{"id":"https://openalex.org/W4205544573","doi":"https://doi.org/10.1021/acs.nanolett.1c03569","title":"Regulating and Directionally Controlling Electron Emission from Gold Nanorods with Silica Coatings","display_name":"Regulating and Directionally Controlling Electron Emission from Gold Nanorods with Silica Coatings","publication_year":2022,"publication_date":"2022-01-06","ids":{"openalex":"https://openalex.org/W4205544573","doi":"https://doi.org/10.1021/acs.nanolett.1c03569","pmid":"https://pubmed.ncbi.nlm.nih.gov/34989588"},"language":"en","primary_location":{"id":"doi:10.1021/acs.nanolett.1c03569","doi":"https://doi.org/10.1021/acs.nanolett.1c03569","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.nanolett.1c03569","pdf_url":null,"source":{"id":"https://openalex.org/S143846845","display_name":"Nano Letters","issn_l":"1530-6984","issn":["1530-6984","1530-6992"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-2","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano Letters","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5073993022","display_name":"Fabio Medeghini","orcid":"https://orcid.org/0000-0002-0508-3365","observed_orcids":["https://orcid.org/0000-0002-0508-3365"]},"institutions":[{"id":"https://openalex.org/I1321296531","display_name":"National Institute of Standards and Technology","ror":"https://ror.org/05xpvk416","country_code":"US","type":"government","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065"]},{"id":"https://openalex.org/I137473845","display_name":"Joint Institute for Laboratory Astrophysics","ror":"https://ror.org/008hybe55","country_code":"US","type":"facility","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065","https://openalex.org/I137473845","https://openalex.org/I188538660"]},{"id":"https://openalex.org/I188538660","display_name":"University of Colorado Boulder","ror":"https://ror.org/02ttsq026","country_code":"US","type":"education","lineage":["https://openalex.org/I188538660"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Fabio Medeghini","raw_affiliation_strings":["JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I1321296531","https://openalex.org/I137473845","https://openalex.org/I188538660"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5055823881","display_name":"Jacob Pettine","orcid":"https://orcid.org/0000-0003-2102-1743","observed_orcids":["https://orcid.org/0000-0003-2102-1743"]},"institutions":[{"id":"https://openalex.org/I1321296531","display_name":"National Institute of Standards and Technology","ror":"https://ror.org/05xpvk416","country_code":"US","type":"government","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065"]},{"id":"https://openalex.org/I137473845","display_name":"Joint Institute for Laboratory Astrophysics","ror":"https://ror.org/008hybe55","country_code":"US","type":"facility","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065","https://openalex.org/I137473845","https://openalex.org/I188538660"]},{"id":"https://openalex.org/I188538660","display_name":"University of Colorado Boulder","ror":"https://ror.org/02ttsq026","country_code":"US","type":"education","lineage":["https://openalex.org/I188538660"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Jacob Pettine","raw_affiliation_strings":["Department of Physics, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Physics, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I188538660"]},{"raw_affiliation_string":"JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I1321296531","https://openalex.org/I137473845","https://openalex.org/I188538660"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5086561882","display_name":"Sean M. Meyer","orcid":"https://orcid.org/0000-0003-0771-5095","observed_orcids":["https://orcid.org/0000-0003-0771-5095"]},"institutions":[{"id":"https://openalex.org/I157725225","display_name":"University of Illinois Urbana-Champaign","ror":"https://ror.org/047426m28","country_code":"US","type":"education","lineage":["https://openalex.org/I157725225"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Sean M. Meyer","raw_affiliation_strings":["Department of Chemistry, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States"],"raw_orcid":"https://orcid.org/0000-0003-0771-5095","affiliations":[{"raw_affiliation_string":"Department of Chemistry, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States","institution_ids":["https://openalex.org/I157725225"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5030076676","display_name":"Catherine Jones Murphy","orcid":"https://orcid.org/0000-0001-7066-5575","observed_orcids":["https://orcid.org/0000-0001-7066-5575"]},"institutions":[{"id":"https://openalex.org/I157725225","display_name":"University of Illinois Urbana-Champaign","ror":"https://ror.org/047426m28","country_code":"US","type":"education","lineage":["https://openalex.org/I157725225"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Catherine J. Murphy","raw_affiliation_strings":["Department of Chemistry, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States","Materials Research Laboratory, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States"],"raw_orcid":"https://orcid.org/0000-0001-7066-5575","affiliations":[{"raw_affiliation_string":"Department of Chemistry, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States","institution_ids":["https://openalex.org/I157725225"]},{"raw_affiliation_string":"Materials Research Laboratory, University of Illinois at Urbana\u2212Champaign, Urbana, Illinois 61801, United States","institution_ids":["https://openalex.org/I157725225"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5084872177","display_name":"David J. Nesbitt","orcid":"https://orcid.org/0000-0001-5365-1120","observed_orcids":["https://orcid.org/0000-0001-5365-1120","https://orcid.org/0000-0003-3614-9723"]},"institutions":[{"id":"https://openalex.org/I1321296531","display_name":"National Institute of Standards and Technology","ror":"https://ror.org/05xpvk416","country_code":"US","type":"government","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065"]},{"id":"https://openalex.org/I137473845","display_name":"Joint Institute for Laboratory Astrophysics","ror":"https://ror.org/008hybe55","country_code":"US","type":"facility","lineage":["https://openalex.org/I1321296531","https://openalex.org/I1343035065","https://openalex.org/I137473845","https://openalex.org/I188538660"]},{"id":"https://openalex.org/I188538660","display_name":"University of Colorado Boulder","ror":"https://ror.org/02ttsq026","country_code":"US","type":"education","lineage":["https://openalex.org/I188538660"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"David J. Nesbitt","raw_affiliation_strings":["Department of Chemistry, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","Department of Physics, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States"],"raw_orcid":"https://orcid.org/0000-0001-5365-1120","affiliations":[{"raw_affiliation_string":"Department of Chemistry, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I188538660"]},{"raw_affiliation_string":"Department of Physics, University of Colorado\u2500Boulder, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I188538660"]},{"raw_affiliation_string":"JILA, University of Colorado\u2500Boulder and National Institute of Standards and Technology, Boulder, Colorado 80309, United States","institution_ids":["https://openalex.org/I1321296531","https://openalex.org/I137473845","https://openalex.org/I188538660"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":4,"corresponding_author_ids":["https://openalex.org/A5030076676","https://openalex.org/A5084872177"],"corresponding_institution_ids":["https://openalex.org/I1321296531","https://openalex.org/I137473845","https://openalex.org/I157725225","https://openalex.org/I188538660"],"apc_list":{"value":5000,"currency":"USD","value_usd":5000},"apc_paid":null,"fwci":0.6338,"has_fulltext":false,"cited_by_count":11,"citation_normalized_percentile":{"value":0.55975908,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":93,"max":98},"biblio":{"volume":"22","issue":"2","first_page":"644","last_page":"651"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10131","display_name":"Gold and Silver Nanoparticles Synthesis and Applications","score":0.6865000128746033,"subfield":{"id":"https://openalex.org/subfields/2504","display_name":"Electronic, Optical and Magnetic Materials"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10131","display_name":"Gold and Silver Nanoparticles Synthesis and Applications","score":0.6865000128746033,"subfield":{"id":"https://openalex.org/subfields/2504","display_name":"Electronic, Optical and Magnetic Materials"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10295","display_name":"Plasmonic and Surface Plasmon Research","score":0.22499999403953552,"subfield":{"id":"https://openalex.org/subfields/2204","display_name":"Biomedical Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11907","display_name":"Copper-based nanomaterials and applications","score":0.01940000057220459,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/gold-nanorods","display_name":"gold nanorods","score":0.9959999918937683},{"id":"https://openalex.org/keywords/silica-coating","display_name":"silica coating","score":0.9070000052452087},{"id":"https://openalex.org/keywords/mesoporous-silica","display_name":"mesoporous silica","score":0.9110000133514404},{"id":"https://openalex.org/keywords/photoemission","display_name":"photoemission","score":0.7850000262260437},{"id":"https://openalex.org/keywords/electron-escape-probability","display_name":"electron escape probability","score":0.7379999756813049},{"id":"https://openalex.org/keywords/coating-defects","display_name":"coating defects","score":0.625},{"id":"https://openalex.org/keywords/velocity-map-imaging","display_name":"velocity map imaging","score":0.7049999833106995},{"id":"https://openalex.org/keywords/nanoplasmonics","display_name":"nanoplasmonics","score":0.7760000228881836},{"id":"https://openalex.org/keywords/photocathodes","display_name":"photocathodes","score":0.7319999933242798},{"id":"https://openalex.org/keywords/nanocatalysis","display_name":"nanocatalysis","score":0.9139999747276306}],"concepts":[{"id":"https://openalex.org/C126201875","wikidata":"https://www.wikidata.org/wiki/Q2684948","display_name":"Nanorod","level":2,"score":0.9242409467697144},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.8190493583679199},{"id":"https://openalex.org/C2779845233","wikidata":"https://www.wikidata.org/wiki/Q3381567","display_name":"Photocurrent","level":2,"score":0.7614454627037048},{"id":"https://openalex.org/C45206210","wikidata":"https://www.wikidata.org/wiki/Q2415817","display_name":"Nanoscopic scale","level":2,"score":0.670788586139679},{"id":"https://openalex.org/C2781448156","wikidata":"https://www.wikidata.org/wiki/Q1570182","display_name":"Coating","level":2,"score":0.6093355417251587},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.6068491339683533},{"id":"https://openalex.org/C186187911","wikidata":"https://www.wikidata.org/wiki/Q1093894","display_name":"Nanostructure","level":2,"score":0.5571999549865723},{"id":"https://openalex.org/C82776694","wikidata":"https://www.wikidata.org/wiki/Q380049","display_name":"Mesoporous material","level":3,"score":0.5304412841796875},{"id":"https://openalex.org/C49040817","wikidata":"https://www.wikidata.org/wiki/Q193091","display_name":"Optoelectronics","level":1,"score":0.5241503715515137},{"id":"https://openalex.org/C2777496208","wikidata":"https://www.wikidata.org/wiki/Q17156473","display_name":"Mesoporous silica","level":4,"score":0.5235739946365356},{"id":"https://openalex.org/C147120987","wikidata":"https://www.wikidata.org/wiki/Q2225","display_name":"Electron","level":2,"score":0.4641135334968567},{"id":"https://openalex.org/C146088050","wikidata":"https://www.wikidata.org/wiki/Q744818","display_name":"Transmission electron microscopy","level":2,"score":0.4436095952987671},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.08736255764961243},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.0},{"id":"https://openalex.org/C55493867","wikidata":"https://www.wikidata.org/wiki/Q7094","display_name":"Biochemistry","level":1,"score":0.0},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.0},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.0}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/acs.nanolett.1c03569","doi":"https://doi.org/10.1021/acs.nanolett.1c03569","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.nanolett.1c03569","pdf_url":null,"source":{"id":"https://openalex.org/S143846845","display_name":"Nano Letters","issn_l":"1530-6984","issn":["1530-6984","1530-6992"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-2","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano Letters","raw_type":"journal-article"},{"id":"pmid:34989588","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/34989588","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano letters","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[],"sustainable_development_goals_aurora":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G1082731045","display_name":null,"funder_award_id":"PHY-1734006","funder_id":"https://openalex.org/F4320336454","funder_display_name":"Division of Physics"},{"id":"https://openalex.org/G759554275","display_name":null,"funder_award_id":"FA9550-15-1- 0090","funder_id":"https://openalex.org/F4320338279","funder_display_name":"Air Force Office of Scientific Research"}],"funders":[{"id":"https://openalex.org/F4320336454","display_name":"Division of Physics","ror":"https://ror.org/04ap5x931"},{"id":"https://openalex.org/F4320338279","display_name":"Air Force Office of Scientific Research","ror":"https://ror.org/011e9bt93"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":60,"referenced_works":["https://openalex.org/W1641577997","https://openalex.org/W1967239920","https://openalex.org/W1968273932","https://openalex.org/W1970181484","https://openalex.org/W1971881806","https://openalex.org/W1972502260","https://openalex.org/W1981864358","https://openalex.org/W1982443994","https://openalex.org/W1984193598","https://openalex.org/W1991656770","https://openalex.org/W1992315661","https://openalex.org/W2002664655","https://openalex.org/W2003035573","https://openalex.org/W2015357699","https://openalex.org/W2029399083","https://openalex.org/W2031171780","https://openalex.org/W2046537181","https://openalex.org/W2049983169","https://openalex.org/W2082760716","https://openalex.org/W2103098225","https://openalex.org/W2119767565","https://openalex.org/W2139516501","https://openalex.org/W2144723048","https://openalex.org/W2257878512","https://openalex.org/W2263602271","https://openalex.org/W2271925974","https://openalex.org/W2314143031","https://openalex.org/W2314438849","https://openalex.org/W2321636847","https://openalex.org/W2323143988","https://openalex.org/W2398762484","https://openalex.org/W2420216801","https://openalex.org/W2460690422","https://openalex.org/W2474718801","https://openalex.org/W2521875908","https://openalex.org/W2533206410","https://openalex.org/W2740356589","https://openalex.org/W2756463498","https://openalex.org/W2773511173","https://openalex.org/W2778345906","https://openalex.org/W2785250573","https://openalex.org/W2794044055","https://openalex.org/W2808852687","https://openalex.org/W2810763654","https://openalex.org/W2884275063","https://openalex.org/W2888701568","https://openalex.org/W2892036852","https://openalex.org/W2894807452","https://openalex.org/W2907755996","https://openalex.org/W2911918558","https://openalex.org/W2912363105","https://openalex.org/W2969829076","https://openalex.org/W2978166361","https://openalex.org/W2982399978","https://openalex.org/W3002532023","https://openalex.org/W3004964251","https://openalex.org/W3010652009","https://openalex.org/W3035975535","https://openalex.org/W3043512533","https://openalex.org/W3084357731"],"related_works":["https://openalex.org/W3035975535","https://openalex.org/W4200561002","https://openalex.org/W3189258601","https://openalex.org/W3024312624","https://openalex.org/W3043512533","https://openalex.org/W2002664655","https://openalex.org/W3184991787","https://openalex.org/W2346696201","https://openalex.org/W2076315673","https://openalex.org/W4200002314"],"abstract_inverted_index":{"Dielectric":[0],"coatings":[1,22,28,47,76],"offer":[2],"a":[3,54,64,106],"versatile":[4],"means":[5],"of":[6,57,66,127],"manipulating":[7],"hot":[8],"carrier":[9],"emission":[10,38],"from":[11,59],"nanoplasmonic":[12],"systems":[13],"for":[14,36,88,144],"emerging":[15],"nanocatalysis":[16],"and":[17,26,41,105],"photocathode":[18],"applications,":[19],"with":[20,74,129],"uniform":[21],"acting":[23],"as":[24,63],"regulators":[25],"nonuniform":[27],"providing":[29],"directional":[30],"photocurrent":[31,146],"control.":[32],"However,":[33],"the":[34,81,93,112,138,149],"mechanisms":[35],"electron":[37,113],"through":[39,92,116,137],"dense":[40,67,75],"mesoporous":[42,69,99],"silica":[43,70,94,100],"(SiO":[44],"2":[45],")":[46],"require":[48],"further":[49],"examination.":[50],"Here,":[51],"we":[52],"present":[53],"systematic":[55],"investigation":[56],"photoemission":[58,134],"single":[60],"gold":[61,78],"nanorods":[62,128],"function":[65],"versus":[68],"coating":[71,130],"thicknesses.":[72],"Studies":[73],"on":[77,148],"nanostructures":[79],"clarify":[80],"short":[82],"(\u223c1":[83],"nm)":[84],"attenuation":[85],"length":[86],"responsible":[87],"severely":[89],"reduced":[90],"transmission":[91],"conduction":[95],"band.":[96],"By":[97],"contrast,":[98],"is":[101],"much":[102],"more":[103],"transmissive,":[104],"simple":[107],"geometric":[108],"model":[109],"quantitatively":[110],"recapitulates":[111],"escape":[114],"probability":[115],"nanoscopic":[117],"porous":[118],"channels.":[119],"Finally,":[120],"photoelectron":[121],"velocity":[122],"map":[123],"imaging":[124],"(VMI)":[125],"studies":[126],"defects":[131],"verify":[132],"that":[133],"occurs":[135],"preferentially":[136],"thinner":[139],"regions,":[140],"illustrating":[141],"new":[142],"opportunities":[143],"designing":[145],"distributions":[147],"nanoscale.":[150]},"counts_by_year":[{"year":2024,"cited_by_count":3},{"year":2023,"cited_by_count":6},{"year":2022,"cited_by_count":2}],"updated_date":"2026-10-16T09:59:22.235173","created_date":"2022-01-26T00:00:00"}