{"id":"https://openalex.org/W4407985508","doi":"https://doi.org/10.1002/adfm.202417139","title":"Customizing Synchronous Charge Tunneling Photosystems Toward Solar CO2 Conversion","display_name":"Customizing Synchronous Charge Tunneling Photosystems Toward Solar CO2 Conversion","publication_year":2025,"publication_date":"2025-02-24","ids":{"openalex":"https://openalex.org/W4407985508","doi":"https://doi.org/10.1002/adfm.202417139"},"language":"en","primary_location":{"id":"doi:10.1002/adfm.202417139","doi":"https://doi.org/10.1002/adfm.202417139","is_oa":false,"landing_page_url":"https://doi.org/10.1002/adfm.202417139","pdf_url":null,"source":{"id":"https://openalex.org/S135204980","display_name":"Advanced Functional Materials","issn_l":"1616-301X","issn":["1616-301X","1616-3028"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-3","ki-jl-3","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320595","host_organization_name":"Wiley","host_organization_lineage":["https://openalex.org/P4310320595"],"host_organization_lineage_names":["Wiley"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Advanced Functional Materials","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5100371368","display_name":"Qing Chen","orcid":"https://orcid.org/0000-0002-7919-5159","observed_orcids":["https://orcid.org/0000-0002-7919-5159"]},"institutions":[{"id":"https://openalex.org/I80947539","display_name":"Fuzhou University","ror":"https://ror.org/011xvna82","country_code":"CN","type":"education","lineage":["https://openalex.org/I80947539"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Qing Chen","raw_affiliation_strings":["College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","institution_ids":["https://openalex.org/I80947539"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5045044576","display_name":"Yihan Chen","orcid":"https://orcid.org/0000-0003-2085-9480","observed_orcids":["https://orcid.org/0000-0003-2085-9480","https://orcid.org/0009-0006-0036-560X","https://orcid.org/0009-0009-6889-2731"]},"institutions":[{"id":"https://openalex.org/I80947539","display_name":"Fuzhou University","ror":"https://ror.org/011xvna82","country_code":"CN","type":"education","lineage":["https://openalex.org/I80947539"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Yi\u2010Han Chen","raw_affiliation_strings":["College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","institution_ids":["https://openalex.org/I80947539"]}]},{"author_position":"middle","author":{"id":null,"display_name":"Jun\u2010Rong Zhu","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I80947539","display_name":"Fuzhou University","ror":"https://ror.org/011xvna82","country_code":"CN","type":"education","lineage":["https://openalex.org/I80947539"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Jun\u2010Rong Zhu","raw_affiliation_strings":["College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","institution_ids":["https://openalex.org/I80947539"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5100448281","display_name":"Zhenzhen Li","orcid":"https://orcid.org/0009-0008-8553-6475","observed_orcids":["https://orcid.org/0009-0008-8553-6475","https://orcid.org/0000-0001-8237-7781"]},"institutions":[{"id":"https://openalex.org/I80947539","display_name":"Fuzhou University","ror":"https://ror.org/011xvna82","country_code":"CN","type":"education","lineage":["https://openalex.org/I80947539"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Zhuang\u2010Yan Li","raw_affiliation_strings":["College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","institution_ids":["https://openalex.org/I80947539"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5001193862","display_name":"Fang\u2010Xing Xiao","orcid":"https://orcid.org/0000-0001-5673-5362","observed_orcids":["https://orcid.org/0000-0001-5673-5362"]},"institutions":[{"id":"https://openalex.org/I19820366","display_name":"Chinese Academy of Sciences","ror":"https://ror.org/034t30j35","country_code":"CN","type":"government","lineage":["https://openalex.org/I19820366"]},{"id":"https://openalex.org/I4210119098","display_name":"Fujian Institute of Research on the Structure of Matter","ror":"https://ror.org/02j89k719","country_code":"CN","type":"facility","lineage":["https://openalex.org/I19820366","https://openalex.org/I4210119098"]},{"id":"https://openalex.org/I4391767757","display_name":"State Key Laboratory of Structural Chemistry","ror":"https://ror.org/023fpv336","country_code":"CN","type":"facility","lineage":["https://openalex.org/I19820366","https://openalex.org/I4210119098","https://openalex.org/I4391767757"]},{"id":"https://openalex.org/I80947539","display_name":"Fuzhou University","ror":"https://ror.org/011xvna82","country_code":"CN","type":"education","lineage":["https://openalex.org/I80947539"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Fang\u2010Xing Xiao","raw_affiliation_strings":["College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 P. R. China"],"raw_orcid":"https://orcid.org/0000-0001-5673-5362","affiliations":[{"raw_affiliation_string":"College of Materials Science and Engineering Fuzhou University  New Campus Minhou Fujian 350108 P. R. China","institution_ids":["https://openalex.org/I80947539"]},{"raw_affiliation_string":"State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences  Fuzhou Fujian 350002 P. R. China","institution_ids":["https://openalex.org/I19820366","https://openalex.org/I4210119098","https://openalex.org/I4391767757"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":4,"corresponding_author_ids":["https://openalex.org/A5001193862"],"corresponding_institution_ids":["https://openalex.org/I19820366","https://openalex.org/I4210119098","https://openalex.org/I4391767757","https://openalex.org/I80947539"],"apc_list":{"value":5790,"currency":"USD","value_usd":5790},"apc_paid":null,"fwci":6.1695,"has_fulltext":false,"cited_by_count":46,"citation_normalized_percentile":{"value":0.97751148,"is_in_top_1_percent":false,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":99,"max":100},"biblio":{"volume":"35","issue":"13","first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.9916999936103821,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.9916999936103821,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11784","display_name":"CO2 Reduction Techniques and Catalysts","score":0.007199999876320362,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10024","display_name":"TiO2 Photocatalysis and Solar Cells","score":0.0003000000142492354,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/solar-co2-reduction","display_name":"solar CO2 reduction","score":0.8500000238418579},{"id":"https://openalex.org/keywords/charge-tunneling","display_name":"charge tunneling","score":0.7570000290870667},{"id":"https://openalex.org/keywords/artificial-photosystems","display_name":"artificial photosystems","score":0.8349999785423279},{"id":"https://openalex.org/keywords/layered-double-hydroxides","display_name":"layered double hydroxides","score":0.9129999876022339},{"id":"https://openalex.org/keywords/transition-metal-chalcogenides","display_name":"transition metal chalcogenides","score":0.9980000257492065},{"id":"https://openalex.org/keywords/layer-by-layer-assembly","display_name":"layer-by-layer assembly","score":0.9440000057220459},{"id":"https://openalex.org/keywords/charge-separation","display_name":"charge separation","score":0.8930000066757202},{"id":"https://openalex.org/keywords/co2-adsorption","display_name":"CO2 adsorption","score":0.7039999961853027},{"id":"https://openalex.org/keywords/photocatalysis","display_name":"photocatalysis","score":0.6359999775886536},{"id":"https://openalex.org/keywords/solar-energy-conversion","display_name":"solar energy conversion","score":0.6240000128746033}],"concepts":[{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.8296478986740112},{"id":"https://openalex.org/C120398109","wikidata":"https://www.wikidata.org/wiki/Q175751","display_name":"Quantum tunnelling","level":2,"score":0.6953434944152832},{"id":"https://openalex.org/C188082385","wikidata":"https://www.wikidata.org/wiki/Q73792","display_name":"Charge (physics)","level":2,"score":0.5740764737129211},{"id":"https://openalex.org/C41291067","wikidata":"https://www.wikidata.org/wiki/Q1897785","display_name":"Photovoltaic system","level":2,"score":0.4219381511211395},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.41709643602371216},{"id":"https://openalex.org/C49040817","wikidata":"https://www.wikidata.org/wiki/Q193091","display_name":"Optoelectronics","level":1,"score":0.414445161819458},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.3704673647880554},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.10743874311447144},{"id":"https://openalex.org/C18903297","wikidata":"https://www.wikidata.org/wiki/Q7150","display_name":"Ecology","level":1,"score":0.0},{"id":"https://openalex.org/C86803240","wikidata":"https://www.wikidata.org/wiki/Q420","display_name":"Biology","level":0,"score":0.0},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.0}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.1002/adfm.202417139","doi":"https://doi.org/10.1002/adfm.202417139","is_oa":false,"landing_page_url":"https://doi.org/10.1002/adfm.202417139","pdf_url":null,"source":{"id":"https://openalex.org/S135204980","display_name":"Advanced Functional Materials","issn_l":"1616-301X","issn":["1616-301X","1616-3028"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-3","ki-jl-3","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320595","host_organization_name":"Wiley","host_organization_lineage":["https://openalex.org/P4310320595"],"host_organization_lineage_names":["Wiley"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Advanced Functional Materials","raw_type":"journal-article"}],"best_oa_location":null,"sustainable_development_goals":[{"id":"https://metadata.un.org/sdg/7","display_name":"Affordable and clean energy","score":0.875},{"id":"https://metadata.un.org/sdg/13","display_name":"Climate action","score":0.75},{"id":"https://metadata.un.org/sdg/9","display_name":"Industry, innovation and infrastructure","score":0.428600013256073}],"study_designs":[],"awards":[{"id":"https://openalex.org/G4836181937","display_name":"\u7b49\u79bb\u6fc0\u5143\u70ed\u7535\u5b50\u8fde\u7eed\u4f20\u8f93\u901a\u9053\u6784\u7b51\u53ca\u53ef\u63a7\u8c03\u8282\u673a\u5236\u7814\u7a76","funder_award_id":"22072025","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G8490994796","display_name":null,"funder_award_id":"21703038","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"}],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":73,"referenced_works":["https://openalex.org/W1995155629","https://openalex.org/W1998150177","https://openalex.org/W2003959873","https://openalex.org/W2070996448","https://openalex.org/W2090729803","https://openalex.org/W2313706429","https://openalex.org/W2586030301","https://openalex.org/W2598141478","https://openalex.org/W2644600533","https://openalex.org/W2736012892","https://openalex.org/W2754328210","https://openalex.org/W2796167332","https://openalex.org/W2886225488","https://openalex.org/W2893900929","https://openalex.org/W2909411138","https://openalex.org/W2921025911","https://openalex.org/W2944410561","https://openalex.org/W2951356243","https://openalex.org/W2963049339","https://openalex.org/W2963174219","https://openalex.org/W2971634515","https://openalex.org/W2993163882","https://openalex.org/W2994629904","https://openalex.org/W3011683090","https://openalex.org/W3012524773","https://openalex.org/W3017221539","https://openalex.org/W3018120389","https://openalex.org/W3022350592","https://openalex.org/W3042293217","https://openalex.org/W3085214668","https://openalex.org/W3088598452","https://openalex.org/W3100649385","https://openalex.org/W3111059218","https://openalex.org/W3111662315","https://openalex.org/W3125246356","https://openalex.org/W3131801860","https://openalex.org/W3133942007","https://openalex.org/W3136421533","https://openalex.org/W3154016898","https://openalex.org/W3155700919","https://openalex.org/W3159662645","https://openalex.org/W3164257734","https://openalex.org/W3168714167","https://openalex.org/W3199894363","https://openalex.org/W3199935889","https://openalex.org/W3199952910","https://openalex.org/W3209445663","https://openalex.org/W3211349002","https://openalex.org/W3211349691","https://openalex.org/W4200227609","https://openalex.org/W4200604158","https://openalex.org/W4205221041","https://openalex.org/W4206326572","https://openalex.org/W4212812133","https://openalex.org/W4213082032","https://openalex.org/W4220746820","https://openalex.org/W4226463449","https://openalex.org/W4307178572","https://openalex.org/W4308156602","https://openalex.org/W4311882471","https://openalex.org/W4313652772","https://openalex.org/W4362454035","https://openalex.org/W4385282361","https://openalex.org/W4385827872","https://openalex.org/W4389572814","https://openalex.org/W4390730029","https://openalex.org/W4390841416","https://openalex.org/W4392634020","https://openalex.org/W4396705042","https://openalex.org/W4399294753","https://openalex.org/W4400834868","https://openalex.org/W4400900347","https://openalex.org/W4401326413"],"related_works":["https://openalex.org/W4311882471","https://openalex.org/W4411394217","https://openalex.org/W7116661979","https://openalex.org/W4390014174","https://openalex.org/W4376566196","https://openalex.org/W4399294753","https://openalex.org/W4401326413","https://openalex.org/W2336050635","https://openalex.org/W4313627900","https://openalex.org/W4285586998"],"abstract_inverted_index":{"Abstract":[0],"Solar\u2010driven":[1],"CO2":[2,32,52,57,140,156,179],"conversion":[3],"to":[4,39,138,165],"high\u2010value\u2010added":[5],"chemical":[6],"fuels":[7],"has":[8],"been":[9],"deemed":[10],"as":[11],"an":[12],"emerging":[13],"way":[14],"of":[15,26,51,56,71,88],"alleviating":[16],"deteriorating":[17],"energy":[18,184],"depletion":[19],"and":[20,48,60,99,134,152,172],"greenhouse":[21],"effect.":[22],"Nevertheless,":[23],"precise":[24],"modulation":[25],"spatial":[27],"vectorial":[28],"charge":[29,42,45,75,150],"migration/separation":[30],"in":[31],"artificial":[33,170],"photosystem":[34,77],"remains":[35],"challenging":[36],"due":[37],"predominantly":[38],"the":[40,69,108,122,139,144,149,154,174,178],"ultrashort":[41],"lifetime,":[43],"sluggish":[44],"transfer":[46],"kinetics,":[47],"ultra\u2010stable":[49],"symmetry":[50],"molecules,":[53],"rendering":[54],"stimulation":[55],"adsorption,":[58],"activation":[59],"reduction":[61],"a":[62,72,79,162],"grand":[63],"challenge.":[64],"Herein,":[65],"we":[66],"conceptually":[67],"demonstrate":[68],"design":[70],"novel":[73,168],"semiconductor\u2010insulator\u2010cocatalyst":[74],"tunneling":[76],"via":[78],"layer\u2010by\u2010layer":[80],"(LbL)":[81],"assembly":[82],"strategy,":[83],"which":[84],"involves":[85],"progressive":[86],"intercalation":[87],"dual":[89],"ultrathin":[90],"insulating":[91,123],"polymer":[92,124],"layers":[93],"in\u2010between":[94],"layered":[95],"double":[96],"hydroxides":[97],"(LDHs)":[98],"transition":[100],"metal":[101],"chalcogenide":[102],"(TMC).":[103],"It":[104],"is":[105],"demonstrated":[106],"for":[107],"first":[109],"time":[110],"unleash":[111],"that":[112],"electron\u2010hole":[113],"pairs":[114],"photoexcited":[115],"over":[116],"TMC":[117],"can":[118],"simultaneously":[119],"tunnel":[120],"through":[121],"interim":[125],"layers,":[126],"followed":[127],"by":[128,131],"holes":[129],"trapping":[130],"terminal":[132],"LDHs":[133],"directional":[135],"electrons":[136],"migration":[137],"molecules":[141],"absorbing":[142],"on":[143,177],"polymers":[145],"surface,":[146],"synergistically":[147],"boosting":[148],"separation":[151],"reinforcing":[153],"solar":[155,183],"reduction.":[157],"This":[158],"work":[159],"would":[160],"open":[161],"shining":[163],"frontier":[164],"strategically":[166],"craft":[167],"charge\u2010tunneling":[169],"photosystems":[171],"benefit":[173],"fundamental":[175],"understanding":[176],"photoreduction":[180],"technology":[181],"toward":[182],"conversion.":[185]},"counts_by_year":[{"year":2026,"cited_by_count":30},{"year":2025,"cited_by_count":16}],"updated_date":"2026-11-07T11:25:07.637180","created_date":"2025-02-27T00:00:00"}
