{"id":"https://openalex.org/W7225201589","doi":"https://doi.org/10.1021/acsnano.6c17609","title":"Site-Differentiated High-Entropy Alloy Surface Enables Efficient Hydrogen Evolution in Acidic and Alkaline Media","display_name":"Site-Differentiated High-Entropy Alloy Surface Enables Efficient Hydrogen Evolution in Acidic and Alkaline Media","publication_year":2026,"publication_date":"2026-11-03","ids":{"openalex":"https://openalex.org/W7225201589","doi":"https://doi.org/10.1021/acsnano.6c17609"},"language":"en","primary_location":{"id":"doi:10.1021/acsnano.6c17609","doi":"https://doi.org/10.1021/acsnano.6c17609","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsnano.6c17609","pdf_url":null,"source":{"id":"https://openalex.org/S145476921","display_name":"ACS Nano","issn_l":"1936-0851","issn":["1936-0851","1936-086X"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","doyens","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Nano","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5002535975","display_name":"Tongde Wang","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I116953780","display_name":"Tongji University","ror":"https://ror.org/03rc6as71","country_code":"CN","type":"education","lineage":["https://openalex.org/I116953780"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Tongde Wang","raw_affiliation_strings":["Tongji University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Tongji University , , ,","institution_ids":["https://openalex.org/I116953780"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5133087191","display_name":"Jiale Li","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I111599522","display_name":"Jiangnan University","ror":"https://ror.org/04mkzax54","country_code":"CN","type":"education","lineage":["https://openalex.org/I111599522"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Jiale Li","raw_affiliation_strings":["Jiangnan University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Jiangnan University , , ,","institution_ids":["https://openalex.org/I111599522"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5160525565","display_name":"Xiuyan Quan","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I116953780","display_name":"Tongji University","ror":"https://ror.org/03rc6as71","country_code":"CN","type":"education","lineage":["https://openalex.org/I116953780"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Xiuyan Quan","raw_affiliation_strings":["Tongji University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Tongji University , , ,","institution_ids":["https://openalex.org/I116953780"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5160498586","display_name":"Lele Liu","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I111599522","display_name":"Jiangnan University","ror":"https://ror.org/04mkzax54","country_code":"CN","type":"education","lineage":["https://openalex.org/I111599522"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Lele Liu","raw_affiliation_strings":["Jiangnan University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Jiangnan University , , ,","institution_ids":["https://openalex.org/I111599522"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5001042698","display_name":"Guohua Gao","orcid":"https://orcid.org/0000-0002-4233-5357","observed_orcids":["https://orcid.org/0000-0002-4233-5357"]},"institutions":[{"id":"https://openalex.org/I116953780","display_name":"Tongji University","ror":"https://ror.org/03rc6as71","country_code":"CN","type":"education","lineage":["https://openalex.org/I116953780"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Guohua Gao","raw_affiliation_strings":["Tongji University , , ,"],"raw_orcid":"https://orcid.org/0000-0002-4233-5357","affiliations":[{"raw_affiliation_string":"Tongji University , , ,","institution_ids":["https://openalex.org/I116953780"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5153330593","display_name":"Chanyuan Jin","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I4210095659","display_name":"Peking University School and Hospital of Stomatology","ror":"https://ror.org/00s2xkh70","country_code":"CN","type":"healthcare","lineage":["https://openalex.org/I4210095659"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Chanyuan Jin","raw_affiliation_strings":["Peking University School and Hospital of Stomatology & National Center for Stomatology & National Engineering Research Center of Oral Biomaterials and Digital Medical Devices , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Peking University School and Hospital of Stomatology & National Center for Stomatology & National Engineering Research Center of Oral Biomaterials and Digital Medical Devices , ,","institution_ids":["https://openalex.org/I4210095659"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5014327956","display_name":"Han Zhu","orcid":"https://orcid.org/0000-0002-6274-852X","observed_orcids":["https://orcid.org/0000-0002-6274-852X"]},"institutions":[{"id":"https://openalex.org/I111599522","display_name":"Jiangnan University","ror":"https://ror.org/04mkzax54","country_code":"CN","type":"education","lineage":["https://openalex.org/I111599522"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Han Zhu","raw_affiliation_strings":["Jiangnan University , , ,"],"raw_orcid":"https://orcid.org/0000-0002-6274-852X","affiliations":[{"raw_affiliation_string":"Jiangnan University , , ,","institution_ids":["https://openalex.org/I111599522"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5128765176","display_name":"Guangming Wu","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I116953780","display_name":"Tongji University","ror":"https://ror.org/03rc6as71","country_code":"CN","type":"education","lineage":["https://openalex.org/I116953780"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Guangming Wu","raw_affiliation_strings":["Tongji University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Tongji University , , ,","institution_ids":["https://openalex.org/I116953780"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":3,"corresponding_author_ids":["https://openalex.org/A5001042698","https://openalex.org/A5014327956","https://openalex.org/A5128765176","https://openalex.org/A5153330593"],"corresponding_institution_ids":["https://openalex.org/I111599522","https://openalex.org/I116953780","https://openalex.org/I4210095659"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":0.0,"has_fulltext":false,"cited_by_count":0,"citation_normalized_percentile":{"value":0.64834461,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9994999766349792,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9994999766349792,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10811","display_name":"Hydrogen Storage and Materials","score":9.999999747378752e-05,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11143","display_name":"High Entropy Alloys Studies","score":0.0,"subfield":{"id":"https://openalex.org/subfields/2210","display_name":"Mechanical Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/hydrogen-evolution-reaction","display_name":"hydrogen evolution reaction","score":0.9570000171661377},{"id":"https://openalex.org/keywords/high-entropy-alloys","display_name":"high-entropy alloys","score":0.746999979019165},{"id":"https://openalex.org/keywords/carbon-nanofibers","display_name":"carbon nanofibers","score":0.9850000143051147},{"id":"https://openalex.org/keywords/electronic-reconstruction","display_name":"electronic reconstruction","score":0.9070000052452087},{"id":"https://openalex.org/keywords/anion-exchange-membrane-water-electrolyzer","display_name":"anion exchange membrane water electrolyzer","score":0.8560000061988831},{"id":"https://openalex.org/keywords/electrocatalysis","display_name":"electrocatalysis","score":0.6520000100135803}],"concepts":[{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.714900016784668},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.6022999882698059},{"id":"https://openalex.org/C2780026712","wikidata":"https://www.wikidata.org/wiki/Q37756","display_name":"Alloy","level":2,"score":0.5809999704360962},{"id":"https://openalex.org/C102931765","wikidata":"https://www.wikidata.org/wiki/Q189673","display_name":"Dissociation (chemistry)","level":2,"score":0.5807999968528748},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.5418999791145325},{"id":"https://openalex.org/C162711632","wikidata":"https://www.wikidata.org/wiki/Q905514","display_name":"Desorption","level":3,"score":0.5389000177383423},{"id":"https://openalex.org/C150394285","wikidata":"https://www.wikidata.org/wiki/Q180254","display_name":"Adsorption","level":2,"score":0.5277000069618225},{"id":"https://openalex.org/C152365726","wikidata":"https://www.wikidata.org/wiki/Q1048589","display_name":"Density functional theory","level":2,"score":0.4932999908924103},{"id":"https://openalex.org/C512968161","wikidata":"https://www.wikidata.org/wiki/Q556","display_name":"Hydrogen","level":2,"score":0.46889999508857727},{"id":"https://openalex.org/C49110097","wikidata":"https://www.wikidata.org/wiki/Q175233","display_name":"Cathode","level":2,"score":0.44110000133514404},{"id":"https://openalex.org/C179104552","wikidata":"https://www.wikidata.org/wiki/Q11165","display_name":"Inorganic chemistry","level":1,"score":0.41990000009536743},{"id":"https://openalex.org/C35590869","wikidata":"https://www.wikidata.org/wiki/Q2697332","display_name":"Water splitting","level":4,"score":0.3522999882698059},{"id":"https://openalex.org/C48256821","wikidata":"https://www.wikidata.org/wiki/Q903456","display_name":"Electrolysis of water","level":5,"score":0.3517000079154968},{"id":"https://openalex.org/C2780443040","wikidata":"https://www.wikidata.org/wiki/Q3737863","display_name":"Bifunctional","level":3,"score":0.35109999775886536},{"id":"https://openalex.org/C2775896084","wikidata":"https://www.wikidata.org/wiki/Q425597","display_name":"Hydroxide","level":2,"score":0.34220001101493835},{"id":"https://openalex.org/C55904794","wikidata":"https://www.wikidata.org/wiki/Q82682","display_name":"Redox","level":2,"score":0.3402000069618225},{"id":"https://openalex.org/C177367955","wikidata":"https://www.wikidata.org/wiki/Q4468924","display_name":"Carbon nanofiber","level":3,"score":0.33410000801086426},{"id":"https://openalex.org/C155672457","wikidata":"https://www.wikidata.org/wiki/Q61231","display_name":"Nanoparticle","level":2,"score":0.32280001044273376},{"id":"https://openalex.org/C89395315","wikidata":"https://www.wikidata.org/wiki/Q181232","display_name":"Anode","level":3,"score":0.3091999888420105},{"id":"https://openalex.org/C163127949","wikidata":"https://www.wikidata.org/wiki/Q64403","display_name":"Electrolysis","level":4,"score":0.2935999929904938},{"id":"https://openalex.org/C68044625","wikidata":"https://www.wikidata.org/wiki/Q1203442","display_name":"Hydrogen storage","level":3,"score":0.28999999165534973},{"id":"https://openalex.org/C198091228","wikidata":"https://www.wikidata.org/wiki/Q19557","display_name":"Alkali metal","level":2,"score":0.2777999937534332},{"id":"https://openalex.org/C202189072","wikidata":"https://www.wikidata.org/wiki/Q1929999","display_name":"Hydrogen production","level":3,"score":0.2773999869823456},{"id":"https://openalex.org/C140205800","wikidata":"https://www.wikidata.org/wiki/Q5860","display_name":"Carbon fibers","level":3,"score":0.27379998564720154},{"id":"https://openalex.org/C86025842","wikidata":"https://www.wikidata.org/wiki/Q5358432","display_name":"Electronic structure","level":2,"score":0.27000001072883606},{"id":"https://openalex.org/C32891209","wikidata":"https://www.wikidata.org/wiki/Q483666","display_name":"Spectroscopy","level":2,"score":0.257999986410141},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.2565000057220459},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.2524000108242035}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.1021/acsnano.6c17609","doi":"https://doi.org/10.1021/acsnano.6c17609","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsnano.6c17609","pdf_url":null,"source":{"id":"https://openalex.org/S145476921","display_name":"ACS Nano","issn_l":"1936-0851","issn":["1936-0851","1936-086X"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","doyens","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Nano","raw_type":"journal-article"}],"best_oa_location":null,"sustainable_development_goals":[{"display_name":"Affordable and clean energy","score":0.9853000044822693,"id":"https://metadata.un.org/sdg/7"}],"study_designs":[],"awards":[],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":57,"referenced_works":["https://openalex.org/W2346817778","https://openalex.org/W3208084272","https://openalex.org/W4205719490","https://openalex.org/W4210611825","https://openalex.org/W4280561292","https://openalex.org/W4291285610","https://openalex.org/W4311664023","https://openalex.org/W4313551473","https://openalex.org/W4313656748","https://openalex.org/W4382795539","https://openalex.org/W4384938716","https://openalex.org/W4386304401","https://openalex.org/W4387223609","https://openalex.org/W4388287953","https://openalex.org/W4390670670","https://openalex.org/W4390683852","https://openalex.org/W4391718332","https://openalex.org/W4391778484","https://openalex.org/W4392658994","https://openalex.org/W4393866085","https://openalex.org/W4394815022","https://openalex.org/W4396674745","https://openalex.org/W4398177340","https://openalex.org/W4399435678","https://openalex.org/W4400977020","https://openalex.org/W4401277047","https://openalex.org/W4401652842","https://openalex.org/W4403519944","https://openalex.org/W4404029055","https://openalex.org/W4404114967","https://openalex.org/W4404838431","https://openalex.org/W4405260572","https://openalex.org/W4406062946","https://openalex.org/W4406597965","https://openalex.org/W4407319746","https://openalex.org/W4408719457","https://openalex.org/W4409122540","https://openalex.org/W4410077898","https://openalex.org/W4410487488","https://openalex.org/W4410566567","https://openalex.org/W4410616615","https://openalex.org/W4410748016","https://openalex.org/W4411134091","https://openalex.org/W4412188113","https://openalex.org/W4412601249","https://openalex.org/W4412711088","https://openalex.org/W4414149245","https://openalex.org/W4414415649","https://openalex.org/W4414543735","https://openalex.org/W4415649680","https://openalex.org/W4416388700","https://openalex.org/W4416827390","https://openalex.org/W7082993076","https://openalex.org/W7117459202","https://openalex.org/W7122686863","https://openalex.org/W7123345159","https://openalex.org/W7134285504"],"related_works":["https://openalex.org/W7154513535","https://openalex.org/W3113658169","https://openalex.org/W4412845096","https://openalex.org/W3165565733","https://openalex.org/W4394578575","https://openalex.org/W2810452996","https://openalex.org/W4412818028","https://openalex.org/W7167619261","https://openalex.org/W4413991879","https://openalex.org/W3109602832"],"abstract_inverted_index":{"Abstract":[0],"Efficient":[1],"hydrogen":[2],"evolution":[3],"reaction":[4],"(HER)":[5],"in":[6,149],"acidic":[7,125,189],"and":[8,20,64,78,90,141,153,190],"alkaline":[9,94,191],"media":[10],"requires":[11,138],"distinct":[12],"catalytic":[13,31],"functions,":[14],"including":[15],"H2O":[16,88,102],"activation,":[17],"*H":[18],"adsorption/desorption":[19,122],"*OH":[21,91],"regulation,":[22],"which":[23],"are":[24,43],"difficult":[25],"to":[26,49,144],"integrate":[27],"within":[28,195],"a":[29,51,60,100,128,185],"single":[30],"surface.":[32,55,199],"Herein,":[33],"PtNiRuFeW":[34],"high-entropy":[35,57,182],"alloy":[36,198],"nanoparticles":[37],"anchored":[38],"on":[39],"carbon":[40],"nanofibers":[41],"(PtNiRuFeW/CNFs)":[42],"constructed":[44],"through":[45],"electrospinning-assisted":[46],"carbothermal":[47],"reduction":[48],"create":[50],"continuous":[52,197],"site-differentiated":[53,181],"multicomponent":[54],"The":[56,136],"configuration":[58],"induces":[59],"broad":[61],"d-state":[62],"distribution":[63],"pronounced":[65],"electronic":[66],"reconstruction,":[67],"generating":[68],"element-dependent":[69],"adsorption":[70],"environments":[71],"for":[72,175,187],"HER":[73,192],"intermediates.":[74],"In":[75],"situ":[76],"spectroscopy":[77],"density":[79],"functional":[80],"theory":[81],"calculations":[82],"reveal":[83],"that":[84],"Fe/Ni-associated":[85],"sites":[86,98,109,118],"promote":[87],"activation":[89],"stabilization":[92],"during":[93],"HER,":[95],"with":[96],"Fe":[97],"exhibiting":[99],"low":[101,129],"dissociation":[103],"barrier":[104,132],"of":[105,133],"0.08":[106],"eV.":[107,135],"Ru-associated":[108],"preferentially":[110],"accommodate":[111],"H*":[112,121,130],"intermediates,":[113],"while":[114],"electronically":[115],"reconstructed":[116],"Pt":[117],"optimize":[119],"the":[120,166],"balance":[123],"under":[124],"conditions,":[126],"giving":[127],"desorption":[131],"0.22":[134],"PtNiRuFeW/CNFs":[137,164],"only":[139],"45":[140],"90":[142],"mV":[143],"reach":[145],"100":[146],"mA":[147,173],"cm\u20132":[148,174],"1.0":[150],"M":[151,155],"KOH":[152],"0.5":[154],"H2SO4,":[156],"respectively.":[157],"Moreover,":[158],"an":[159],"anion-exchange-membrane":[160],"water":[161],"electrolyzer":[162],"using":[163],"as":[165,184],"cathode":[167],"maintains":[168],"stable":[169],"operation":[170],"at":[171],"500":[172],"470":[176],"h.":[177],"This":[178],"work":[179],"establishes":[180],"catalysis":[183],"strategy":[186],"coupling":[188],"elementary":[193],"steps":[194],"one":[196]},"counts_by_year":[],"updated_date":"2026-11-05T12:25:35.769452","created_date":"2026-11-04T00:00:00"}
