{"id":"https://openalex.org/W2979464332","doi":"https://doi.org/10.1021/acs.accounts.9b00380","title":"Artificial Photosynthesis at Efficiencies Greatly Exceeding That of Natural Photosynthesis","display_name":"Artificial Photosynthesis at Efficiencies Greatly Exceeding That of Natural Photosynthesis","publication_year":2019,"publication_date":"2019-10-08","ids":{"openalex":"https://openalex.org/W2979464332","doi":"https://doi.org/10.1021/acs.accounts.9b00380","mag":"2979464332","pmid":"https://pubmed.ncbi.nlm.nih.gov/31593438"},"language":"en","primary_location":{"id":"doi:10.1021/acs.accounts.9b00380","doi":"https://doi.org/10.1021/acs.accounts.9b00380","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.accounts.9b00380","pdf_url":null,"source":{"id":"https://openalex.org/S145378405","display_name":"Accounts of Chemical Research","issn_l":"0001-4842","issn":["0001-4842","1520-4898"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Accounts of Chemical Research","raw_type":"journal-article"},"volume":null,"type":"review","indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5001120923","display_name":"Dilek K. Dogutan","orcid":"https://orcid.org/0000-0002-2935-4393","observed_orcids":["https://orcid.org/0000-0002-2935-4393"]},"institutions":[{"id":"https://openalex.org/I136199984","display_name":"Harvard University","ror":"https://ror.org/03vek6s52","country_code":"US","type":"education","lineage":["https://openalex.org/I136199984"]},{"id":"https://openalex.org/I2801851002","display_name":"Harvard University Press","ror":"https://ror.org/006v7bf86","country_code":"US","type":"other","lineage":["https://openalex.org/I136199984","https://openalex.org/I2801851002"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Dilek\nK. Dogutan","raw_affiliation_strings":["Harvard University , , 12 Oxford Street , , ,","Department of Chemistry and Chemical Biology, Harvard University, 12 Oxford Street, Cambridge, Massachusetts 02138-2902, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Harvard University , , 12 Oxford Street , , ,","institution_ids":["https://openalex.org/I136199984","https://openalex.org/I2801851002"]},{"raw_affiliation_string":"Department of Chemistry and Chemical Biology, Harvard University, 12 Oxford Street, Cambridge, Massachusetts 02138-2902, United States","institution_ids":["https://openalex.org/I136199984"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5056442308","display_name":"Daniel G. Nocera","orcid":"https://orcid.org/0000-0001-5055-320X","observed_orcids":["https://orcid.org/0000-0001-5055-320X"]},"institutions":[{"id":"https://openalex.org/I136199984","display_name":"Harvard University","ror":"https://ror.org/03vek6s52","country_code":"US","type":"education","lineage":["https://openalex.org/I136199984"]},{"id":"https://openalex.org/I2801851002","display_name":"Harvard University Press","ror":"https://ror.org/006v7bf86","country_code":"US","type":"other","lineage":["https://openalex.org/I136199984","https://openalex.org/I2801851002"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Daniel G. Nocera","raw_affiliation_strings":["Harvard University , , 12 Oxford Street , , ,","Department of Chemistry and Chemical Biology, Harvard University, 12 Oxford Street, Cambridge, Massachusetts 02138-2902, United States"],"raw_orcid":"https://orcid.org/0000-0001-5055-320X","affiliations":[{"raw_affiliation_string":"Harvard University , , 12 Oxford Street , , ,","institution_ids":["https://openalex.org/I136199984","https://openalex.org/I2801851002"]},{"raw_affiliation_string":"Department of Chemistry and Chemical Biology, Harvard University, 12 Oxford Street, Cambridge, Massachusetts 02138-2902, United States","institution_ids":["https://openalex.org/I136199984"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5056442308"],"corresponding_institution_ids":["https://openalex.org/I136199984","https://openalex.org/I2801851002"],"apc_list":{"value":5000,"currency":"USD","value_usd":5000},"apc_paid":null,"fwci":1.3821,"has_fulltext":false,"cited_by_count":397,"citation_normalized_percentile":{"value":0.78958333,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":99,"max":100},"biblio":{"volume":"52","issue":"11","first_page":"3143","last_page":"3148"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.7875999808311462,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.7875999808311462,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10303","display_name":"Photosynthetic Processes and Mechanisms","score":0.11569999903440475,"subfield":{"id":"https://openalex.org/subfields/1312","display_name":"Molecular Biology"},"field":{"id":"https://openalex.org/fields/13","display_name":"Biochemistry, Genetics and Molecular Biology"},"domain":{"id":"https://openalex.org/domains/1","display_name":"Life Sciences"}},{"id":"https://openalex.org/T11626","display_name":"Metalloenzymes and iron-sulfur proteins","score":0.051899999380111694,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/artificial-photosynthesis","display_name":"artificial photosynthesis","score":0.9990000128746033},{"id":"https://openalex.org/keywords/solar-water-splitting","display_name":"solar water splitting","score":0.6869999766349792},{"id":"https://openalex.org/keywords/artificial-leaf","display_name":"artificial leaf","score":0.7749999761581421},{"id":"https://openalex.org/keywords/photosystem-ii-oxygen-evolving-complex","display_name":"photosystem II oxygen-evolving complex","score":0.7599999904632568},{"id":"https://openalex.org/keywords/self-healing-catalysts","display_name":"self-healing catalysts","score":0.9309999942779541},{"id":"https://openalex.org/keywords/hydrogenase","display_name":"hydrogenase","score":0.3970000147819519},{"id":"https://openalex.org/keywords/cupriavidus-necator","display_name":"Cupriavidus necator","score":0.9129999876022339},{"id":"https://openalex.org/keywords/co2-fixation","display_name":"CO2 fixation","score":0.531000018119812},{"id":"https://openalex.org/keywords/solar-energy-conversion","display_name":"solar energy conversion","score":0.4169999957084656}],"concepts":[{"id":"https://openalex.org/C87803896","wikidata":"https://www.wikidata.org/wiki/Q654623","display_name":"Artificial photosynthesis","level":4,"score":0.8713704347610474},{"id":"https://openalex.org/C183688256","wikidata":"https://www.wikidata.org/wiki/Q11982","display_name":"Photosynthesis","level":2,"score":0.6841323375701904},{"id":"https://openalex.org/C35590869","wikidata":"https://www.wikidata.org/wiki/Q2697332","display_name":"Water splitting","level":4,"score":0.606103241443634},{"id":"https://openalex.org/C2776303644","wikidata":"https://www.wikidata.org/wiki/Q1020499","display_name":"Interfacing","level":2,"score":0.5331931114196777},{"id":"https://openalex.org/C541104983","wikidata":"https://www.wikidata.org/wiki/Q40015","display_name":"Solar energy","level":2,"score":0.5102107524871826},{"id":"https://openalex.org/C39432304","wikidata":"https://www.wikidata.org/wiki/Q188847","display_name":"Environmental science","level":0,"score":0.4197606146335602},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.4110249876976013},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.3725772202014923},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.2274324595928192},{"id":"https://openalex.org/C65165184","wikidata":"https://www.wikidata.org/wiki/Q218831","display_name":"Photocatalysis","level":3,"score":0.22391769289970398},{"id":"https://openalex.org/C18903297","wikidata":"https://www.wikidata.org/wiki/Q7150","display_name":"Ecology","level":1,"score":0.17875909805297852},{"id":"https://openalex.org/C41008148","wikidata":"https://www.wikidata.org/wiki/Q21198","display_name":"Computer science","level":0,"score":0.12807106971740723},{"id":"https://openalex.org/C86803240","wikidata":"https://www.wikidata.org/wiki/Q420","display_name":"Biology","level":0,"score":0.10743197798728943},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.07408574223518372},{"id":"https://openalex.org/C9390403","wikidata":"https://www.wikidata.org/wiki/Q3966","display_name":"Computer hardware","level":1,"score":0.0},{"id":"https://openalex.org/C55493867","wikidata":"https://www.wikidata.org/wiki/Q7094","display_name":"Biochemistry","level":1,"score":0.0}],"mesh":[{"descriptor_ui":"D001688","descriptor_name":"Biological Products","qualifier_ui":"Q000378","qualifier_name":"metabolism","is_major_topic":true},{"descriptor_ui":"D001688","descriptor_name":"Biological Products","qualifier_ui":"Q000737","qualifier_name":"chemistry","is_major_topic":false},{"descriptor_ui":"D010788","descriptor_name":"Photosynthesis","qualifier_ui":null,"qualifier_name":null,"is_major_topic":false},{"descriptor_ui":"D045332","descriptor_name":"Photosystem II Protein Complex","qualifier_ui":"Q000378","qualifier_name":"metabolism","is_major_topic":false},{"descriptor_ui":"D045332","descriptor_name":"Photosystem II Protein Complex","qualifier_ui":"Q000737","qualifier_name":"chemistry","is_major_topic":false}],"locations_count":2,"locations":[{"id":"doi:10.1021/acs.accounts.9b00380","doi":"https://doi.org/10.1021/acs.accounts.9b00380","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.accounts.9b00380","pdf_url":null,"source":{"id":"https://openalex.org/S145378405","display_name":"Accounts of Chemical Research","issn_l":"0001-4842","issn":["0001-4842","1520-4898"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Accounts of Chemical Research","raw_type":"journal-article"},{"id":"pmid:31593438","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/31593438","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Accounts of chemical research","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[{"display_name":"Affordable and clean energy","id":"https://metadata.un.org/sdg/7","score":0.9853000044822693},{"display_name":"Climate action","id":"https://metadata.un.org/sdg/13","score":0.4399999976158142}],"study_designs":[],"awards":[],"funders":[{"id":"https://openalex.org/F4320317864","display_name":"TomKat Foundation","ror":"https://ror.org/0108mj224"}],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":30,"referenced_works":["https://openalex.org/W1077411222","https://openalex.org/W1971113415","https://openalex.org/W1983101755","https://openalex.org/W1987446448","https://openalex.org/W1989500990","https://openalex.org/W2018959415","https://openalex.org/W2028201857","https://openalex.org/W2038591363","https://openalex.org/W2039481223","https://openalex.org/W2067238339","https://openalex.org/W2073128200","https://openalex.org/W2075580171","https://openalex.org/W2125645956","https://openalex.org/W2138111524","https://openalex.org/W2144305584","https://openalex.org/W2321284911","https://openalex.org/W2343163627","https://openalex.org/W2412520413","https://openalex.org/W2555006999","https://openalex.org/W2597651742","https://openalex.org/W2597732775","https://openalex.org/W2614884730","https://openalex.org/W2621908234","https://openalex.org/W2623208246","https://openalex.org/W2748504006","https://openalex.org/W2752114742","https://openalex.org/W2764073433","https://openalex.org/W2804287315","https://openalex.org/W2901030934","https://openalex.org/W2921275266"],"related_works":["https://openalex.org/W2159657691","https://openalex.org/W4306954532","https://openalex.org/W2469019039","https://openalex.org/W2038591363","https://openalex.org/W2736891633","https://openalex.org/W2189724662","https://openalex.org/W1501959408","https://openalex.org/W1941120611","https://openalex.org/W7054976816","https://openalex.org/W4300617559"],"abstract_inverted_index":{"Conspectus":[0],"Sunlight":[1],"is":[2,198],"an":[3,163,346],"abundant":[4],"energy":[5,33,265,274,304],"source":[6],"for":[7,82,202,210,236],"a":[8,302,317],"sustainable":[9],"society.":[10],"Indeed,":[11],"photosynthetic":[12,59,132,349],"organisms":[13],"harness":[14],"solar":[15,53,142,264],"radiation":[16],"to":[17,78,95,107,118,150,190,218,244,253,256,269,275,300],"build":[18],"the":[19,37,41,46,80,114,123,136,141,160,172,179,183,199,204,211,225,230,237,248,251,263,280,283,312,329,336,364],"world":[20],"around":[21],"us":[22],"by":[23,90],"synthesizing":[24],"energy-rich":[25],"compounds":[26],"from":[27,266,325,332],"water":[28,93,112,149,188,195,215,241,267,286],"and":[29,111,127,152,223,258,341,357],"CO2.":[30],"However,":[31],"numerous":[32],"conversion":[34],"bottlenecks":[35],"in":[36,122,247],"natural":[38,145,369],"system":[39],"limits":[40],"overall":[42],"efficiency":[43,305],"of":[44,56,125,144,148,167,176,182,214,240,282,314,335,368],"photosynthesis;":[45],"most":[47,173],"efficient":[48],"plants":[49],"do":[50],"not":[51],"exceed":[52,363],"storage":[54],"efficiencies":[55,360,367],"1%.":[57],"Artificial":[58,137,161,205,337],"solar-to-fuels":[60],"cycles":[61],"may":[62,87],"occur":[63],"at":[64,72,296,355],"higher":[65],"intrinsic":[66],"efficiencies,":[67],"but":[68],"they":[69],"typically":[70],"terminate":[71],"hydrogen,":[73],"with":[74,135,328],"no":[75],"process":[76,143],"installed":[77],"complete":[79],"cycle":[81,133],"carbon":[83,120,323],"fixation.":[84],"This":[85,130],"limitation":[86],"be":[88,191,254,270,290],"overcome":[89],"interfacing":[91,213,239],"solar-driven":[92],"splitting":[94,147,189,216,242,268,287],"H2-oxidizing":[96],"microorganisms.":[97],"To":[98,158],"this":[99],"end,":[100],"hybrid":[101,226,284],"biological\u2013inorganic":[102,227],"constructs":[103],"have":[104],"been":[105],"created":[106],"use":[108],"sunlight,":[109],"air,":[110,326],"as":[113,207,221,233],"only":[115],"starting":[116],"materials":[117,219],"accomplish":[119],"fixation":[121],"form":[124],"biomass":[126,340],"liquid":[128,342],"fuels.":[129],"artificial":[131,348],"begins":[134],"Leaf,":[138,162,206,232,338],"which":[139,177,197],"accomplishes":[140],"photosynthesis\ue5f8the":[146],"hydrogen":[151,252,294,330],"oxygen":[153,164,309],"using":[154,193],"sunlight\ue5f8under":[155],"ambient":[156],"conditions.":[157],"create":[159],"evolving":[165],"complex":[166],"Photosystem":[168],"II":[169],"was":[170,178],"mimicked,":[171],"important":[174],"property":[175],"self-healing":[180],"nature":[181],"catalyst.":[184],"Self-healing":[185],"catalysts":[186,288,334],"permit":[187],"accomplished":[192],"any":[194],"source,":[196],"critical":[200],"development":[201],"(1)":[203],"it":[208,234],"allows":[209,235],"facile":[212,238],"catalysis":[217,243],"such":[220,333],"silicon,":[222],"(2)":[224],"construct,":[228],"called":[229],"Bionic":[231,352],"bioorganisms.":[245],"Hydrogenases":[246],"bioorganism":[249],"allow":[250],"coupled":[255],"NADPH":[257],"ATP":[259],"production,":[260],"thus":[261,344],"allowing":[262],"converted":[271],"into":[272,339],"cellular":[273,277],"drive":[276],"biosynthesis.":[278],"In":[279],"design":[281],"system,":[285],"must":[289],"designed":[291],"that":[292,361],"support":[293],"generation":[295],"low":[297],"applied":[298],"potential":[299],"ensure":[301],"high":[303],"while":[306],"avoiding":[307],"reactive":[308],"species.":[310],"Using":[311],"tools":[313],"synthetic":[315],"biology,":[316],"bioengineered":[318],"bacterium,":[319],"Ralstonia":[320],"eutropha,":[321],"converts":[322],"dioxide":[324],"along":[327],"produced":[331],"fuels,":[343],"closing":[345],"entire":[347],"cycle.":[350],"The":[351],"Leaf":[353],"operates":[354],"solar-to-biomass":[356,366],"solar-to-liquid":[358],"fuels":[359],"greatly":[362],"highest":[365],"photosynthesis.":[370]},"counts_by_year":[{"year":2026,"cited_by_count":52},{"year":2025,"cited_by_count":71},{"year":2024,"cited_by_count":61},{"year":2023,"cited_by_count":70},{"year":2022,"cited_by_count":60},{"year":2021,"cited_by_count":46},{"year":2020,"cited_by_count":36}],"updated_date":"2026-11-04T10:54:05.112534","created_date":"2019-10-18T00:00:00"}
