{"id":"https://openalex.org/W7123493261","doi":"https://doi.org/10.1038/s41467-026-68386-4","title":"Efficient and stable catalytic hydrolysis of perfluorocarbon enabled by SO2-mediated proton supply","display_name":"Efficient and stable catalytic hydrolysis of perfluorocarbon enabled by SO2-mediated proton supply","publication_year":2026,"publication_date":"2026-01-14","ids":{"openalex":"https://openalex.org/W7123493261","doi":"https://doi.org/10.1038/s41467-026-68386-4","pmid":"https://pubmed.ncbi.nlm.nih.gov/41535297"},"language":"en","primary_location":{"id":"doi:10.1038/s41467-026-68386-4","doi":"https://doi.org/10.1038/s41467-026-68386-4","is_oa":true,"landing_page_url":"https://doi.org/10.1038/s41467-026-68386-4","pdf_url":"https://www.nature.com/articles/s41467-026-68386-4_reference.pdf","source":{"id":"https://openalex.org/S64187185","display_name":"Nature Communications","issn_l":"2041-1723","issn":["2041-1723"],"is_oa":true,"is_in_doaj":true,"is_core":true,"listed_in":["anvur-class-a","anvur-scientific","cwts-core","doaj","dongbi-a","doyens","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nature Communications","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["crossref","doaj","pubmed"],"open_access":{"is_oa":true,"oa_status":"gold","oa_url":"https://www.nature.com/articles/s41467-026-68386-4_reference.pdf","any_repository_has_fulltext":true},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5122977266","display_name":"Hang Zhang","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]},{"id":"https://openalex.org/I8204097","display_name":"Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen","ror":"https://ror.org/05591te55","country_code":"DE","type":"education","lineage":["https://openalex.org/I8204097"]}],"countries":["CN","DE"],"is_corresponding":false,"raw_author_name":"Hang Zhang","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]},{"raw_affiliation_string":"Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany","institution_ids":["https://openalex.org/I8204097"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5122953801","display_name":"Tao Luo","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]},{"id":"https://openalex.org/I169541294","display_name":"Flinders University","ror":"https://ror.org/01kpzv902","country_code":"AU","type":"education","lineage":["https://openalex.org/I169541294"]}],"countries":["AU","CN"],"is_corresponding":false,"raw_author_name":"Tao Luo","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","Institute for Nanoscale Science & Technology, Flinders University, Bedford Park, SA, Australia"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]},{"raw_affiliation_string":"Institute for Nanoscale Science & Technology, Flinders University, Bedford Park, SA, Australia","institution_ids":["https://openalex.org/I169541294"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5122965253","display_name":"Yingkang Chen","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Yingkang Chen","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5073834787","display_name":"Xiaojian Wang","orcid":"https://orcid.org/0009-0000-6819-0160","observed_orcids":["https://orcid.org/0009-0000-6819-0160"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Xiaojian Wang","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5122926498","display_name":"Edoardo Mariani","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I8204097","display_name":"Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen","ror":"https://ror.org/05591te55","country_code":"DE","type":"education","lineage":["https://openalex.org/I8204097"]}],"countries":["DE"],"is_corresponding":false,"raw_author_name":"Edoardo Mariani","raw_affiliation_strings":["Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany","institution_ids":["https://openalex.org/I8204097"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5100389896","display_name":"Kang Liu","orcid":"https://orcid.org/0000-0002-3436-7850","observed_orcids":["https://orcid.org/0000-0002-3436-7850","https://orcid.org/0000-0002-3150-0185"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Kang Liu","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5122928634","display_name":"Junwei Fu","orcid":"https://orcid.org/0000-0003-0190-1663","observed_orcids":["https://orcid.org/0000-0003-0190-1663"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Junwei Fu","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China"],"raw_orcid":"https://orcid.org/0000-0003-0190-1663","affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5122930042","display_name":"Changxu Liu","orcid":"https://orcid.org/0000-0003-1196-7447","observed_orcids":["https://orcid.org/0000-0003-1196-7447"]},"institutions":[{"id":"https://openalex.org/I23923803","display_name":"University of Exeter","ror":"https://ror.org/03yghzc09","country_code":"GB","type":"education","lineage":["https://openalex.org/I23923803"]}],"countries":["GB"],"is_corresponding":false,"raw_author_name":"Changxu Liu","raw_affiliation_strings":["Centre for Metamaterial Research & Innovation, Department of Engineering, University of Exeter, Exeter, United Kingdom"],"raw_orcid":"https://orcid.org/0000-0003-1196-7447","affiliations":[{"raw_affiliation_string":"Centre for Metamaterial Research & Innovation, Department of Engineering, University of Exeter, Exeter, United Kingdom","institution_ids":["https://openalex.org/I23923803"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5100387656","display_name":"Hui Liu","orcid":"https://orcid.org/0000-0003-2693-2546","observed_orcids":["https://orcid.org/0000-0003-2693-2546","https://orcid.org/0000-0001-8183-9446","https://orcid.org/0000-0002-1080-0883"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Hui Liu","raw_affiliation_strings":["School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5100628318","display_name":"Zhang Lin","orcid":"https://orcid.org/0000-0002-6600-2055","observed_orcids":["https://orcid.org/0000-0002-6600-2055","https://orcid.org/0009-0004-0817-8134"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Zhang Lin","raw_affiliation_strings":["School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China"],"raw_orcid":"https://orcid.org/0000-0002-6600-2055","affiliations":[{"raw_affiliation_string":"School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5079893090","display_name":"Liyuan Chai","orcid":"https://orcid.org/0000-0001-8641-9774","observed_orcids":["https://orcid.org/0000-0001-8641-9774"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Liyuan Chai","raw_affiliation_strings":["School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China","institution_ids":["https://openalex.org/I139660479"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5083158068","display_name":"Michelle L. Coote","orcid":"https://orcid.org/0000-0003-0828-7053","observed_orcids":["https://orcid.org/0000-0003-0828-7053"]},"institutions":[{"id":"https://openalex.org/I169541294","display_name":"Flinders University","ror":"https://ror.org/01kpzv902","country_code":"AU","type":"education","lineage":["https://openalex.org/I169541294"]}],"countries":["AU"],"is_corresponding":false,"raw_author_name":"Michelle L. Coote","raw_affiliation_strings":["Institute for Nanoscale Science & Technology, Flinders University, Bedford Park, SA, Australia"],"raw_orcid":"https://orcid.org/0000-0003-0828-7053","affiliations":[{"raw_affiliation_string":"Institute for Nanoscale Science & Technology, Flinders University, Bedford Park, SA, Australia","institution_ids":["https://openalex.org/I169541294"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5049936709","display_name":"Emiliano Cort\u00e9s","orcid":"https://orcid.org/0000-0001-8248-4165","observed_orcids":["https://orcid.org/0000-0001-8248-4165"]},"institutions":[{"id":"https://openalex.org/I8204097","display_name":"Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen","ror":"https://ror.org/05591te55","country_code":"DE","type":"education","lineage":["https://openalex.org/I8204097"]}],"countries":["DE"],"is_corresponding":true,"raw_author_name":"Emiliano Cort\u00e9s","raw_affiliation_strings":["Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany. Emiliano.Cortes@lmu.de"],"raw_orcid":"https://orcid.org/0000-0001-8248-4165","affiliations":[{"raw_affiliation_string":"Nanoinstitut M\u00fcnchen, Fakult\u00e4t f\u00fcr Physik, Ludwig-Maximilians-Universit\u00e4t M\u00fcnchen, M\u00fcnchen, Germany. Emiliano.Cortes@lmu.de","institution_ids":["https://openalex.org/I8204097"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5122921115","display_name":"Min Liu","orcid":"https://orcid.org/0000-0002-9007-4817","observed_orcids":["https://orcid.org/0000-0002-9007-4817"]},"institutions":[{"id":"https://openalex.org/I139660479","display_name":"Central South University","ror":"https://ror.org/00f1zfq44","country_code":"CN","type":"education","lineage":["https://openalex.org/I139660479"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Min Liu","raw_affiliation_strings":["Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China. minliu@csu.edu.cn","School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China. minliu@csu.edu.cn"],"raw_orcid":"https://orcid.org/0000-0002-9007-4817","affiliations":[{"raw_affiliation_string":"Hunan Joint International Research Center for Carbon Dioxide Resource Utilization, School of Physics, Central South University, Changsha, Hunan, PR China. minliu@csu.edu.cn","institution_ids":["https://openalex.org/I139660479"]},{"raw_affiliation_string":"School of Metallurgy and Environment, Central South University, Changsha, Hunan, PR China. minliu@csu.edu.cn","institution_ids":["https://openalex.org/I139660479"]}]}],"institutions":[],"countries_distinct_count":4,"institutions_distinct_count":4,"corresponding_author_ids":["https://openalex.org/A5049936709","https://openalex.org/A5122921115"],"corresponding_institution_ids":["https://openalex.org/I139660479","https://openalex.org/I8204097"],"apc_list":{"value":6990,"currency":"USD","value_usd":6990},"apc_paid":{"value":6990,"currency":"USD","value_usd":6990},"fwci":19.6503,"has_fulltext":true,"cited_by_count":10,"citation_normalized_percentile":{"value":0.99492691,"is_in_top_1_percent":true,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":99,"max":100},"biblio":{"volume":"17","issue":"1","first_page":"597","last_page":"597"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T11869","display_name":"Per- and polyfluoroalkyl substances research","score":0.44510000944137573,"subfield":{"id":"https://openalex.org/subfields/2304","display_name":"Environmental Chemistry"},"field":{"id":"https://openalex.org/fields/23","display_name":"Environmental Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T11869","display_name":"Per- and polyfluoroalkyl substances research","score":0.44510000944137573,"subfield":{"id":"https://openalex.org/subfields/2304","display_name":"Environmental Chemistry"},"field":{"id":"https://openalex.org/fields/23","display_name":"Environmental Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T12646","display_name":"Inorganic Fluorides and Related Compounds","score":0.16189999878406525,"subfield":{"id":"https://openalex.org/subfields/1604","display_name":"Inorganic Chemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10192","display_name":"Catalytic Processes in Materials Science","score":0.09610000252723694,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/catalytic-hydrolysis","display_name":"catalytic hydrolysis","score":0.8740000128746033},{"id":"https://openalex.org/keywords/carbon-tetrafluoride","display_name":"carbon tetrafluoride","score":0.8709999918937683},{"id":"https://openalex.org/keywords/perfluorocarbons","display_name":"perfluorocarbons","score":0.7870000004768372},{"id":"https://openalex.org/keywords/pfas-degradation","display_name":"PFAS degradation","score":0.8370000123977661},{"id":"https://openalex.org/keywords/c-f-bond-activation","display_name":"C\u2013F bond activation","score":0.8479999899864197},{"id":"https://openalex.org/keywords/sulfur-dioxide","display_name":"sulfur dioxide","score":0.6919999718666077},{"id":"https://openalex.org/keywords/proton-supply","display_name":"proton supply","score":0.8870000243186951},{"id":"https://openalex.org/keywords/catalyst-stability","display_name":"catalyst stability","score":0.5929999947547913},{"id":"https://openalex.org/keywords/defluorination","display_name":"defluorination","score":0.7940000295639038},{"id":"https://openalex.org/keywords/active-site-regeneration","display_name":"active site regeneration","score":0.7049999833106995}],"concepts":[{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.8382999897003174},{"id":"https://openalex.org/C94412978","wikidata":"https://www.wikidata.org/wiki/Q103135","display_name":"Hydrolysis","level":2,"score":0.6733999848365784},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.6274999976158142},{"id":"https://openalex.org/C102931765","wikidata":"https://www.wikidata.org/wiki/Q189673","display_name":"Dissociation (chemistry)","level":2,"score":0.6068999767303467},{"id":"https://openalex.org/C54516573","wikidata":"https://www.wikidata.org/wiki/Q2294","display_name":"Proton","level":2,"score":0.6067000031471252},{"id":"https://openalex.org/C154256306","wikidata":"https://www.wikidata.org/wiki/Q41795528","display_name":"Inert","level":2,"score":0.573199987411499},{"id":"https://openalex.org/C124681953","wikidata":"https://www.wikidata.org/wiki/Q339062","display_name":"Decomposition","level":2,"score":0.4706999957561493},{"id":"https://openalex.org/C2779679103","wikidata":"https://www.wikidata.org/wiki/Q5251805","display_name":"Degradation (telecommunications)","level":2,"score":0.4693000018596649},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.446399986743927},{"id":"https://openalex.org/C21951064","wikidata":"https://www.wikidata.org/wiki/Q899212","display_name":"Combinatorial chemistry","level":1,"score":0.4065999984741211},{"id":"https://openalex.org/C18762648","wikidata":"https://www.wikidata.org/wiki/Q42213","display_name":"Work (physics)","level":2,"score":0.4041999876499176},{"id":"https://openalex.org/C3044715","wikidata":"https://www.wikidata.org/wiki/Q3952437","display_name":"Bond cleavage","level":3,"score":0.3409000039100647},{"id":"https://openalex.org/C95121573","wikidata":"https://www.wikidata.org/wiki/Q190474","display_name":"Activation energy","level":2,"score":0.3366999924182892},{"id":"https://openalex.org/C2777822432","wikidata":"https://www.wikidata.org/wiki/Q216681","display_name":"In situ","level":2,"score":0.32679998874664307},{"id":"https://openalex.org/C75473681","wikidata":"https://www.wikidata.org/wiki/Q188651","display_name":"Photochemistry","level":1,"score":0.31139999628067017},{"id":"https://openalex.org/C129652920","wikidata":"https://www.wikidata.org/wiki/Q17152746","display_name":"Synergistic catalysis","level":3,"score":0.3050000071525574},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.29589998722076416},{"id":"https://openalex.org/C32909587","wikidata":"https://www.wikidata.org/wiki/Q11369","display_name":"Molecule","level":2,"score":0.2930000126361847},{"id":"https://openalex.org/C148898269","wikidata":"https://www.wikidata.org/wiki/Q1108792","display_name":"Kinetics","level":2,"score":0.28529998660087585},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.274399995803833},{"id":"https://openalex.org/C175583648","wikidata":"https://www.wikidata.org/wiki/Q903156","display_name":"Heterogeneous catalysis","level":3,"score":0.2734000086784363},{"id":"https://openalex.org/C98045186","wikidata":"https://www.wikidata.org/wiki/Q205663","display_name":"Process (computing)","level":2,"score":0.2606000006198883},{"id":"https://openalex.org/C2985973956","wikidata":"https://www.wikidata.org/wiki/Q1617745","display_name":"High energy","level":2,"score":0.2515999972820282},{"id":"https://openalex.org/C65024703","wikidata":"https://www.wikidata.org/wiki/Q373406","display_name":"Reaction mechanism","level":3,"score":0.25130000710487366}],"mesh":[],"locations_count":4,"locations":[{"id":"doi:10.1038/s41467-026-68386-4","doi":"https://doi.org/10.1038/s41467-026-68386-4","is_oa":true,"landing_page_url":"https://doi.org/10.1038/s41467-026-68386-4","pdf_url":"https://www.nature.com/articles/s41467-026-68386-4_reference.pdf","source":{"id":"https://openalex.org/S64187185","display_name":"Nature Communications","issn_l":"2041-1723","issn":["2041-1723"],"is_oa":true,"is_in_doaj":true,"is_core":true,"listed_in":["anvur-class-a","anvur-scientific","cwts-core","doaj","dongbi-a","doyens","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nature Communications","raw_type":"journal-article"},{"id":"pmid:41535297","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/41535297","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nature communications","raw_type":"Journal Article"},{"id":"pmh:oai:doaj.org/article:0a4035ef957a41af979c72cb4f15666f","doi":null,"is_oa":true,"landing_page_url":"https://doaj.org/article/0a4035ef957a41af979c72cb4f15666f","pdf_url":null,"source":{"id":"https://openalex.org/S4306401280","display_name":"DOAJ (DOAJ: Directory of Open Access Journals)","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by-sa","license_id":"https://openalex.org/licenses/cc-by-sa","version":"submittedVersion","is_accepted":false,"is_published":false,"raw_source_name":"Nature Communications, Vol 17, Iss 1, Pp 1-9 (2026)","raw_type":"article"},{"id":"pmh:oai:pubmedcentral.nih.gov:12808091","doi":null,"is_oa":true,"landing_page_url":"https://pmc.ncbi.nlm.nih.gov/articles/PMC12808091/","pdf_url":null,"source":{"id":"https://openalex.org/S2764455111","display_name":"PubMed Central","issn_l":null,"issn":null,"is_oa":true,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"submittedVersion","is_accepted":false,"is_published":false,"raw_source_name":"Nat Commun","raw_type":"Text"}],"best_oa_location":{"id":"doi:10.1038/s41467-026-68386-4","doi":"https://doi.org/10.1038/s41467-026-68386-4","is_oa":true,"landing_page_url":"https://doi.org/10.1038/s41467-026-68386-4","pdf_url":"https://www.nature.com/articles/s41467-026-68386-4_reference.pdf","source":{"id":"https://openalex.org/S64187185","display_name":"Nature Communications","issn_l":"2041-1723","issn":["2041-1723"],"is_oa":true,"is_in_doaj":true,"is_core":true,"listed_in":["anvur-class-a","anvur-scientific","cwts-core","doaj","dongbi-a","doyens","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nature Communications","raw_type":"journal-article"},"sustainable_development_goals":[{"display_name":"Affordable and clean energy","id":"https://metadata.un.org/sdg/7","score":0.5690000057220459}],"sustainable_development_goals_aurora":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G1811448865","display_name":null,"funder_award_id":"52372253","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G2776590582","display_name":null,"funder_award_id":"22403108","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G4265792850","display_name":null,"funder_award_id":"22376222","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G715747571","display_name":null,"funder_award_id":"52121004","funder_id":"https://openalex.org/F4320327720","funder_display_name":"Foundation for Innovative Research Groups of the National Natural Science Foundation of China"},{"id":"https://openalex.org/G7865460087","display_name":null,"funder_award_id":"52121004","funder_id":"https://openalex.org/F4320321514","funder_display_name":"Central South University"},{"id":"https://openalex.org/G8414565904","display_name":null,"funder_award_id":"52121004","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"}],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"},{"id":"https://openalex.org/F4320321514","display_name":"Central South University","ror":"https://ror.org/00f1zfq44"},{"id":"https://openalex.org/F4320322725","display_name":"China Scholarship Council","ror":"https://ror.org/04atp4p48"},{"id":"https://openalex.org/F4320327720","display_name":"Foundation for Innovative Research Groups of the National Natural Science Foundation of China","ror":null}],"has_content":{"grobid_xml":true,"pdf":true},"content_urls":{"pdf":"https://content.openalex.org/works/W7123493261.pdf","grobid_xml":"https://content.openalex.org/works/W7123493261.grobid-xml"},"referenced_works_count":42,"referenced_works":["https://openalex.org/W1971208206","https://openalex.org/W2000969751","https://openalex.org/W2020544670","https://openalex.org/W2029478231","https://openalex.org/W2052853684","https://openalex.org/W2316765721","https://openalex.org/W2525274716","https://openalex.org/W2940828526","https://openalex.org/W2945334153","https://openalex.org/W2966517673","https://openalex.org/W3033113583","https://openalex.org/W3100685193","https://openalex.org/W3141985989","https://openalex.org/W3171517443","https://openalex.org/W3213227683","https://openalex.org/W4210721336","https://openalex.org/W4223914023","https://openalex.org/W4224300595","https://openalex.org/W4281294354","https://openalex.org/W4283312955","https://openalex.org/W4283817916","https://openalex.org/W4312205083","https://openalex.org/W4321435581","https://openalex.org/W4365444188","https://openalex.org/W4366603531","https://openalex.org/W4375948269","https://openalex.org/W4386279597","https://openalex.org/W4387755809","https://openalex.org/W4390562330","https://openalex.org/W4391886011","https://openalex.org/W4392356547","https://openalex.org/W4393974844","https://openalex.org/W4403915785","https://openalex.org/W4404566619","https://openalex.org/W4405333779","https://openalex.org/W4406268019","https://openalex.org/W4406399940","https://openalex.org/W4406633746","https://openalex.org/W4406893782","https://openalex.org/W4407136997","https://openalex.org/W4407744964","https://openalex.org/W4407750616"],"related_works":[],"abstract_inverted_index":{"Abstract":[0],"Catalytic":[1],"hydrolysis":[2],"is":[3],"an":[4,51],"effective":[5],"strategy":[6],"for":[7,91,129,139,148],"decomposing":[8],"tetrafluoromethane":[9],"(CF":[10],"4":[11,72,118],"),":[12],"one":[13],"of":[14,70,124,153],"the":[15,66,88,112,149],"most":[16],"chemically":[17],"inert":[18],"per-":[19],"and":[20,38,63,73,78,143],"polyfluoroalkyl":[21],"substances":[22],"(PFAS).":[23],"A":[24],"key":[25],"challenge":[26],"in":[27,31,67],"this":[28],"process":[29],"lies":[30],"enhancing":[32],"proton":[33,141],"availability":[34],"to":[35,56],"facilitate":[36],"efficient":[37],"stable":[39,127],"C\u2013F":[40,92],"bond":[41,93],"activation":[42,94],"while":[43],"ensuring":[44],"long-term":[45],"catalyst":[46,107,114],"stability.":[47],"Here":[48],"we":[49],"present":[50],"SO":[52],"2":[53,60],"-driven":[54],"approach":[55],"significantly":[57],"enhance":[58],"H":[59],"O":[61],"dissociation":[62],"proton-supplying":[64],"through":[65],"situ":[68],"formation":[69],"Al\u2013HSO":[71],"Ga\u2013HS":[74],"species.":[75],"Combined":[76],"experimental":[77],"theoretical":[79],"investigations":[80],"reveal":[81],"that":[82],"these":[83],"species":[84],"not":[85],"only":[86],"lower":[87],"energy":[89],"barrier":[90],"but":[95],"also":[96],"promote":[97],"active":[98],"site":[99],"regeneration":[100],"by":[101],"facilitating":[102],"defluorination,":[103],"thus":[104],"effectively":[105],"overcoming":[106],"deactivation.":[108],"As":[109],"a":[110,121,136,145],"result,":[111],"optimized":[113],"enables":[115],"complete":[116],"CF":[117],"decomposition":[119],"at":[120],"low":[122],"temperature":[123],"550\u00b0C,":[125],"with":[126],"operation":[128],"over":[130],"2500":[131],"hours.":[132],"This":[133],"work":[134],"establishes":[135],"new":[137],"paradigm":[138],"regulating":[140],"transfer":[142],"offers":[144],"viable":[146],"route":[147],"efficient,":[150],"durable":[151],"degradation":[152],"gaseous":[154],"PFAS.":[155]},"counts_by_year":[{"year":2026,"cited_by_count":10}],"updated_date":"2026-10-14T16:39:01.820549","created_date":"2026-01-14T00:00:00"}
