{"id":"https://openalex.org/W4361007474","doi":"https://doi.org/10.26434/chemrxiv-2023-t26wg","title":"Is there any correlation between impedance shapes and electrocatalytic activity?","display_name":"Is there any correlation between impedance shapes and electrocatalytic activity?","publication_year":2023,"publication_date":"2023-03-27","ids":{"openalex":"https://openalex.org/W4361007474","doi":"https://doi.org/10.26434/chemrxiv-2023-t26wg"},"language":"en","primary_location":{"id":"doi:10.26434/chemrxiv-2023-t26wg","doi":"https://doi.org/10.26434/chemrxiv-2023-t26wg","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2023-t26wg","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/641dd3a2647e3dca997293ce/original/is-there-any-correlation-between-impedance-shapes-and-electrocatalytic-activity.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by-nc-nd","license_id":"https://openalex.org/licenses/cc-by-nc-nd","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"},"volume":null,"type":"preprint","indexed_in":["crossref"],"open_access":{"is_oa":true,"oa_status":"green","oa_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/641dd3a2647e3dca997293ce/original/is-there-any-correlation-between-impedance-shapes-and-electrocatalytic-activity.pdf","any_repository_has_fulltext":true},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5052713328","display_name":"Jun Huang","orcid":"https://orcid.org/0000-0002-1668-5361","observed_orcids":["https://orcid.org/0000-0002-1668-5361","https://orcid.org/0000-0001-9190-9233"]},"institutions":[{"id":"https://openalex.org/I171892758","display_name":"Forschungszentrum J\u00fclich","ror":"https://ror.org/02nv7yv05","country_code":"DE","type":"facility","lineage":["https://openalex.org/I1305996414","https://openalex.org/I171892758"]},{"id":"https://openalex.org/I887968799","display_name":"RWTH Aachen University","ror":"https://ror.org/04xfq0f34","country_code":"DE","type":"education","lineage":["https://openalex.org/I887968799"]}],"countries":["DE"],"is_corresponding":true,"raw_author_name":"Jun Huang","raw_affiliation_strings":["Forschungszentrum J\u00fclich","RWTH Aachen University"],"raw_orcid":"https://orcid.org/0000-0002-1668-5361","affiliations":[{"raw_affiliation_string":"Forschungszentrum J\u00fclich","institution_ids":["https://openalex.org/I171892758"]},{"raw_affiliation_string":"RWTH Aachen University","institution_ids":["https://openalex.org/I887968799"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5052713328"],"corresponding_institution_ids":["https://openalex.org/I171892758","https://openalex.org/I887968799"],"apc_list":null,"apc_paid":null,"fwci":null,"has_fulltext":true,"cited_by_count":0,"citation_normalized_percentile":null,"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9818999767303467,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10030","display_name":"Electrocatalysts for Energy Conversion","score":0.9818999767303467,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11434","display_name":"Electrochemical Analysis and Applications","score":0.010400000028312206,"subfield":{"id":"https://openalex.org/subfields/1603","display_name":"Electrochemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10310","display_name":"Corrosion Behavior and Inhibition","score":0.0007999999797903001,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/electrocatalytic-activity","display_name":"electrocatalytic activity","score":0.8690000176429749},{"id":"https://openalex.org/keywords/electrochemical-impedance-spectroscopy","display_name":"electrochemical impedance spectroscopy","score":0.9120000004768372},{"id":"https://openalex.org/keywords/reaction-mechanism","display_name":"reaction mechanism","score":0.6679999828338623},{"id":"https://openalex.org/keywords/transfer-coefficient","display_name":"transfer coefficient","score":0.703000009059906},{"id":"https://openalex.org/keywords/regime-diagram","display_name":"regime diagram","score":0.8059999942779541},{"id":"https://openalex.org/keywords/side-reactions","display_name":"side reactions","score":0.7829999923706055},{"id":"https://openalex.org/keywords/circuit-modeling","display_name":"circuit modeling","score":0.6959999799728394}],"concepts":[{"id":"https://openalex.org/C7040849","wikidata":"https://www.wikidata.org/wiki/Q899580","display_name":"Dielectric spectroscopy","level":4,"score":0.7249050736427307},{"id":"https://openalex.org/C17829176","wikidata":"https://www.wikidata.org/wiki/Q179043","display_name":"Electrical impedance","level":2,"score":0.571847140789032},{"id":"https://openalex.org/C117251300","wikidata":"https://www.wikidata.org/wiki/Q1849855","display_name":"Parametric statistics","level":2,"score":0.5513996481895447},{"id":"https://openalex.org/C2778572836","wikidata":"https://www.wikidata.org/wiki/Q380933","display_name":"Space (punctuation)","level":2,"score":0.4385339319705963},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.42716965079307556},{"id":"https://openalex.org/C186399060","wikidata":"https://www.wikidata.org/wiki/Q959962","display_name":"Diagram","level":2,"score":0.4261326789855957},{"id":"https://openalex.org/C23572009","wikidata":"https://www.wikidata.org/wiki/Q964981","display_name":"Equivalent circuit","level":3,"score":0.41950535774230957},{"id":"https://openalex.org/C97355855","wikidata":"https://www.wikidata.org/wiki/Q11473","display_name":"Thermodynamics","level":1,"score":0.4118032455444336},{"id":"https://openalex.org/C52859227","wikidata":"https://www.wikidata.org/wiki/Q7877","display_name":"Electrochemistry","level":3,"score":0.3911433815956116},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.38207390904426575},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.37472838163375854},{"id":"https://openalex.org/C121864883","wikidata":"https://www.wikidata.org/wiki/Q677916","display_name":"Statistical physics","level":1,"score":0.35097622871398926},{"id":"https://openalex.org/C41008148","wikidata":"https://www.wikidata.org/wiki/Q21198","display_name":"Computer science","level":0,"score":0.2245994210243225},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.21116918325424194},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.20378610491752625},{"id":"https://openalex.org/C33923547","wikidata":"https://www.wikidata.org/wiki/Q395","display_name":"Mathematics","level":0,"score":0.19943088293075562},{"id":"https://openalex.org/C17525397","wikidata":"https://www.wikidata.org/wiki/Q176140","display_name":"Electrode","level":2,"score":0.17417848110198975},{"id":"https://openalex.org/C77088390","wikidata":"https://www.wikidata.org/wiki/Q8513","display_name":"Database","level":1,"score":0.0},{"id":"https://openalex.org/C111919701","wikidata":"https://www.wikidata.org/wiki/Q9135","display_name":"Operating system","level":1,"score":0.0},{"id":"https://openalex.org/C165801399","wikidata":"https://www.wikidata.org/wiki/Q25428","display_name":"Voltage","level":2,"score":0.0},{"id":"https://openalex.org/C105795698","wikidata":"https://www.wikidata.org/wiki/Q12483","display_name":"Statistics","level":1,"score":0.0},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.0}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.26434/chemrxiv-2023-t26wg","doi":"https://doi.org/10.26434/chemrxiv-2023-t26wg","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2023-t26wg","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/641dd3a2647e3dca997293ce/original/is-there-any-correlation-between-impedance-shapes-and-electrocatalytic-activity.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by-nc-nd","license_id":"https://openalex.org/licenses/cc-by-nc-nd","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"}],"best_oa_location":{"id":"doi:10.26434/chemrxiv-2023-t26wg","doi":"https://doi.org/10.26434/chemrxiv-2023-t26wg","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2023-t26wg","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/641dd3a2647e3dca997293ce/original/is-there-any-correlation-between-impedance-shapes-and-electrocatalytic-activity.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by-nc-nd","license_id":"https://openalex.org/licenses/cc-by-nc-nd","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"},"sustainable_development_goals":[],"sustainable_development_goals_aurora":[],"study_designs":[],"awards":[],"funders":[],"has_content":{"grobid_xml":true,"pdf":true},"content_urls":{"pdf":"https://content.openalex.org/works/W4361007474.pdf","grobid_xml":"https://content.openalex.org/works/W4361007474.grobid-xml"},"referenced_works_count":56,"referenced_works":["https://openalex.org/W1242529710","https://openalex.org/W1480171480","https://openalex.org/W1966484515","https://openalex.org/W1966815836","https://openalex.org/W1967678058","https://openalex.org/W1967914823","https://openalex.org/W1971436814","https://openalex.org/W1985162070","https://openalex.org/W1987222779","https://openalex.org/W1990547760","https://openalex.org/W1993698251","https://openalex.org/W2014305756","https://openalex.org/W2015752102","https://openalex.org/W2016366655","https://openalex.org/W2026125074","https://openalex.org/W2039140156","https://openalex.org/W2044142269","https://openalex.org/W2044530855","https://openalex.org/W2054724284","https://openalex.org/W2057925905","https://openalex.org/W2060805189","https://openalex.org/W2065187211","https://openalex.org/W2066043230","https://openalex.org/W2073207018","https://openalex.org/W2075219690","https://openalex.org/W2077727443","https://openalex.org/W2078978190","https://openalex.org/W2081115662","https://openalex.org/W2083812527","https://openalex.org/W2083908418","https://openalex.org/W2085623669","https://openalex.org/W2091775405","https://openalex.org/W2167103427","https://openalex.org/W2169574440","https://openalex.org/W2326134158","https://openalex.org/W2561476697","https://openalex.org/W2573377826","https://openalex.org/W2785768358","https://openalex.org/W2791707683","https://openalex.org/W2949437120","https://openalex.org/W2956067998","https://openalex.org/W2981486874","https://openalex.org/W3006422887","https://openalex.org/W3006469803","https://openalex.org/W3080766492","https://openalex.org/W3088980491","https://openalex.org/W3096270437","https://openalex.org/W3190395647","https://openalex.org/W3205490568","https://openalex.org/W4234783278","https://openalex.org/W4240182682","https://openalex.org/W4249477235","https://openalex.org/W4252329803","https://openalex.org/W4299392305","https://openalex.org/W4309768012","https://openalex.org/W4322734747"],"related_works":["https://openalex.org/W2568003367","https://openalex.org/W4382021005","https://openalex.org/W2068623945","https://openalex.org/W2896568827","https://openalex.org/W4243773385","https://openalex.org/W4206569389","https://openalex.org/W2050511751","https://openalex.org/W2117283676","https://openalex.org/W3202183310","https://openalex.org/W2393144863"],"abstract_inverted_index":{"Though":[0],"electrochemical":[1],"impedance":[2],"spectroscopy":[3],"(EIS)":[4],"has":[5],"been":[6],"widely":[7],"used":[8],"in":[9,62,114,131,160,172],"mechanistic":[10],"investigations":[11],"of":[12,20,33,39,46,71,88,101,106,129,134,144,167],"electrocatalytic":[13,25,34,72],"reactions,":[14],"the":[15,18,30,42,51,79,112,115,132,182],"correlation":[16,52],"between":[17],"shape":[19,67],"an":[21,37],"EIS":[22,66,104,161],"diagram":[23,100],"and":[24,44,58,74,92,152,170],"activity":[26],"is":[27,81,109],"largely":[28],"unclear;":[29],"rich":[31],"complexity":[32],"reactions":[35,91,108,121],"casts":[36],"air":[38],"pessimism":[40],"over":[41],"existence":[43],"stability":[45],"such":[47],"a":[48,69,84],"correlation.":[49],"Understanding":[50],"can":[53],"help":[54],"select":[55],"reaction":[56,168,173],"mechanisms":[57,169],"electrical":[59],"circuit":[60],"models":[61],"data":[63],"analysis,":[64],"use":[65],"as":[68],"descriptor":[70],"activity,":[73],"detect":[75],"side":[76],"reactions.":[77,96],"Herein,":[78],"problem":[80],"tackled":[82],"by":[83],"systematic":[85],"mathematical":[86],"analysis":[87,113],"firstly":[89],"single-adsorbate":[90,107,120],"then":[93],"more":[94],"complicated":[95],"A":[97],"complete":[98],"regime":[99],"all":[102],"possible":[103],"shapes":[105,162],"provided,":[110],"navigating":[111],"multi-dimensional":[116],"parametric":[117],"space.":[118],"For":[119],"involving":[122],"two":[123],"steps":[124],"with":[125],"identical":[126],"transfer":[127,150],"coefficients":[128,151],"0.5":[130],"absence":[133],"lateral":[135,153],"adsorbate":[136],"interactions,":[137],"several":[138,158],"rigorous":[139],"corollaries":[140],"are":[141,155,163],"derived.":[142],"Most":[143],"them":[145],"fail":[146],"miserably":[147],"when":[148],"different":[149],"interactions":[154],"considered.":[156],"Nevertheless,":[157],"trends":[159],"robust":[164],"against":[165],"complexities":[166],"variations":[171],"parameters,":[174],"which":[175],"also":[176],"receive":[177],"experimental":[178],"evidence":[179],"collected":[180],"from":[181],"literature.":[183]},"counts_by_year":[],"updated_date":"2026-10-17T09:40:24.721904","created_date":"2025-10-10T00:00:00"}