{"id":"https://openalex.org/W4294324903","doi":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","title":"Reintroducing diffusion to the collision theory for bimolecular reactions in diluted solutions","display_name":"Reintroducing diffusion to the collision theory for bimolecular reactions in diluted solutions","publication_year":2022,"publication_date":"2022-08-31","ids":{"openalex":"https://openalex.org/W4294324903","doi":"https://doi.org/10.26434/chemrxiv-2022-fdt7c"},"language":"en","primary_location":{"id":"doi:10.26434/chemrxiv-2022-fdt7c","doi":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/630bee5e11986ceefa49b9e2/original/reintroducing-diffusion-to-the-collision-theory-for-bimolecular-reactions-in-diluted-solutions.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"},"volume":null,"type":"preprint","indexed_in":["crossref"],"open_access":{"is_oa":true,"oa_status":"green","oa_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/630bee5e11986ceefa49b9e2/original/reintroducing-diffusion-to-the-collision-theory-for-bimolecular-reactions-in-diluted-solutions.pdf","any_repository_has_fulltext":true},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5088937367","display_name":"Jixin Chen","orcid":"https://orcid.org/0000-0001-7381-0918","observed_orcids":["https://orcid.org/0000-0001-7381-0918","https://orcid.org/0000-0003-1763-8644"]},"institutions":[{"id":"https://openalex.org/I4210106879","display_name":"Ohio University","ror":"https://ror.org/01jr3y717","country_code":"US","type":"education","lineage":["https://openalex.org/I4210106879"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Jixin Chen","raw_affiliation_strings":["Ohio University"],"raw_orcid":"https://orcid.org/0000-0001-7381-0918","affiliations":[{"raw_affiliation_string":"Ohio University","institution_ids":["https://openalex.org/I4210106879"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":1,"corresponding_author_ids":["https://openalex.org/A5088937367"],"corresponding_institution_ids":["https://openalex.org/I4210106879"],"apc_list":null,"apc_paid":null,"fwci":null,"has_fulltext":true,"cited_by_count":0,"citation_normalized_percentile":null,"cited_by_percentile_year":null,"biblio":{"volume":null,"issue":null,"first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T12044","display_name":"Advanced Physical and Chemical Molecular Interactions","score":0.7914999723434448,"subfield":{"id":"https://openalex.org/subfields/1606","display_name":"Physical and Theoretical Chemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T12044","display_name":"Advanced Physical and Chemical Molecular Interactions","score":0.7914999723434448,"subfield":{"id":"https://openalex.org/subfields/1606","display_name":"Physical and Theoretical Chemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T13187","display_name":"Diffusion and Search Dynamics","score":0.12780000269412994,"subfield":{"id":"https://openalex.org/subfields/1312","display_name":"Molecular Biology"},"field":{"id":"https://openalex.org/fields/13","display_name":"Biochemistry, Genetics and Molecular Biology"},"domain":{"id":"https://openalex.org/domains/1","display_name":"Life Sciences"}},{"id":"https://openalex.org/T13675","display_name":"Diffusion Coefficients in Liquids","score":0.04179999977350235,"subfield":{"id":"https://openalex.org/subfields/1607","display_name":"Spectroscopy"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/collision-theory","display_name":"collision theory","score":0.8619999885559082},{"id":"https://openalex.org/keywords/bimolecular-reactions","display_name":"bimolecular reactions","score":0.9440000057220459},{"id":"https://openalex.org/keywords/diffusion","display_name":"diffusion","score":0.3720000088214874},{"id":"https://openalex.org/keywords/reaction-kinetics","display_name":"reaction kinetics","score":0.7570000290870667},{"id":"https://openalex.org/keywords/dilute-solutions","display_name":"dilute solutions","score":0.7770000100135803},{"id":"https://openalex.org/keywords/collision-frequency","display_name":"collision frequency","score":0.9850000143051147},{"id":"https://openalex.org/keywords/collision-model","display_name":"collision model","score":0.39800000190734863}],"concepts":[{"id":"https://openalex.org/C121704057","wikidata":"https://www.wikidata.org/wiki/Q352070","display_name":"Collision","level":2,"score":0.7136712074279785},{"id":"https://openalex.org/C96618451","wikidata":"https://www.wikidata.org/wiki/Q3028008","display_name":"Dilution","level":2,"score":0.7031570672988892},{"id":"https://openalex.org/C69357855","wikidata":"https://www.wikidata.org/wiki/Q163214","display_name":"Diffusion","level":2,"score":0.6326514482498169},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.620225191116333},{"id":"https://openalex.org/C112951337","wikidata":"https://www.wikidata.org/wiki/Q5147502","display_name":"Collision frequency","level":3,"score":0.5469685792922974},{"id":"https://openalex.org/C150394285","wikidata":"https://www.wikidata.org/wiki/Q180254","display_name":"Adsorption","level":2,"score":0.5447902679443359},{"id":"https://openalex.org/C148898269","wikidata":"https://www.wikidata.org/wiki/Q1108792","display_name":"Kinetics","level":2,"score":0.5412895083427429},{"id":"https://openalex.org/C74134386","wikidata":"https://www.wikidata.org/wiki/Q907823","display_name":"Collision theory","level":3,"score":0.5193708539009094},{"id":"https://openalex.org/C175113610","wikidata":"https://www.wikidata.org/wiki/Q3394849","display_name":"Reaction rate","level":3,"score":0.4985692501068115},{"id":"https://openalex.org/C177801218","wikidata":"https://www.wikidata.org/wiki/Q36534","display_name":"Chemical reaction","level":2,"score":0.4983386993408203},{"id":"https://openalex.org/C36663273","wikidata":"https://www.wikidata.org/wiki/Q209082","display_name":"Chemical kinetics","level":3,"score":0.47537270188331604},{"id":"https://openalex.org/C32909587","wikidata":"https://www.wikidata.org/wiki/Q11369","display_name":"Molecule","level":2,"score":0.45635488629341125},{"id":"https://openalex.org/C143002175","wikidata":"https://www.wikidata.org/wiki/Q971184","display_name":"Smoluchowski coagulation equation","level":2,"score":0.44285744428634644},{"id":"https://openalex.org/C97355855","wikidata":"https://www.wikidata.org/wiki/Q11473","display_name":"Thermodynamics","level":1,"score":0.4423838257789612},{"id":"https://openalex.org/C154256306","wikidata":"https://www.wikidata.org/wiki/Q41795528","display_name":"Inert","level":2,"score":0.43966981768608093},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.4174365997314453},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.2910853624343872},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.21945622563362122},{"id":"https://openalex.org/C121864883","wikidata":"https://www.wikidata.org/wiki/Q677916","display_name":"Statistical physics","level":1,"score":0.19733673334121704},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.12798675894737244},{"id":"https://openalex.org/C74650414","wikidata":"https://www.wikidata.org/wiki/Q11397","display_name":"Classical mechanics","level":1,"score":0.1260870099067688},{"id":"https://openalex.org/C41008148","wikidata":"https://www.wikidata.org/wiki/Q21198","display_name":"Computer science","level":0,"score":0.09858128428459167},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.09504491090774536},{"id":"https://openalex.org/C38652104","wikidata":"https://www.wikidata.org/wiki/Q3510521","display_name":"Computer security","level":1,"score":0.0},{"id":"https://openalex.org/C145148216","wikidata":"https://www.wikidata.org/wiki/Q36496","display_name":"Ion","level":2,"score":0.0}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.26434/chemrxiv-2022-fdt7c","doi":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/630bee5e11986ceefa49b9e2/original/reintroducing-diffusion-to-the-collision-theory-for-bimolecular-reactions-in-diluted-solutions.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"}],"best_oa_location":{"id":"doi:10.26434/chemrxiv-2022-fdt7c","doi":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","is_oa":true,"landing_page_url":"https://doi.org/10.26434/chemrxiv-2022-fdt7c","pdf_url":"https://chemrxiv.org/engage/api-gateway/chemrxiv/assets/orp/resource/item/630bee5e11986ceefa49b9e2/original/reintroducing-diffusion-to-the-collision-theory-for-bimolecular-reactions-in-diluted-solutions.pdf","source":{"id":"https://openalex.org/S4393918830","display_name":"ChemRxiv","issn_l":"2573-2293","issn":["2573-2293"],"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":null,"host_organization_name":null,"host_organization_lineage":[],"host_organization_lineage_names":[],"type":"repository"},"license":"cc-by","license_id":"https://openalex.org/licenses/cc-by","version":"acceptedVersion","is_accepted":true,"is_published":false,"raw_source_name":null,"raw_type":"posted-content"},"sustainable_development_goals":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G3112304589","display_name":"Super-Resolution Optical Mapping for DNA Analysis Using Triplex-Forming Oligonucleotides as Stochastic Molecular Probes","funder_award_id":"R15HG009972","funder_id":"https://openalex.org/F4320337348","funder_display_name":"National Human Genome Research Institute"}],"funders":[{"id":"https://openalex.org/F4320332161","display_name":"National Institutes of Health","ror":"https://ror.org/01cwqze88"},{"id":"https://openalex.org/F4320337348","display_name":"National Human Genome Research Institute","ror":"https://ror.org/00baak391"}],"has_content":{"pdf":true,"grobid_xml":true},"content_urls":{"pdf":"https://content.openalex.org/works/W4294324903.pdf","grobid_xml":"https://content.openalex.org/works/W4294324903.grobid-xml"},"referenced_works_count":17,"referenced_works":["https://openalex.org/W8456792","https://openalex.org/W46860574","https://openalex.org/W561716561","https://openalex.org/W1576320143","https://openalex.org/W1621033879","https://openalex.org/W2004790462","https://openalex.org/W2025396755","https://openalex.org/W2034665579","https://openalex.org/W2050574242","https://openalex.org/W2057980421","https://openalex.org/W2099926307","https://openalex.org/W2172250191","https://openalex.org/W2469417314","https://openalex.org/W4205898344","https://openalex.org/W4230060386","https://openalex.org/W4234239026","https://openalex.org/W4240384253"],"related_works":["https://openalex.org/W4311580222","https://openalex.org/W4307251694","https://openalex.org/W7117412474","https://openalex.org/W2075871360","https://openalex.org/W4395677275","https://openalex.org/W347660838","https://openalex.org/W2131998091","https://openalex.org/W1987616212","https://openalex.org/W2054045522","https://openalex.org/W2090629368"],"abstract_inverted_index":{"Predicting":[0],"the":[1,53,79,94,106,126,138,144],"reaction":[2,8,54,64],"kinetics,":[3],"i.e.,":[4],"how":[5],"fast":[6],"a":[7,12,63,66,72,91,101,113,119,131],"can":[9],"happen":[10],"in":[11,34,40,65,89,112,147],"solution,":[13,75],"is":[14,84,98,123],"essential":[15],"information":[16],"for":[17],"many":[18],"processes,":[19],"such":[20,90],"as":[21,100],"industrial":[22],"chemical":[23],"manufacturing,":[24],"refining,":[25],"synthesis":[26],"and":[27,36,43,134],"separation":[28],"of":[29,56,109,128],"petroleum":[30],"products,":[31],"environmental":[32],"processes":[33],"air":[35],"water,":[37],"biological":[38],"reactions":[39,58],"cells,":[41],"biosensing,":[42],"drug":[44],"delivery.":[45],"Collision":[46],"theory":[47],"was":[48],"originally":[49],"developed":[50],"to":[51,86,104,136],"explain":[52,137],"kinetics":[55],"gas":[57,69],"with":[59],"no":[60],"dilution.":[61],"For":[62],"diluted":[67,73,114,148],"inert":[68],"solution":[70],"or":[71],"liquid":[74],"diffusion":[76,88],"often":[77],"dominates":[78],"collision":[80,107,121,139],"process.":[81],"Thus,":[82],"it":[83],"necessary":[85],"include":[87],"calculation.":[92],"Traditionally":[93],"classical":[95],"Smoluchowski":[96,145],"rate":[97],"used":[99,135],"starting":[102],"point":[103],"predict":[105],"frequency":[108,140],"two":[110],"molecules":[111,129],"solution.":[115,149],"In":[116],"this":[117],"report,":[118],"different":[120],"model":[122,146],"derived":[124],"from":[125],"adsorption":[127],"on":[130],"flat":[132],"surface":[133],"more":[141],"intuitively":[142],"than":[143]},"counts_by_year":[],"updated_date":"2026-10-30T12:39:25.321706","created_date":"2022-09-02T00:00:00"}
