{"id":"https://openalex.org/W3045468070","doi":"https://doi.org/10.1103/physrevmaterials.4.102601","title":"Yielding and bifurcated aging in nanofibrillar networks","display_name":"Yielding and bifurcated aging in nanofibrillar networks","publication_year":2020,"publication_date":"2020-10-28","ids":{"openalex":"https://openalex.org/W3045468070","doi":"https://doi.org/10.1103/physrevmaterials.4.102601","mag":"3045468070"},"language":"en","primary_location":{"id":"doi:10.1103/physrevmaterials.4.102601","doi":"https://doi.org/10.1103/physrevmaterials.4.102601","is_oa":false,"landing_page_url":"https://doi.org/10.1103/physrevmaterials.4.102601","pdf_url":null,"source":{"id":"https://openalex.org/S2786256796","display_name":"Physical Review Materials","issn_l":"2475-9953","issn":["2475-9953","2476-0455"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","norway-1","poland-70","russia-white-list-1"],"host_organization":"https://openalex.org/P4310320261","host_organization_name":"American Physical Society","host_organization_lineage":["https://openalex.org/P4310320261"],"host_organization_lineage_names":["American Physical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Physical Review Materials","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["arxiv","crossref","datacite"],"open_access":{"is_oa":true,"oa_status":"green","oa_url":"https://arxiv.org/pdf/2007.12763","any_repository_has_fulltext":true},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5006448711","display_name":"Ryan Poling\u2010Skutvik","orcid":"https://orcid.org/0000-0002-1614-1647","observed_orcids":["https://orcid.org/0000-0002-1614-1647"]},"institutions":[{"id":"https://openalex.org/I79576946","display_name":"University of Pennsylvania","ror":"https://ror.org/00b30xv10","country_code":"US","type":"education","lineage":["https://openalex.org/I79576946"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Ryan Poling-Skutvik","raw_affiliation_strings":["Department of Chemical and Biomolecular Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA"],"raw_orcid":"https://orcid.org/0000-0002-1614-1647","affiliations":[{"raw_affiliation_string":"Department of Chemical and Biomolecular Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5046804270","display_name":"E\u00f3in McEvoy","orcid":"https://orcid.org/0000-0002-8804-8177","observed_orcids":["https://orcid.org/0000-0002-8804-8177"]},"institutions":[{"id":"https://openalex.org/I79576946","display_name":"University of Pennsylvania","ror":"https://ror.org/00b30xv10","country_code":"US","type":"education","lineage":["https://openalex.org/I79576946"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Eoin McEvoy","raw_affiliation_strings":["Center for Engineering Mechanobiology, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Center for Engineering Mechanobiology, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]},{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5011906405","display_name":"Vivek B. Shenoy","orcid":"https://orcid.org/0000-0002-2645-1016","observed_orcids":["https://orcid.org/0000-0002-2645-1016"]},"institutions":[{"id":"https://openalex.org/I79576946","display_name":"University of Pennsylvania","ror":"https://ror.org/00b30xv10","country_code":"US","type":"education","lineage":["https://openalex.org/I79576946"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Vivek Shenoy","raw_affiliation_strings":["Center for Engineering Mechanobiology, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Center for Engineering Mechanobiology, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]},{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5006270385","display_name":"Chinedum O. Osuji","orcid":"https://orcid.org/0000-0003-0261-3065","observed_orcids":["https://orcid.org/0000-0003-0261-3065"]},"institutions":[{"id":"https://openalex.org/I79576946","display_name":"University of Pennsylvania","ror":"https://ror.org/00b30xv10","country_code":"US","type":"education","lineage":["https://openalex.org/I79576946"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Chinedum O. Osuji","raw_affiliation_strings":["Department of Chemical and Biomolecular Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Chemical and Biomolecular Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104, USA","institution_ids":["https://openalex.org/I79576946"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":1,"corresponding_author_ids":[],"corresponding_institution_ids":["https://openalex.org/I79576946"],"apc_list":null,"apc_paid":null,"fwci":0.2549,"has_fulltext":true,"cited_by_count":10,"citation_normalized_percentile":{"value":0.3528538,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":88,"max":98},"biblio":{"volume":"4","issue":"10","first_page":null,"last_page":null},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10610","display_name":"Advanced Cellulose Research Studies","score":0.6547999978065491,"subfield":{"id":"https://openalex.org/subfields/2502","display_name":"Biomaterials"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10610","display_name":"Advanced Cellulose Research Studies","score":0.6547999978065491,"subfield":{"id":"https://openalex.org/subfields/2502","display_name":"Biomaterials"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11379","display_name":"Rheology and Fluid Dynamics Studies","score":0.19859999418258667,"subfield":{"id":"https://openalex.org/subfields/1507","display_name":"Fluid Flow and Transfer Processes"},"field":{"id":"https://openalex.org/fields/15","display_name":"Chemical Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10474","display_name":"Material Dynamics and Properties","score":0.07509999722242355,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/yield-stress","display_name":"yield stress","score":0.9629999995231628},{"id":"https://openalex.org/keywords/bifurcation","display_name":"bifurcation","score":0.7850000262260437},{"id":"https://openalex.org/keywords/aging-materials","display_name":"aging materials","score":0.8109999895095825},{"id":"https://openalex.org/keywords/thixotropy","display_name":"thixotropy","score":0.8119999766349792},{"id":"https://openalex.org/keywords/disentanglement","display_name":"disentanglement","score":0.7009999752044678},{"id":"https://openalex.org/keywords/fibrillar-network","display_name":"fibrillar network","score":0.7160000205039978},{"id":"https://openalex.org/keywords/waiting-time","display_name":"waiting time","score":0.5630000233650208},{"id":"https://openalex.org/keywords/critical-stress","display_name":"critical stress","score":0.675000011920929},{"id":"https://openalex.org/keywords/entanglement-density","display_name":"entanglement density","score":0.6840000152587891},{"id":"https://openalex.org/keywords/disordered-materials","display_name":"disordered materials","score":0.6710000038146973},{"id":"https://openalex.org/keywords/time-dependent-behavior","display_name":"time-dependent behavior","score":0.3569999933242798}],"concepts":[{"id":"https://openalex.org/C2778049214","wikidata":"https://www.wikidata.org/wiki/Q7512234","display_name":"Sigma","level":2,"score":0.7922605872154236},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.7710886001586914},{"id":"https://openalex.org/C134121241","wikidata":"https://www.wikidata.org/wiki/Q899301","display_name":"Yield (engineering)","level":2,"score":0.6601077318191528},{"id":"https://openalex.org/C21036866","wikidata":"https://www.wikidata.org/wiki/Q181767","display_name":"Stress (linguistics)","level":2,"score":0.6375737190246582},{"id":"https://openalex.org/C121040770","wikidata":"https://www.wikidata.org/wiki/Q215675","display_name":"Quantum entanglement","level":3,"score":0.5053070187568665},{"id":"https://openalex.org/C87976508","wikidata":"https://www.wikidata.org/wiki/Q1498213","display_name":"Microstructure","level":2,"score":0.4403397738933563},{"id":"https://openalex.org/C26873012","wikidata":"https://www.wikidata.org/wiki/Q214781","display_name":"Condensed matter physics","level":1,"score":0.3984059989452362},{"id":"https://openalex.org/C121864883","wikidata":"https://www.wikidata.org/wiki/Q677916","display_name":"Statistical physics","level":1,"score":0.373540997505188},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.30726975202560425},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.18322372436523438},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.08076643943786621},{"id":"https://openalex.org/C84114770","wikidata":"https://www.wikidata.org/wiki/Q46344","display_name":"Quantum","level":2,"score":0.0},{"id":"https://openalex.org/C138885662","wikidata":"https://www.wikidata.org/wiki/Q5891","display_name":"Philosophy","level":0,"score":0.0},{"id":"https://openalex.org/C41895202","wikidata":"https://www.wikidata.org/wiki/Q8162","display_name":"Linguistics","level":1,"score":0.0}],"mesh":[],"locations_count":3,"locations":[{"id":"doi:10.1103/physrevmaterials.4.102601","doi":"https://doi.org/10.1103/physrevmaterials.4.102601","is_oa":false,"landing_page_url":"https://doi.org/10.1103/physrevmaterials.4.102601","pdf_url":null,"source":{"id":"https://openalex.org/S2786256796","display_name":"Physical Review Materials","issn_l":"2475-9953","issn":["2475-9953","2476-0455"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","norway-1","poland-70","russia-white-list-1"],"host_organization":"https://openalex.org/P4310320261","host_organization_name":"American Physical Society","host_organization_lineage":["https://openalex.org/P4310320261"],"host_organization_lineage_names":["American Physical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Physical Review Materials","raw_type":"journal-article"},{"id":"pmh:oai:arXiv.org:2007.12763","doi":null,"is_oa":true,"landing_page_url":"http://arxiv.org/abs/2007.12763","pdf_url":"https://arxiv.org/pdf/2007.12763","source":{"id":"https://openalex.org/S4306400194","display_name":"arXiv (Cornell University)","issn_l":"2331-8422","issn":["2331-8422"],"is_oa":true,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I205783295","host_organization_name":"Cornell University","host_organization_lineage":["https://openalex.org/I205783295"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"submittedVersion","is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"text"},{"id":"doi:10.48550/arxiv.2007.12763","doi":"https://doi.org/10.48550/arxiv.2007.12763","is_oa":true,"landing_page_url":"https://doi.org/10.48550/arxiv.2007.12763","pdf_url":null,"source":{"id":"https://openalex.org/S4306400194","display_name":"arXiv (Cornell University)","issn_l":"2331-8422","issn":["2331-8422"],"is_oa":true,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I205783295","host_organization_name":"Cornell University","host_organization_lineage":["https://openalex.org/I205783295"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":null,"is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"article-journal"}],"best_oa_location":{"id":"pmh:oai:arXiv.org:2007.12763","doi":null,"is_oa":true,"landing_page_url":"http://arxiv.org/abs/2007.12763","pdf_url":"https://arxiv.org/pdf/2007.12763","source":{"id":"https://openalex.org/S4306400194","display_name":"arXiv (Cornell University)","issn_l":"2331-8422","issn":["2331-8422"],"is_oa":true,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I205783295","host_organization_name":"Cornell University","host_organization_lineage":["https://openalex.org/I205783295"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"submittedVersion","is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":"text"},"sustainable_development_goals":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G1870677656","display_name":null,"funder_award_id":"CMMI: 15\u201048571","funder_id":"https://openalex.org/F4320306076","funder_display_name":"National Science Foundation"},{"id":"https://openalex.org/G2567800894","display_name":null,"funder_award_id":"DMR\u20101720530","funder_id":"https://openalex.org/F4320333422","funder_display_name":"Materials Research Science and Engineering Center, Harvard University"},{"id":"https://openalex.org/G4481177325","display_name":null,"funder_award_id":"15\u201348571","funder_id":"https://openalex.org/F4320337391","funder_display_name":"Division of Civil, Mechanical and Manufacturing Innovation"}],"funders":[{"id":"https://openalex.org/F4320306076","display_name":"National Science Foundation","ror":"https://ror.org/021nxhr62"},{"id":"https://openalex.org/F4320333422","display_name":"Materials Research Science and Engineering Center, Harvard University","ror":"https://ror.org/01qa5ep47"},{"id":"https://openalex.org/F4320337391","display_name":"Division of Civil, Mechanical and Manufacturing Innovation","ror":"https://ror.org/028yd4c30"}],"has_content":{"grobid_xml":true,"pdf":true},"content_urls":{"pdf":"https://content.openalex.org/works/W3045468070.pdf","grobid_xml":"https://content.openalex.org/works/W3045468070.grobid-xml"},"referenced_works_count":61,"referenced_works":["https://openalex.org/W189494361","https://openalex.org/W1539004828","https://openalex.org/W1653213478","https://openalex.org/W1785332051","https://openalex.org/W1975697874","https://openalex.org/W1976827080","https://openalex.org/W1986016321","https://openalex.org/W1986024456","https://openalex.org/W1987576086","https://openalex.org/W1987610434","https://openalex.org/W1988671390","https://openalex.org/W1993776218","https://openalex.org/W1994952188","https://openalex.org/W1996583965","https://openalex.org/W2001245625","https://openalex.org/W2002791142","https://openalex.org/W2006340321","https://openalex.org/W2022613733","https://openalex.org/W2025855717","https://openalex.org/W2028557999","https://openalex.org/W2030462673","https://openalex.org/W2036542429","https://openalex.org/W2041914224","https://openalex.org/W2046457747","https://openalex.org/W2052292106","https://openalex.org/W2065225076","https://openalex.org/W2070430913","https://openalex.org/W2075866529","https://openalex.org/W2086522572","https://openalex.org/W2093878161","https://openalex.org/W2111242220","https://openalex.org/W2115855885","https://openalex.org/W2125361970","https://openalex.org/W2126393142","https://openalex.org/W2130206554","https://openalex.org/W2144815200","https://openalex.org/W2150317163","https://openalex.org/W2175684487","https://openalex.org/W2209539636","https://openalex.org/W2221947135","https://openalex.org/W2431599800","https://openalex.org/W2473926928","https://openalex.org/W2508204386","https://openalex.org/W2548947358","https://openalex.org/W2570873504","https://openalex.org/W2763195259","https://openalex.org/W2770290347","https://openalex.org/W2782178842","https://openalex.org/W2784385082","https://openalex.org/W2785354276","https://openalex.org/W2807227931","https://openalex.org/W2888589461","https://openalex.org/W2892153306","https://openalex.org/W2897988151","https://openalex.org/W2923044739","https://openalex.org/W2935105928","https://openalex.org/W2943335962","https://openalex.org/W2945475794","https://openalex.org/W2950068980","https://openalex.org/W2962409944","https://openalex.org/W2977088262"],"related_works":["https://openalex.org/W2951452359","https://openalex.org/W7125566522","https://openalex.org/W2061211353","https://openalex.org/W2006340321","https://openalex.org/W7095178621","https://openalex.org/W984050439","https://openalex.org/W4403304570","https://openalex.org/W2242175232","https://openalex.org/W1988081498","https://openalex.org/W7221809921"],"abstract_inverted_index":{"Although":[0],"phenomenologically":[1],"simple":[2],"to":[3,11,75,92,115,131],"define,":[4],"the":[5,31,44,58,73,85,94,99,109,117,123,129,132,141,144,152,155,162],"yield":[6,45,62,100,164],"stress":[7,46,148,165],"is":[8,113],"often":[9],"difficult":[10],"quantify":[12],"unambiguously":[13],"in":[14,30,47,166],"practice,":[15],"especially":[16],"for":[17],"thixotropic":[18,173],"materials":[19,49],"with":[20,50,78],"complex":[21],"shear":[22,176],"histories.":[23],"Here,":[24],"we":[25,39],"identify":[26],"a":[27,105],"stress-controlled":[28],"bifurcation":[29],"yielding":[32,56,76,124],"response":[33,153],"of":[34,68,128,140,154,171],"cellulose":[35],"nanofibril":[36],"gels,":[37],"which":[38],"show":[40],"can":[41],"rigorously":[42],"localize":[43],"disordered":[48,168],"time-dependent":[51],"behavior.":[52],"After":[53],"an":[54],"initial":[55],"event,":[57],"fibrillar":[59],"networks":[60],"subsequently":[61],"faster":[63],"and":[64,82,125,137],"at":[65,104],"lower":[66],"magnitudes":[67],"stress.":[69,95,119],"For":[70,96],"low":[71],"stresses,":[72,98],"time":[74,80,101],"increases":[77],"waiting":[79],"${t}_{w}$":[81],"diverges":[83],"once":[84],"network":[86,111,130],"has":[87],"restored":[88],"sufficient":[89],"entanglement":[90],"density":[91,112],"support":[93,116],"higher":[97],"instead":[102],"plateaus":[103],"finite":[106],"value":[107],"because":[108],"developed":[110],"insufficient":[114],"applied":[118],"We":[120],"quantitatively":[121],"relate":[122],"aging":[126],"behavior":[127],"competition":[133],"between":[134,157],"stress-induced":[135],"disentanglement":[136],"dynamic":[138],"fluctuations":[139],"fibrils":[142],"rebuilding":[143],"network.":[145],"The":[146],"critical":[147],"${\\ensuremath{\\sigma}}_{c}$":[149],"that":[150],"bifurcates":[151],"material":[156],"these":[158,167],"two":[159],"states":[160],"identifies":[161],"intrinsic":[163],"materials,":[169],"independent":[170],"aging,":[172],"effects,":[174],"or":[175],"history.":[177]},"counts_by_year":[{"year":2026,"cited_by_count":1},{"year":2025,"cited_by_count":4},{"year":2024,"cited_by_count":1},{"year":2023,"cited_by_count":2},{"year":2022,"cited_by_count":1},{"year":2021,"cited_by_count":1}],"updated_date":"2026-11-05T12:25:35.769452","created_date":"2020-07-29T00:00:00"}
