{"id":"https://openalex.org/W6889894687","doi":"https://doi.org/10.3204/pubdb-2025-00929","title":"Operando-informed precatalyst programming towards reliable high-current-density electrolysis","display_name":"Operando-informed precatalyst programming towards reliable high-current-density electrolysis","publication_year":2025,"publication_date":"2025-01-01","ids":{"openalex":"https://openalex.org/W6889894687","doi":"https://doi.org/10.3204/pubdb-2025-00929"},"language":"en","primary_location":{"id":"doi:10.3204/pubdb-2025-00929","doi":"https://doi.org/10.3204/pubdb-2025-00929","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-00929","pdf_url":null,"source":{"id":"https://openalex.org/S103895331","display_name":"Nature Materials","issn_l":"1476-1122","issn":["1476-1122","1476-4660"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["anvur-scientific","cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"article-journal"},"volume":null,"type":"article","indexed_in":["datacite"],"open_access":{"is_oa":true,"oa_status":"bronze","oa_url":"https://doi.org/10.3204/pubdb-2025-00929","any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":null,"display_name":"Xia, Lu","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Xia, Lu","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5035058862","display_name":"Bruna Ferreira Gomes","orcid":"https://orcid.org/0000-0002-6879-3583","observed_orcids":["https://orcid.org/0000-0002-6879-3583"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Gomes, Bruna Ferreira","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5019193826","display_name":"Wulyu Jiang","orcid":"https://orcid.org/0000-0003-2258-8688","observed_orcids":["https://orcid.org/0000-0003-2258-8688"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Jiang, Wulyu","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5053923970","display_name":"Daniel Escalera\u2010L\u00f3pez","orcid":"https://orcid.org/0000-0002-2001-9775","observed_orcids":["https://orcid.org/0000-0002-2001-9775"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Escalera-L\u00f3pez, Daniel","raw_affiliation_strings":[],"raw_orcid":"https://orcid.org/0000-0002-2001-9775","affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Wang, Yang","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Wang, Yang","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Hu, Yang","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Hu, Yang","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5005278041","display_name":"Alaa Y. Faid","orcid":"https://orcid.org/0000-0003-3008-9774","observed_orcids":["https://orcid.org/0000-0003-3008-9774"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Faid, Alaa Y.","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Wang, Kaiwen","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Wang, Kaiwen","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5135826775","display_name":"Tengyu Chen","orcid":"https://orcid.org/0009-0006-6288-507X","observed_orcids":["https://orcid.org/0009-0006-6288-507X"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Chen, Tengyu","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5134690255","display_name":"Kaiqi Zhao","orcid":"https://orcid.org/0000-0002-0990-1003","observed_orcids":["https://orcid.org/0000-0002-0990-1003"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Zhao, Kaiqi","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Zhang, Xu","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Zhang, Xu","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Zhou, Yingtang","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Zhou, Yingtang","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5057264101","display_name":"Ranit Ram","orcid":"https://orcid.org/0000-0002-7999-5551","observed_orcids":["https://orcid.org/0000-0002-7999-5551"]},"institutions":[{"id":"https://openalex.org/I4210138560","display_name":"European Molecular Biology Laboratory","ror":"https://ror.org/03mstc592","country_code":"DE","type":"government","lineage":["https://openalex.org/I4210138560"]},{"id":"https://openalex.org/I4210153543","display_name":"European Molecular Biology Laboratory","ror":"https://ror.org/050589e39","country_code":"DE","type":"government","lineage":["https://openalex.org/I4210138560","https://openalex.org/I4210153543"]}],"countries":["DE"],"is_corresponding":false,"raw_author_name":"Ram, Ranit","raw_affiliation_strings":["European Molecular Biology Laboratory"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"European Molecular Biology Laboratory","institution_ids":["https://openalex.org/I4210138560","https://openalex.org/I4210153543"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5091700266","display_name":"B\u00e1rbara B. Polesso","orcid":"https://orcid.org/0000-0003-4722-7491","observed_orcids":["https://orcid.org/0000-0003-4722-7491"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Polesso, Barbara","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5033159909","display_name":"Anku Guha","orcid":"https://orcid.org/0000-0003-4533-6336","observed_orcids":["https://orcid.org/0000-0003-4533-6336"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Guha, Anku","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5050546873","display_name":"Jiaqi Su","orcid":"https://orcid.org/0000-0003-2010-8388","observed_orcids":["https://orcid.org/0000-0003-2010-8388","https://orcid.org/0009-0006-6814-5136"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Su, Jiaqi","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5011283254","display_name":"Carlos Manuel Silva Lobo","orcid":"https://orcid.org/0000-0002-7727-008X","observed_orcids":["https://orcid.org/0000-0002-7727-008X"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Lobo, Carlos","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5008932544","display_name":"Michael Haumann","orcid":"https://orcid.org/0000-0001-7008-1764","observed_orcids":["https://orcid.org/0000-0001-7008-1764"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Haumann, Michael","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5038651709","display_name":"Robert Spatschek","orcid":"https://orcid.org/0000-0002-0087-677X","observed_orcids":["https://orcid.org/0000-0002-0087-677X"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Spatschek, Robert","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5082270903","display_name":"Svein Sunde","orcid":"https://orcid.org/0000-0003-3711-8822","observed_orcids":["https://orcid.org/0000-0003-3711-8822"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Sunde, Svein","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Gan, Lin","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Gan, Lin","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Huang, Ming","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Huang, Ming","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Zhou, Xiaoyuan","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Zhou, Xiaoyuan","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5031585159","display_name":"Christina Roth","orcid":"https://orcid.org/0000-0003-1159-2956","observed_orcids":["https://orcid.org/0000-0003-1159-2956"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Roth, Christina","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5091841971","display_name":"Werner Lehnert","orcid":"https://orcid.org/0000-0002-7423-872X","observed_orcids":["https://orcid.org/0000-0002-7423-872X"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Lehnert, Werner","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":"https://openalex.org/A5073666601","display_name":"Serhiy Cherevko","orcid":"https://orcid.org/0000-0002-7188-4857","observed_orcids":["https://orcid.org/0000-0002-7188-4857"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Cherevko, Serhiy","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Gan, Liyong","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Gan, Liyong","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"middle","author":{"id":null,"display_name":"Garcia de Arquer, F. Pelayo","orcid":null,"observed_orcids":[]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Garcia de Arquer, F. Pelayo","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]},{"author_position":"last","author":{"id":"https://openalex.org/A5025547811","display_name":"Meital Shviro","orcid":"https://orcid.org/0000-0002-9494-0233","observed_orcids":["https://orcid.org/0000-0002-9494-0233"]},"institutions":[],"countries":[],"is_corresponding":false,"raw_author_name":"Shviro, Meital","raw_affiliation_strings":[],"raw_orcid":null,"affiliations":[]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":[],"corresponding_institution_ids":[],"apc_list":{"value":12690,"currency":"USD","value_usd":12690},"apc_paid":null,"fwci":0.0,"has_fulltext":false,"cited_by_count":0,"citation_normalized_percentile":{"value":0.14441828,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":true,"primary_topic":{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9994999766349792,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9994999766349792,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11784","display_name":"CO2 Reduction Techniques and Catalysts","score":0.00019999999494757503,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10409","display_name":"Fuel Cells and Related Materials","score":9.999999747378752e-05,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/oxygen-evolution-reaction","display_name":"oxygen evolution reaction","score":0.9300000071525574},{"id":"https://openalex.org/keywords/surface-reconstruction","display_name":"surface reconstruction","score":0.7160000205039978},{"id":"https://openalex.org/keywords/fe-oxidation","display_name":"Fe oxidation","score":0.7749999761581421},{"id":"https://openalex.org/keywords/catalyst-deactivation","display_name":"catalyst deactivation","score":0.8700000047683716},{"id":"https://openalex.org/keywords/catalyst-stability","display_name":"catalyst stability","score":0.6169999837875366},{"id":"https://openalex.org/keywords/anion-exchange-membrane-water-electrolysis","display_name":"anion exchange membrane water electrolysis","score":0.8970000147819519},{"id":"https://openalex.org/keywords/high-current-density-electrolysis","display_name":"high current density electrolysis","score":0.8840000033378601},{"id":"https://openalex.org/keywords/catalyst-design","display_name":"catalyst design","score":0.382999986410141}],"concepts":[{"id":"https://openalex.org/C48256821","wikidata":"https://www.wikidata.org/wiki/Q903456","display_name":"Electrolysis of water","level":5,"score":0.6502000093460083},{"id":"https://openalex.org/C163127949","wikidata":"https://www.wikidata.org/wiki/Q64403","display_name":"Electrolysis","level":4,"score":0.6262000203132629},{"id":"https://openalex.org/C43214815","wikidata":"https://www.wikidata.org/wiki/Q7310987","display_name":"Reliability (semiconductor)","level":3,"score":0.6080999970436096},{"id":"https://openalex.org/C33989665","wikidata":"https://www.wikidata.org/wiki/Q5357962","display_name":"Electrocatalyst","level":4,"score":0.6055999994277954},{"id":"https://openalex.org/C21880701","wikidata":"https://www.wikidata.org/wiki/Q2144042","display_name":"Process engineering","level":1,"score":0.46389999985694885},{"id":"https://openalex.org/C18762648","wikidata":"https://www.wikidata.org/wiki/Q42213","display_name":"Work (physics)","level":2,"score":0.46070000529289246},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.4571000039577484},{"id":"https://openalex.org/C2779679103","wikidata":"https://www.wikidata.org/wiki/Q5251805","display_name":"Degradation (telecommunications)","level":2,"score":0.4156000018119812},{"id":"https://openalex.org/C135473242","wikidata":"https://www.wikidata.org/wiki/Q4147614","display_name":"Oxygen evolution","level":4,"score":0.39169999957084656},{"id":"https://openalex.org/C104304963","wikidata":"https://www.wikidata.org/wiki/Q5316114","display_name":"Durability","level":2,"score":0.38580000400543213},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.37459999322891235},{"id":"https://openalex.org/C112972136","wikidata":"https://www.wikidata.org/wiki/Q7595718","display_name":"Stability (learning theory)","level":2,"score":0.3675999939441681},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.36660000681877136},{"id":"https://openalex.org/C41008148","wikidata":"https://www.wikidata.org/wiki/Q21198","display_name":"Computer science","level":0,"score":0.32600000500679016},{"id":"https://openalex.org/C2987658370","wikidata":"https://www.wikidata.org/wiki/Q180253","display_name":"Fuel cells","level":2,"score":0.31540000438690186},{"id":"https://openalex.org/C172205157","wikidata":"https://www.wikidata.org/wiki/Q1782962","display_name":"Model predictive control","level":3,"score":0.3066999912261963},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.3050999939441681},{"id":"https://openalex.org/C540031477","wikidata":"https://www.wikidata.org/wiki/Q629","display_name":"Oxygen","level":2,"score":0.296099990606308},{"id":"https://openalex.org/C148898269","wikidata":"https://www.wikidata.org/wiki/Q1108792","display_name":"Kinetics","level":2,"score":0.2851000130176544},{"id":"https://openalex.org/C148043351","wikidata":"https://www.wikidata.org/wiki/Q4456944","display_name":"Current (fluid)","level":2,"score":0.28110000491142273},{"id":"https://openalex.org/C100729193","wikidata":"https://www.wikidata.org/wiki/Q17105319","display_name":"Polymer electrolyte membrane electrolysis","level":5,"score":0.2750999927520752},{"id":"https://openalex.org/C105768512","wikidata":"https://www.wikidata.org/wiki/Q7458208","display_name":"Reaction intermediate","level":3,"score":0.26829999685287476},{"id":"https://openalex.org/C2780302529","wikidata":"https://www.wikidata.org/wiki/Q6815127","display_name":"Membrane electrode assembly","level":4,"score":0.26660001277923584},{"id":"https://openalex.org/C117760992","wikidata":"https://www.wikidata.org/wiki/Q389137","display_name":"Ion exchange","level":3,"score":0.26170000433921814}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.3204/pubdb-2025-00929","doi":"https://doi.org/10.3204/pubdb-2025-00929","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-00929","pdf_url":null,"source":{"id":"https://openalex.org/S103895331","display_name":"Nature Materials","issn_l":"1476-1122","issn":["1476-1122","1476-4660"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["anvur-scientific","cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":null,"raw_source_name":null,"raw_type":"article-journal"}],"best_oa_location":{"id":"doi:10.3204/pubdb-2025-00929","doi":"https://doi.org/10.3204/pubdb-2025-00929","is_oa":true,"landing_page_url":"https://doi.org/10.3204/pubdb-2025-00929","pdf_url":null,"source":{"id":"https://openalex.org/S103895331","display_name":"Nature Materials","issn_l":"1476-1122","issn":["1476-1122","1476-4660"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["anvur-scientific","cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310319908","host_organization_name":"Nature Portfolio","host_organization_lineage":["https://openalex.org/P4310319908","https://openalex.org/P4310319965"],"host_organization_lineage_names":["Nature Portfolio","Springer Nature"],"type":"journal"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"article-journal"},"sustainable_development_goals":[{"score":0.8485000133514404,"display_name":"Affordable and clean energy","id":"https://metadata.un.org/sdg/7"}],"sustainable_development_goals_aurora":[{"score":0.5471130609512329,"display_name":"Industry, innovation and infrastructure","id":"https://metadata.un.org/sdg/9"}],"study_designs":[],"awards":[],"funders":[],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":0,"referenced_works":[],"related_works":[],"abstract_inverted_index":{"Electrocatalysts":[0],"support":[1],"crucial":[2],"industrial":[3,171],"processes":[4],"and":[5,16,32,36,44,62,68,70,86,100,105,163,174],"emerging":[6],"decarbonization":[7],"technologies,":[8],"but":[9],"their":[10],"design":[11,102],"is":[12],"hindered":[13],"by":[14],"structural":[15],"compositional":[17],"changes":[18],"during":[19],"operation,":[20],"especially":[21],"at":[22,154,176],"application-relevant":[23],"current":[24,178],"densities.":[25,179],"Here":[26],"we":[27,77],"use":[28],"operando":[29],"X-ray":[30],"spectroscopy":[31],"modelling":[33,162],"to":[34,58,115,143],"track,":[35],"eventually":[37],"direct,":[38],"the":[39,47,84,101,167],"reconstruction":[40],"of":[41,88,103,129],"iron":[42],"sulfides":[43],"oxides":[45],"for":[46,170],"oxygen":[48],"evolution":[49],"reaction.":[50],"We":[51],"show":[52],"that":[53],"inappropriate":[54],"activation":[55,79],"protocols":[56],"lead":[57],"uncontrollable":[59],"Fe":[60],"oxidation":[61],"irreversible":[63],"catalyst":[64],"degradation,":[65],"compromising":[66],"stability":[67],"reliability":[69,169],"precluding":[71],"predictive":[72,161],"design.":[73],"Based":[74],"on":[75],"these,":[76],"develop":[78],"programming":[80],"strategies":[81],"that,":[82],"considering":[83],"thermodynamics":[85],"kinetics":[87],"surface":[89],"reconstruction,":[90],"offer":[91],"control":[92],"over":[93,134],"precatalyst":[94],"oxidation.":[95],"This":[96,158],"enables":[97],"reliable":[98],"predictions":[99],"active":[104],"stable":[106],"electrocatalysts.":[107],"In":[108],"a":[109,116,125],"Ni$_x$Fe$_{1\u2212x}$S$_2$":[110],"model":[111],"system,":[112],"this":[113],"leads":[114],"threefold":[117],"improvement":[118],"in":[119,146],"durability":[120],"after":[121],"programmed":[122],"activation,":[123],"with":[124],"cell":[126],"degradation":[127],"rate":[128],"0.12":[130],"mV":[131,140],"h$^":[132],"{\u22121}$":[133],"550":[135],"h":[136],"(standard":[137],"operation:":[138],"0.29":[139],"h$^{\u22121}$,":[141],"constrained":[142],"200":[144],"h),":[145],"an":[147],"anion":[148],"exchange":[149],"membrane":[150],"water":[151,172],"electrolyser":[152],"operating":[153],"1":[155],"A":[156],"cm$^{\u22122}$.":[157],"work":[159],"bridges":[160],"experimental":[164],"design,":[165],"improving":[166],"electrocatalyst":[168],"electrolysis":[173],"beyond":[175],"high":[177]},"counts_by_year":[],"updated_date":"2026-10-14T16:39:01.820549","created_date":"2025-10-10T00:00:00"}