{"id":"https://openalex.org/W7207865490","doi":"https://doi.org/10.1021/jacs.6c10274","title":"Programmable Organic Quasi-Superlattices with Molecular-Monolayer Precision for Enhanced Photoconductive Response","display_name":"Programmable Organic Quasi-Superlattices with Molecular-Monolayer Precision for Enhanced Photoconductive Response","publication_year":2026,"publication_date":"2026-09-02","ids":{"openalex":"https://openalex.org/W7207865490","doi":"https://doi.org/10.1021/jacs.6c10274","pmid":"https://pubmed.ncbi.nlm.nih.gov/42915538"},"language":"en","primary_location":{"id":"doi:10.1021/jacs.6c10274","doi":"https://doi.org/10.1021/jacs.6c10274","is_oa":false,"landing_page_url":"https://doi.org/10.1021/jacs.6c10274","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5100463013","display_name":"Wenbin Li","orcid":"https://orcid.org/0000-0003-2317-601X","observed_orcids":["https://orcid.org/0000-0003-2317-601X"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Wenbin Li","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5149654564","display_name":"Xin Wang","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Xin Wang","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5016370328","display_name":"Zhumin Yu","orcid":"https://orcid.org/0009-0000-3188-3078","observed_orcids":["https://orcid.org/0009-0000-3188-3078"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Zhumin Yu","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5149469968","display_name":"Jun Li","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Jun Li","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5149931657","display_name":"Ming Li","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Ming Li","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5068418594","display_name":"Baichuan Jiang","orcid":"https://orcid.org/0009-0002-3883-4003","observed_orcids":["https://orcid.org/0009-0002-3883-4003"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Baichuan Jiang","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5040790080","display_name":"Cailing Ou","orcid":"https://orcid.org/0009-0004-0152-2203","observed_orcids":["https://orcid.org/0009-0004-0152-2203"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Cailing Ou","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5034835168","display_name":"Tingyu Ji","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Tingyu Ji","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5093761910","display_name":"Nannan Dou","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Nannan Dou","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5032913611","display_name":"Xiaoru Cao","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Xiaoru Cao","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5028019331","display_name":"Zixiao Han","orcid":"https://orcid.org/0009-0003-2152-0363","observed_orcids":["https://orcid.org/0009-0003-2152-0363"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Zixiao Han","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5100772014","display_name":"Lei Zhang","orcid":"https://orcid.org/0000-0003-1237-3229","observed_orcids":["https://orcid.org/0000-0003-1237-3229","https://orcid.org/0000-0002-0162-7222"]},"institutions":[{"id":"https://openalex.org/I881766915","display_name":"Nanjing University","ror":"https://ror.org/01rxvg760","country_code":"CN","type":"education","lineage":["https://openalex.org/I881766915"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Lei Zhang","raw_affiliation_strings":["Nanjing University , , ,"],"raw_orcid":"https://orcid.org/0000-0003-1237-3229","affiliations":[{"raw_affiliation_string":"Nanjing University , , ,","institution_ids":["https://openalex.org/I881766915"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":1,"corresponding_author_ids":["https://openalex.org/A5100772014"],"corresponding_institution_ids":["https://openalex.org/I881766915"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":0.0,"has_fulltext":false,"cited_by_count":0,"citation_normalized_percentile":{"value":0.0,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":null,"biblio":{"volume":"148","issue":"36","first_page":"38904","last_page":"38912"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10045","display_name":"Organic Electronics and Photovoltaics","score":0.9442999958992004,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10045","display_name":"Organic Electronics and Photovoltaics","score":0.9442999958992004,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10275","display_name":"2D Materials and Applications","score":0.037700001150369644,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10913","display_name":"Molecular Junctions and Nanostructures","score":0.0044999998062849045,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/van-der-waals-heterostructures","display_name":"van der Waals heterostructures","score":0.8989999890327454},{"id":"https://openalex.org/keywords/polymer-semiconductors","display_name":"semiconducting polymers","score":0.9369999766349792},{"id":"https://openalex.org/keywords/photoconductive-response","display_name":"photoconductive response","score":0.8159999847412109},{"id":"https://openalex.org/keywords/near-infrared-detection","display_name":"near-infrared photodetection","score":0.75},{"id":"https://openalex.org/keywords/dark-current-suppression","display_name":"dark current reduction","score":0.5979999899864197},{"id":"https://openalex.org/keywords/optoelectronic-devices","display_name":"optoelectronic devices","score":0.6290000081062317}],"concepts":[{"id":"https://openalex.org/C7070889","wikidata":"https://www.wikidata.org/wiki/Q902488","display_name":"Monolayer","level":2,"score":0.8090000152587891},{"id":"https://openalex.org/C201999631","wikidata":"https://www.wikidata.org/wiki/Q2601129","display_name":"Photoconductivity","level":2,"score":0.6556000113487244},{"id":"https://openalex.org/C49040817","wikidata":"https://www.wikidata.org/wiki/Q193091","display_name":"Optoelectronics","level":1,"score":0.6155999898910522},{"id":"https://openalex.org/C79794668","wikidata":"https://www.wikidata.org/wiki/Q1616270","display_name":"Heterojunction","level":2,"score":0.6134999990463257},{"id":"https://openalex.org/C94003879","wikidata":"https://www.wikidata.org/wiki/Q1933714","display_name":"Organic semiconductor","level":2,"score":0.5666999816894531},{"id":"https://openalex.org/C120398109","wikidata":"https://www.wikidata.org/wiki/Q175751","display_name":"Quantum tunnelling","level":2,"score":0.5586000084877014},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.5200999975204468},{"id":"https://openalex.org/C126061179","wikidata":"https://www.wikidata.org/wiki/Q189627","display_name":"van der Waals force","level":3,"score":0.4871000051498413},{"id":"https://openalex.org/C105382558","wikidata":"https://www.wikidata.org/wiki/Q332431","display_name":"Superlattice","level":2,"score":0.4106000065803528},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.40720000863075256},{"id":"https://openalex.org/C108225325","wikidata":"https://www.wikidata.org/wiki/Q11456","display_name":"Semiconductor","level":2,"score":0.39410001039505005},{"id":"https://openalex.org/C123057669","wikidata":"https://www.wikidata.org/wiki/Q899903","display_name":"Molecular electronics","level":3,"score":0.33480000495910645},{"id":"https://openalex.org/C57410435","wikidata":"https://www.wikidata.org/wiki/Q505668","display_name":"Chemical vapor deposition","level":2,"score":0.3296000063419342},{"id":"https://openalex.org/C64297162","wikidata":"https://www.wikidata.org/wiki/Q1987070","display_name":"Deposition (geology)","level":3,"score":0.32850000262260437},{"id":"https://openalex.org/C113843644","wikidata":"https://www.wikidata.org/wiki/Q901882","display_name":"Interface (matter)","level":4,"score":0.31130000948905945},{"id":"https://openalex.org/C188082385","wikidata":"https://www.wikidata.org/wiki/Q73792","display_name":"Charge (physics)","level":2,"score":0.2782000005245209},{"id":"https://openalex.org/C2776873873","wikidata":"https://www.wikidata.org/wiki/Q3044964","display_name":"Vacuum deposition","level":3,"score":0.27149999141693115},{"id":"https://openalex.org/C2984497647","wikidata":"https://www.wikidata.org/wiki/Q174211","display_name":"Organic molecules","level":3,"score":0.2531999945640564}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/jacs.6c10274","doi":"https://doi.org/10.1021/jacs.6c10274","is_oa":false,"landing_page_url":"https://doi.org/10.1021/jacs.6c10274","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},{"id":"pmid:42915538","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/42915538","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"}],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":53,"referenced_works":["https://openalex.org/W1969531391","https://openalex.org/W1977380830","https://openalex.org/W1996766314","https://openalex.org/W2011141615","https://openalex.org/W2072333615","https://openalex.org/W2089335743","https://openalex.org/W2090908091","https://openalex.org/W2091691688","https://openalex.org/W2169082874","https://openalex.org/W2280957227","https://openalex.org/W2481949062","https://openalex.org/W2520615830","https://openalex.org/W2562620655","https://openalex.org/W2775441595","https://openalex.org/W2781698763","https://openalex.org/W2786378589","https://openalex.org/W2795196444","https://openalex.org/W2868606376","https://openalex.org/W2925217409","https://openalex.org/W2987219171","https://openalex.org/W3115028708","https://openalex.org/W3120888287","https://openalex.org/W3124257166","https://openalex.org/W3161611462","https://openalex.org/W3161785433","https://openalex.org/W3207358030","https://openalex.org/W4212902471","https://openalex.org/W4280560762","https://openalex.org/W4289653643","https://openalex.org/W4360612048","https://openalex.org/W4387803846","https://openalex.org/W4388203953","https://openalex.org/W4391558313","https://openalex.org/W4392241436","https://openalex.org/W4396237838","https://openalex.org/W4400188938","https://openalex.org/W4400659836","https://openalex.org/W4400959459","https://openalex.org/W4401393427","https://openalex.org/W4401549719","https://openalex.org/W4401993266","https://openalex.org/W4405860513","https://openalex.org/W4407901409","https://openalex.org/W4408320882","https://openalex.org/W4409406475","https://openalex.org/W4409507710","https://openalex.org/W4412412664","https://openalex.org/W4414024122","https://openalex.org/W4414795277","https://openalex.org/W4414959484","https://openalex.org/W4415370270","https://openalex.org/W4415590012","https://openalex.org/W4417076179"],"related_works":["https://openalex.org/W1976169875","https://openalex.org/W7167625400","https://openalex.org/W7222397672","https://openalex.org/W2028950524","https://openalex.org/W4321266259","https://openalex.org/W2054581554","https://openalex.org/W74975144","https://openalex.org/W4405614893","https://openalex.org/W2397075529","https://openalex.org/W2331893389"],"abstract_inverted_index":{"Engineering":[0],"van":[1],"der":[2],"Waals":[3],"organic":[4,47,178],"heterostructures":[5],"with":[6,58,71,111],"monolayer":[7,56],"precision":[8],"offers":[9],"a":[10,132,140,161],"powerful":[11],"route":[12],"to":[13,30,65,103],"modulate":[14],"charge":[15],"transport":[16],"and":[17,34,84,139],"light-matter":[18],"interactions":[19],"in":[20],"molecular":[21,158],"systems.":[22],"However,":[23],"deterministic":[24],"multilayer":[25,179],"assembly":[26,57,176],"remains":[27],"challenging":[28],"due":[29],"pervasive":[31],"interlayer":[32],"interdiffusion":[33],"the":[35,51,77,81,85,88,118,174],"lack":[36],"of":[37,53,79,87,101,120,134,143,177],"generally":[38],"applicable":[39],"high-precision":[40],"deposition":[41],"strategies.":[42],"Here,":[43],"we":[44],"introduce":[45],"programmable":[46,157],"quasi-superlattices":[48,92],"enabled":[49],"by":[50],"integration":[52],"air-water":[54],"interfacial":[55],"sequential":[59],"transfer":[60],"stacking,":[61],"allowing":[62],"polymeric":[63],"semiconductors":[64],"be":[66],"organized":[67],"into":[68],"periodic":[69],"architectures":[70],"molecular-layer":[72],"precision.":[73],"By":[74],"systematically":[75],"tuning":[76],"number":[78],"periods,":[80],"intraperiod":[82],"composition,":[83],"thickness":[86],"tunneling":[89],"spacers,":[90],"these":[91],"exhibit":[93],"markedly":[94],"enhanced":[95],"photoconductive":[96],"performance,":[97],"achieving":[98],"signal-to-noise":[99],"ratios":[100],"up":[102],"2":[104],"\u00d7":[105,136],"106":[106],"under":[107,148],"white-light":[108],"illumination":[109,150],"together":[110],"an":[112],"ultralow":[113,149],"dark":[114],"current":[115],"density":[116],"on":[117],"order":[119],"10-10-10-11":[121],"A":[122],"cm-2.":[123],"Superlattices":[124],"optimized":[125],"for":[126,164],"near-infrared":[127],"detection":[128],"(900":[129],"nm)":[130],"achieve":[131],"detectivity":[133],"2.06":[135],"1012":[137],"Jones":[138],"photoresponse":[141],"time":[142],"less":[144],"than":[145],"0.2":[146],"s":[147],"(21":[151],"\u03bcW":[152],"cm-2).":[153],"These":[154],"findings":[155],"establish":[156],"organization":[159],"as":[160],"general":[162],"strategy":[163],"accessing":[165],"emergent":[166],"optoelectronic":[167],"functionality":[168],"from":[169],"vast":[170],"chemical":[171],"spaces":[172],"via":[173],"controlled":[175],"architectures.":[180]},"counts_by_year":[],"updated_date":"2026-11-08T12:12:28.789561","created_date":"2026-09-04T00:00:00"}