institution_ids":["https://openalex.org/I150229711"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5053095176","display_name":"Yongbing Tang","orcid":"https://orcid.org/0000-0003-2705-4618","observed_orcids":["https://orcid.org/0000-0003-2705-4618"]},"institutions":[{"id":"https://openalex.org/I19820366","display_name":"Chinese Academy of Sciences","ror":"https://ror.org/034t30j35","country_code":"CN","type":"government","lineage":["https://openalex.org/I19820366"]},{"id":"https://openalex.org/I4210145761","display_name":"Shenzhen Institutes of Advanced Technology","ror":"https://ror.org/04gh4er46","country_code":"CN","type":"facility","lineage":["https://openalex.org/I19820366","https://openalex.org/I4210145761"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Yongbing Tang","raw_affiliation_strings":["Advanced Energy Storage Technology Research Center Shenzhen Institutes of Advanced Technology Chinese Academy of Sciences  Shenzhen People's Republic of China"],"raw_orcid":"https://orcid.org/0000-0003-2705-4618","affiliations":[{"raw_affiliation_string":"Advanced Energy Storage Technology Research Center Shenzhen Institutes of Advanced Technology Chinese Academy of Sciences  Shenzhen People's Republic of China","institution_ids":["https://openalex.org/I19820366","https://openalex.org/I4210145761"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5018183694","display_name":"Silu Tao","orcid":"https://orcid.org/0000-0001-6232-9934","observed_orcids":["https://orcid.org/0000-0001-6232-9934"]},"institutions":[{"id":"https://openalex.org/I150229711","display_name":"University of Electronic Science and Technology of China","ror":"https://ror.org/04qr3zq92","country_code":"CN","type":"education","lineage":["https://openalex.org/I150229711"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Silu Tao","raw_affiliation_strings":["School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China"],"raw_orcid":"https://orcid.org/0000-0001-6232-9934","affiliations":[{"raw_affiliation_string":"School of Optoelectronic Science and Engineering University of Electronic Science and Technology of China  Chengdu People's Republic of China","institution_ids":["https://openalex.org/I150229711"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":3,"corresponding_author_ids":["https://openalex.org/A5018183694","https://openalex.org/A5053095176","https://openalex.org/A5062211829"],"corresponding_institution_ids":["https://openalex.org/I150229711","https://openalex.org/I19820366","https://openalex.org/I4210145761"],"apc_list":{"value":5790,"currency":"USD","value_usd":5790},"apc_paid":null,"fwci":0.0,"has_fulltext":false,"cited_by_count":0,"citation_normalized_percentile":{"value":0.0,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":1.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":1.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11690","display_name":"Aqueous and Flow Batteries","score":0.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/solid-state-lithium-metal-batteries","display_name":"solid-state lithium metal batteries","score":0.9929999709129333},{"id":"https://openalex.org/keywords/lithium-dendrite-suppression","display_name":"lithium dendrite suppression","score":0.9610000252723694},{"id":"https://openalex.org/keywords/molecular-polarization","display_name":"molecular polarization","score":0.5339999794960022},{"id":"https://openalex.org/keywords/mof-177","display_name":"MOF-177","score":0.8289999961853027},{"id":"https://openalex.org/keywords/lithium-transference-number","display_name":"lithium transference number","score":0.7350000143051147},{"id":"https://openalex.org/keywords/ionic-conductivity","display_name":"ionic conductivity","score":0.722000002861023},{"id":"https://openalex.org/keywords/wide-temperature-cycling","display_name":"wide-temperature cycling","score":0.8090000152587891},{"id":"https://openalex.org/keywords/lithium-nucleation","display_name":"lithium nucleation","score":0.6669999957084656},{"id":"https://openalex.org/keywords/lithium-metal-anode","display_name":"lithium metal anode","score":0.45399999618530273}],"concepts":[{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.8418999910354614},{"id":"https://openalex.org/C68801617","wikidata":"https://www.wikidata.org/wiki/Q162908","display_name":"Electrolyte","level":3,"score":0.7669000029563904},{"id":"https://openalex.org/C2994426979","wikidata":"https://www.wikidata.org/wiki/Q568","display_name":"Lithium metal","level":4,"score":0.7049999833106995},{"id":"https://openalex.org/C205049153","wikidata":"https://www.wikidata.org/wiki/Q2698605","display_name":"Polarization (electrochemistry)","level":2,"score":0.6489999890327454},{"id":"https://openalex.org/C29705727","wikidata":"https://www.wikidata.org/wiki/Q294562","display_name":"Polar","level":2,"score":0.6176999807357788},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.5347999930381775},{"id":"https://openalex.org/C544153396","wikidata":"https://www.wikidata.org/wiki/Q11426","display_name":"Metal","level":2,"score":0.5097000002861023},{"id":"https://openalex.org/C2182769","wikidata":"https://www.wikidata.org/wiki/Q62500","display_name":"Ionic bonding","level":3,"score":0.492900013923645},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.4893999993801117},{"id":"https://openalex.org/C521977710","wikidata":"https://www.wikidata.org/wiki/Q81163","display_name":"Polymer","level":2,"score":0.4828999936580658},{"id":"https://openalex.org/C2778541603","wikidata":"https://www.wikidata.org/wiki/Q152763","display_name":"Lithium (medication)","level":2,"score":0.4697999954223633},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.39399999380111694},{"id":"https://openalex.org/C84248122","wikidata":"https://www.wikidata.org/wiki/Q5256671","display_name":"Dendrite (mathematics)","level":2,"score":0.3797999918460846},{"id":"https://openalex.org/C138679309","wikidata":"https://www.wikidata.org/wiki/Q6063658","display_name":"Ionic conductivity","level":4,"score":0.37959998846054077},{"id":"https://openalex.org/C117626034","wikidata":"https://www.wikidata.org/wiki/Q26336","display_name":"Electrostatics","level":2,"score":0.36239999532699585},{"id":"https://openalex.org/C2986395496","wikidata":"https://www.wikidata.org/wiki/Q107223477","display_name":"Polymer electrolytes","level":5,"score":0.3301999866962433},{"id":"https://openalex.org/C131540310","wikidata":"https://www.wikidata.org/wiki/Q907564","display_name":"Conductivity","level":2,"score":0.314300000667572},{"id":"https://openalex.org/C38115104","wikidata":"https://www.wikidata.org/wiki/Q582852","display_name":"Concentration polarization","level":3,"score":0.2937999963760376},{"id":"https://openalex.org/C18762648","wikidata":"https://www.wikidata.org/wiki/Q42213","display_name":"Work (physics)","level":2,"score":0.27959999442100525},{"id":"https://openalex.org/C2778722038","wikidata":"https://www.wikidata.org/wiki/Q17030643","display_name":"Homogenization (climate)","level":3,"score":0.2648000121116638}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.1002/adfm.79529","doi":"https://doi.org/10.1002/adfm.79529","is_oa":false,"landing_page_url":"https://doi.org/10.1002/adfm.79529","pdf_url":null,"source":{"id":"https://openalex.org/S135204980","display_name":"Advanced Functional Materials","issn_l":"1616-301X","issn":["1616-301X","1616-3028"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-3","ki-jl-3","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320595","host_organization_name":"Wiley","host_organization_lineage":["https://openalex.org/P4310320595"],"host_organization_lineage_names":["Wiley"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Advanced Functional Materials","raw_type":"journal-article"}],"best_oa_location":null,"sustainable_development_goals":[{"score":0.8485000133514404,"id":"https://metadata.un.org/sdg/7","display_name":"Affordable and clean energy"}],"study_designs":[],"awards":[],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"},{"id":"https://openalex.org/F4320329861","display_name":"Natural Science Foundation of Sichuan Province","ror":null}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":57,"referenced_works":["https://openalex.org/W2055282068","https://openalex.org/W3044672044","https://openalex.org/W3087196714","https://openalex.org/W4206119841","https://openalex.org/W4288441821","https://openalex.org/W4317584327","https://openalex.org/W4321618060","https://openalex.org/W4378172096","https://openalex.org/W4378700635","https://openalex.org/W4386532187","https://openalex.org/W4388022715","https://openalex.org/W4390670057","https://openalex.org/W4390913515","https://openalex.org/W4391135849","https://openalex.org/W4391926362","https://openalex.org/W4393852901","https://openalex.org/W4393995027","https://openalex.org/W4396696357","https://openalex.org/W4399040490","https://openalex.org/W4399366761","https://openalex.org/W4399805164","https://openalex.org/W4399889828","https://openalex.org/W4400423755","https://openalex.org/W4400729979","https://openalex.org/W4403302529","https://openalex.org/W4403778455","https://openalex.org/W4404769494","https://openalex.org/W4404777692","https://openalex.org/W4406231056","https://openalex.org/W4407040095","https://openalex.org/W4407842631","https://openalex.org/W4408956993","https://openalex.org/W4409726817","https://openalex.org/W4410751064","https://openalex.org/W4410906589","https://openalex.org/W4411159809","https://openalex.org/W4412385483","https://openalex.org/W4412854955","https://openalex.org/W4413108997","https://openalex.org/W4413172781","https://openalex.org/W4413411228","https://openalex.org/W4413497967","https://openalex.org/W4413999269","https://openalex.org/W4414300074","https://openalex.org/W4415208713","https://openalex.org/W4415545763","https://openalex.org/W4416399904","https://openalex.org/W4416541863","https://openalex.org/W4416857997","https://openalex.org/W4417319484","https://openalex.org/W4417490349","https://openalex.org/W7087674795","https://openalex.org/W7116904583","https://openalex.org/W7117688178","https://openalex.org/W7127107070","https://openalex.org/W7154958651","https://openalex.org/W7168341934"],"related_works":["https://openalex.org/W7165186290","https://openalex.org/W4407959235","https://openalex.org/W7225305677","https://openalex.org/W7127420750","https://openalex.org/W2987560408","https://openalex.org/W7213446733","https://openalex.org/W7124168712","https://openalex.org/W7170143957","https://openalex.org/W7204190094","https://openalex.org/W4417187873"],"abstract_inverted_index":{"ABSTRACT":[0],"Lithium":[1],"dendrite":[2],"formation":[3],"in":[4],"solid\u2010state":[5,181],"lithium":[6,94,182],"metal":[7,183],"batteries":[8],"originates":[9],"not":[10],"only":[11],"from":[12,17],"mechanical":[13,35],"failure":[14],"but":[15],"also":[16],"spatially":[18],"heterogeneous":[19],"interfacial":[20,39,45,54],"electrostatic":[21,46,82,168],"fields":[22],"that":[23],"induce":[24],"localized":[25],"Li":[26,85,112],"+":[27,86,113],"accumulation.":[28],"However,":[29],"existing":[30],"electrolyte":[31,65],"designs":[32],"mainly":[33],"regulate":[34],"strength":[36],"or":[37],"chemical":[38],"reactions,":[40],"while":[41,147],"dynamic":[42],"regulation":[43,83,169],"of":[44,102,116],"disorder":[47],"remains":[48],"unexplored.":[49],"Here,":[50],"we":[51],"introduce":[52],"an":[53,99],"potential":[55],"homogenization":[56],"enabled":[57],"by":[58],"polarization\u2010mediated":[59],"regulation.":[60],"A":[61],"molecularly":[62],"entangled":[63],"PEO/polyurethane/MOF\u2010177":[64],"is":[66],"constructed,":[67],"where":[68],"polar":[69,171],"polymer":[70],"networks":[71],"and":[72,91,110,157],"MOF":[73],"polarization":[74],"domains":[75],"cooperatively":[76],"redistribute":[77],"local":[78],"electric\u2010field":[79],"fluctuations.":[80],"This":[81,165],"homogenizes":[84],"flux,":[87],"lowers":[88],"migration":[89],"barriers,":[90],"suppresses":[92],"preferential":[93],"nucleation.":[95],"Consequently,":[96],"CPEZ":[97],"exhibits":[98],"ionic":[100],"conductivity":[101],"1.9":[103],"\u00d7":[104],"10":[105],"\u22123":[106],"S":[107],"cm":[108,133],"\u22121":[109],"a":[111,174],"transference":[114],"number":[115],"0.71,":[117],"both":[118],"measured":[119],"at":[120,130,144,155,163],"60\u00b0C.":[121],"The":[122,136],"Li/CPEZ/Li":[123],"cell":[124],"cycles":[125,154,158,162],"stably":[126,159],"for":[127,160,178],"9000":[128],"h":[129],"0.1":[131],"mAh":[132],"\u22122":[134],".":[135],"Li/CPEZ/LFP":[137,148],"retains":[138,149],"90":[139],"%":[140],"capacity":[141,151],"after":[142,152],"5000":[143],"1":[145],"C,":[146],"85%":[150],"500":[153],"100\u00b0C":[156],"150":[161],"\u221215\u00b0C.":[164],"work":[166],"establishes":[167],"via":[170],"interactions":[172],"as":[173],"transferable":[175],"design":[176],"principle":[177],"durable,":[179],"wide\u2010temperature":[180],"batteries.":[184]},"counts_by_year":[],"updated_date":"2026-11-10T11:39:43.021295","created_date":"2026-11-07T00:00:00"}