{"id":"https://openalex.org/W7077166316","doi":"https://doi.org/10.3204/pubdb-2025-02387","title":"High-entropy argyrodite glass\u2013ceramic electrolytes for all-solid-state batteries","display_name":"High-entropy argyrodite glass\u2013ceramic electrolytes for all-solid-state batteries","publication_year":2025,"publication_date":"2025-01-01","ids":{"openalex":"https://openalex.org/W7077166316","doi":"https://doi.org/10.3204/pubdb-2025-02387"},"language":"en","primary_location":{"id":"doi:10.3204/pubdb-2025-02387","doi":"https://doi.org/10.3204/pubdb-2025-02387","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-02387","pdf_url":null,"source":{"id":"https://openalex.org/S4306400383","display_name":"DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron)","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I2801876189","host_organization_name":"Deutsches Elektronen-Synchrotron DESY","host_organization_lineage":["https://openalex.org/I2801876189"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"article-journal"},"volume":null,"type":"article","indexed_in":["datacite"],"open_access":{"is_oa":true,"oa_status":"green","oa_url":"https://doi.org/10.3204/pubdb-2025-02387","any_repository_has_fulltext":true},"authorships":[{"author_position":"first","author":{"id":null,"display_name":"Lin, Jing","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Lin, Jing","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5081935806","display_name":"Mareen Schaller","orcid":"https://orcid.org/0000-0001-6589-2087","observed_orcids":["https://orcid.org/0000-0001-6589-2087"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Schaller, Mareen","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5036391168","display_name":"Ruizhuo Zhang","orcid":"https://orcid.org/0000-0003-0292-5026","observed_orcids":["https://orcid.org/0000-0003-0292-5026"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Zhang, Ruizhuo","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5049456998","display_name":"Volodymyr V. Baran","orcid":"https://orcid.org/0000-0003-2379-3632","observed_orcids":["https://orcid.org/0000-0003-2379-3632","https://orcid.org/0000-0002-9185-3855"]},"institutions":[{"id":"https://openalex.org/I2801876189","display_name":"Deutsches Elektronen-Synchrotron DESY","ror":"https://ror.org/01js2sh04","country_code":"DE","type":"facility","lineage":["https://openalex.org/I1305996414","https://openalex.org/I2801876189"]}],"countries":["DE"],"is_corresponding":false,"raw_author_name":"Baran, Volodymyr","raw_affiliation_strings":["Deutsches Elektronen-Synchrotron"],"raw_orcid":"https://orcid.org/0000-0003-2379-3632","affiliations":[{"raw_affiliation_string":"Deutsches Elektronen-Synchrotron","institution_ids":["https://openalex.org/I2801876189"]}]},{"author_position":"middle","author":{"id":null,"display_name":"Liu, Hao","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Liu, Hao","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5059337815","display_name":"Ziming Ding","orcid":"https://orcid.org/0000-0003-4760-7806","observed_orcids":["https://orcid.org/0000-0003-4760-7806"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Ding, Ziming","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5046099728","display_name":"Sylvio Indris","orcid":"https://orcid.org/0000-0002-5100-113X","observed_orcids":["https://orcid.org/0000-0002-5100-113X"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Indris, Sylvio","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5028425268","display_name":"Aleksandr Kondrakov","orcid":"https://orcid.org/0000-0003-1465-2854","observed_orcids":["https://orcid.org/0000-0003-1465-2854"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Kondrakov, Aleksandr","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Brezesinski, Torsten","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Brezesinski, Torsten","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"last","author":{"id":"https://openalex.org/A5019742727","display_name":"Florian Strauss","orcid":"https://orcid.org/0000-0001-5817-6349","observed_orcids":["https://orcid.org/0000-0001-5817-6349"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Strauss, Florian","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":1,"corresponding_author_ids":[],"corresponding_institution_ids":[],"apc_list":null,"apc_paid":null,"fwci":0.0,"has_fulltext":false,"cited_by_count":0,"citation_normalized_percentile":{"value":0.2528938,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":true,"primary_topic":{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":1.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":1.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.0,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T12875","display_name":"Thermal Expansion and Ionic Conductivity","score":0.0,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/lithium-argyrodite","display_name":"lithium argyrodite","score":0.9150000214576721},{"id":"https://openalex.org/keywords/solid-electrolytes","display_name":"solid electrolytes","score":0.6169999837875366},{"id":"https://openalex.org/keywords/glass-ceramic-electrolytes","display_name":"glass-ceramic electrolytes","score":0.8659999966621399},{"id":"https://openalex.org/keywords/all-solid-state-batteries","display_name":"all-solid-state batteries","score":0.8550000190734863},{"id":"https://openalex.org/keywords/high-entropy-materials","display_name":"high-entropy materials","score":0.8830000162124634},{"id":"https://openalex.org/keywords/ionic-conductivity","display_name":"ionic conductivity","score":0.722000002861023},{"id":"https://openalex.org/keywords/post-annealing","display_name":"post-annealing","score":0.7590000033378601},{"id":"https://openalex.org/keywords/mechanochemical-synthesis","display_name":"mechanochemical synthesis","score":0.7490000128746033},{"id":"https://openalex.org/keywords/crystallinity","display_name":"crystallinity","score":0.3790000081062317},{"id":"https://openalex.org/keywords/defect-concentration","display_name":"defect concentration","score":0.8379999995231628},{"id":"https://openalex.org/keywords/occupational-diseases","display_name":"occupational diseases","score":0.5720000267028809},{"id":"https://openalex.org/keywords/lisicon","display_name":"lithium superionic conductors","score":0.5789999961853027}],"concepts":[{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.7671999931335449},{"id":"https://openalex.org/C138679309","wikidata":"https://www.wikidata.org/wiki/Q6063658","display_name":"Ionic conductivity","level":4,"score":0.7379999756813049},{"id":"https://openalex.org/C68801617","wikidata":"https://www.wikidata.org/wiki/Q162908","display_name":"Electrolyte","level":3,"score":0.7373999953269958},{"id":"https://openalex.org/C46275449","wikidata":"https://www.wikidata.org/wiki/Q2458815","display_name":"Crystallinity","level":2,"score":0.7077000141143799},{"id":"https://openalex.org/C109883240","wikidata":"https://www.wikidata.org/wiki/Q1672053","display_name":"Fast ion conductor","level":4,"score":0.5705999732017517},{"id":"https://openalex.org/C2778541603","wikidata":"https://www.wikidata.org/wiki/Q152763","display_name":"Lithium (medication)","level":2,"score":0.5555999875068665},{"id":"https://openalex.org/C57863236","wikidata":"https://www.wikidata.org/wiki/Q1130571","display_name":"Doping","level":2,"score":0.5152999758720398},{"id":"https://openalex.org/C131540310","wikidata":"https://www.wikidata.org/wiki/Q907564","display_name":"Conductivity","level":2,"score":0.4871000051498413},{"id":"https://openalex.org/C2182769","wikidata":"https://www.wikidata.org/wiki/Q62500","display_name":"Ionic bonding","level":3,"score":0.438400000333786},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.4309000074863434},{"id":"https://openalex.org/C179104552","wikidata":"https://www.wikidata.org/wiki/Q11165","display_name":"Inorganic chemistry","level":1,"score":0.38749998807907104},{"id":"https://openalex.org/C138999460","wikidata":"https://www.wikidata.org/wiki/Q787619","display_name":"Solid solution","level":2,"score":0.3086000084877014},{"id":"https://openalex.org/C207114421","wikidata":"https://www.wikidata.org/wiki/Q133900","display_name":"Diffraction","level":2,"score":0.3012000024318695},{"id":"https://openalex.org/C69990965","wikidata":"https://www.wikidata.org/wiki/Q65402698","display_name":"Electrical resistivity and conductivity","level":2,"score":0.28049999475479126},{"id":"https://openalex.org/C202374169","wikidata":"https://www.wikidata.org/wiki/Q124291","display_name":"Electrical conductor","level":2,"score":0.2775999903678894},{"id":"https://openalex.org/C145148216","wikidata":"https://www.wikidata.org/wiki/Q36496","display_name":"Ion","level":2,"score":0.25929999351501465}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.3204/pubdb-2025-02387","doi":"https://doi.org/10.3204/pubdb-2025-02387","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-02387","pdf_url":null,"source":{"id":"https://openalex.org/S4306400383","display_name":"DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron)","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I2801876189","host_organization_name":"Deutsches Elektronen-Synchrotron DESY","host_organization_lineage":["https://openalex.org/I2801876189"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":null,"raw_source_name":null,"raw_type":"article-journal"}],"best_oa_location":{"id":"doi:10.3204/pubdb-2025-02387","doi":"https://doi.org/10.3204/pubdb-2025-02387","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-02387","pdf_url":null,"source":{"id":"https://openalex.org/S4306400383","display_name":"DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron)","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I2801876189","host_organization_name":"Deutsches Elektronen-Synchrotron DESY","host_organization_lineage":["https://openalex.org/I2801876189"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"article-journal"},"sustainable_development_goals":[{"id":"https://metadata.un.org/sdg/7","score":0.75,"display_name":"Affordable and clean energy"}],"sustainable_development_goals_aurora":[],"study_designs":[],"awards":[],"funders":[],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":0,"referenced_works":[],"related_works":[],"abstract_inverted_index":{"Lithium":[0],"argyrodite":[1,35,69],"superionic":[2],"conductors":[3],"with":[4],"the":[5,25,43,129,160,163,175],"general":[6],"formula":[7],"Li$_6$PS$_5$X":[8],"(X":[9],"=":[10],"Cl,":[11],"Br,":[12],"I)":[13],"have":[14],"been":[15,56],"intensively":[16],"investigated":[17],"in":[18,24,139],"recent":[19],"years":[20],"and":[21,90,99,131],"successfully":[22],"adopted":[23],"field":[26],"of":[27,34,45,70,115,165,177],"solid-state":[28],"batteries":[29],"(SSBs).":[30],"The":[31,143],"transport":[32],"properties":[33,176],"solid":[36],"electrolytes":[37],"(SEs)":[38],"usually":[39],"strongly":[40],"depend":[41],"on":[42],"degree":[44],"occupational":[46],"disorder.":[47],"Increasing":[48],"disorder":[49],"through":[50],"complex":[51],"doping":[52],"or":[53],"substitution":[54],"has":[55],"shown":[57],"to":[58,107,150],"directly":[59],"affect":[60],"ionic":[61,113],"conductivity.":[62],"Herein,":[63],"we":[64,93],"explore":[65],"a":[66,110],"high-entropy":[67],"lithium":[68,178],"nominal":[71],"composition":[72],"Li$_{6.6}$[P$_{0.2}$Si$_{0.2}$Sn$_{0.2}$Ge$_{0.2}$Sb$_{0.2}$]S$_5$I.":[73],"This":[74],"material":[75],"can":[76,125],"be":[77,126],"readily":[78],"prepared":[79,145],"by":[80,102],"mechanochemistry.":[81],"Using":[82],"complementary":[83],"diffraction":[84],"techniques,":[85],"nuclear":[86],"magnetic":[87],"resonance":[88],"spectroscopy,":[89],"charge-transport":[91],"measurements,":[92],"show":[94],"that":[95],"upon":[96],"tailoring":[97],"crystallinity":[98],"defect":[100],"concentration":[101],"post-annealing":[103],"at":[104],"temperatures":[105],"up":[106],"220":[108,134],"\u00b0C,":[109],"high":[111],"room-temperature":[112],"conductivity":[114],"about":[116],"0.9":[117],"mS":[118,121],"cm$^{\u22121}$":[119,122],"(\u223c4.4":[120],"bulk":[123],"conductivity)":[124],"achieved.":[127],"Both":[128],"as-prepared":[130],"annealed":[132],"(at":[133],"\u00b0C)":[135],"samples":[136],"were":[137],"tested":[138],"pellet-stack":[140],"SSB":[141,181],"cells.":[142],"mechanochemically":[144],"glass\u2013ceramic":[146],"SE":[147],"was":[148],"found":[149],"exhibit":[151],"superior":[152],"performance,":[153],"even":[154],"outperforming":[155],"commercially":[156],"available":[157],"Li$_6$PS$_5$Cl.":[158],"Collectively,":[159],"results":[161],"highlight":[162],"importance":[164],"considering":[166],"structural":[167],"aspects":[168],"across":[169],"different":[170],"length":[171],"scales":[172],"when":[173],"optimizing":[174],"argyrodites":[179],"for":[180],"applications.":[182]},"counts_by_year":[],"updated_date":"2026-10-14T16:39:01.820549","created_date":"2025-10-10T00:00:00"}