{"id":"https://openalex.org/W2940879486","doi":"https://doi.org/10.1021/acsami.9b02771","title":"Greatly Enhanced Photoabsorption and Photothermal Conversion of Antimonene Quantum Dots through Spontaneously Partial Oxidation","display_name":"Greatly Enhanced Photoabsorption and Photothermal Conversion of Antimonene Quantum Dots through Spontaneously Partial Oxidation","publication_year":2019,"publication_date":"2019-04-26","ids":{"openalex":"https://openalex.org/W2940879486","doi":"https://doi.org/10.1021/acsami.9b02771","mag":"2940879486","pmid":"https://pubmed.ncbi.nlm.nih.gov/31025563"},"language":"en","primary_location":{"id":"doi:10.1021/acsami.9b02771","doi":"https://doi.org/10.1021/acsami.9b02771","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsami.9b02771","pdf_url":null,"source":{"id":"https://openalex.org/S164001016","display_name":"ACS Applied Materials & Interfaces","issn_l":"1944-8244","issn":["1944-8244","1944-8252"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Applied Materials & Interfaces","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5045012383","display_name":"Xianghong Niu","orcid":"https://orcid.org/0000-0001-6475-8839","observed_orcids":["https://orcid.org/0000-0001-6475-8839"]},"institutions":[{"id":"https://openalex.org/I41198531","display_name":"Nanjing University of Posts and Telecommunications","ror":"https://ror.org/043bpky34","country_code":"CN","type":"education","lineage":["https://openalex.org/I41198531"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Xianghong Niu","raw_affiliation_strings":["New Energy Technology Engineering Laboratory of Jiangsu Province & School of Science, Nanjing University of Posts and Telecommunications (NJUPT), Nanjing 210023, China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"New Energy Technology Engineering Laboratory of Jiangsu Province & School of Science, Nanjing University of Posts and Telecommunications (NJUPT), Nanjing 210023, China","institution_ids":["https://openalex.org/I41198531"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5101640730","display_name":"Yunhai Li","orcid":"https://orcid.org/0000-0003-4692-8114","observed_orcids":["https://orcid.org/0000-0003-4692-8114"]},"institutions":[{"id":"https://openalex.org/I76569877","display_name":"Southeast University","ror":"https://ror.org/04ct4d772","country_code":"CN","type":"education","lineage":["https://openalex.org/I76569877"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Yunhai Li","raw_affiliation_strings":["School of Physics, Southeast University, Nanjing 211189, China"],"raw_orcid":"https://orcid.org/0000-0003-4692-8114","affiliations":[{"raw_affiliation_string":"School of Physics, Southeast University, Nanjing 211189, China","institution_ids":["https://openalex.org/I76569877"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5101870977","display_name":"Yehui Zhang","orcid":"https://orcid.org/0009-0001-9198-2825","observed_orcids":["https://orcid.org/0009-0001-9198-2825"]},"institutions":[{"id":"https://openalex.org/I76569877","display_name":"Southeast University","ror":"https://ror.org/04ct4d772","country_code":"CN","type":"education","lineage":["https://openalex.org/I76569877"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Yehui Zhang","raw_affiliation_strings":["School of Physics, Southeast University, Nanjing 211189, China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Physics, Southeast University, Nanjing 211189, China","institution_ids":["https://openalex.org/I76569877"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5017958319","display_name":"Zhaobo Zhou","orcid":"https://orcid.org/0000-0003-2904-1845","observed_orcids":["https://orcid.org/0000-0003-2904-1845"]},"institutions":[{"id":"https://openalex.org/I76569877","display_name":"Southeast University","ror":"https://ror.org/04ct4d772","country_code":"CN","type":"education","lineage":["https://openalex.org/I76569877"]}],"countries":["CN"],"is_corresponding":false,"raw_author_name":"Zhaobo Zhou","raw_affiliation_strings":["School of Physics, Southeast University, Nanjing 211189, China"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Physics, Southeast University, Nanjing 211189, China","institution_ids":["https://openalex.org/I76569877"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5020585562","display_name":"Jinlan Wang","orcid":"https://orcid.org/0000-0002-4529-874X","observed_orcids":["https://orcid.org/0000-0002-4529-874X"]},"institutions":[{"id":"https://openalex.org/I76569877","display_name":"Southeast University","ror":"https://ror.org/04ct4d772","country_code":"CN","type":"education","lineage":["https://openalex.org/I76569877"]}],"countries":["CN"],"is_corresponding":true,"raw_author_name":"Jinlan Wang","raw_affiliation_strings":["School of Physics, Southeast University, Nanjing 211189, China"],"raw_orcid":"https://orcid.org/0000-0002-4529-874X","affiliations":[{"raw_affiliation_string":"School of Physics, Southeast University, Nanjing 211189, China","institution_ids":["https://openalex.org/I76569877"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5020585562"],"corresponding_institution_ids":["https://openalex.org/I76569877"],"apc_list":{"value":5000,"currency":"USD","value_usd":5000},"apc_paid":null,"fwci":1.7987,"has_fulltext":false,"cited_by_count":36,"citation_normalized_percentile":{"value":0.83705847,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":93,"max":99},"biblio":{"volume":"11","issue":"19","first_page":"17987","last_page":"17993"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10782","display_name":"Nanoplatforms for cancer theranostics","score":0.9771000146865845,"subfield":{"id":"https://openalex.org/subfields/2204","display_name":"Biomedical Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10782","display_name":"Nanoplatforms for cancer theranostics","score":0.9771000146865845,"subfield":{"id":"https://openalex.org/subfields/2204","display_name":"Biomedical Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10275","display_name":"2D Materials and Applications","score":0.01510000042617321,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10321","display_name":"Quantum Dots Synthesis And Properties","score":0.002300000051036477,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/two-dimensional-quantum-dots","display_name":"two-dimensional quantum dots","score":0.8930000066757202},{"id":"https://openalex.org/keywords/photothermal-conversion","display_name":"photothermal conversion","score":0.8610000014305115},{"id":"https://openalex.org/keywords/photothermal-therapy","display_name":"photothermal therapy","score":0.9459999799728394},{"id":"https://openalex.org/keywords/photoabsorption","display_name":"photon absorption","score":0.8360000252723694},{"id":"https://openalex.org/keywords/excited-state-dynamics","display_name":"excited-state dynamics","score":0.9549999833106995},{"id":"https://openalex.org/keywords/nonradiative-transitions","display_name":"radiationless transitions","score":0.6769999861717224},{"id":"https://openalex.org/keywords/band-edge-states","display_name":"band edge states","score":0.8899999856948853},{"id":"https://openalex.org/keywords/transition-dipole-moment","display_name":"transition dipole moment","score":0.9860000014305115},{"id":"https://openalex.org/keywords/nonadiabatic-dynamics","display_name":"nonadiabatic dynamics","score":0.7590000033378601},{"id":"https://openalex.org/keywords/time-dependent-density-functional-theory","display_name":"time-dependent density functional theory","score":0.8859999775886536}],"concepts":[{"id":"https://openalex.org/C182606246","wikidata":"https://www.wikidata.org/wiki/Q7187926","display_name":"Photothermal therapy","level":2,"score":0.8702206611633301},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.6873748898506165},{"id":"https://openalex.org/C124657808","wikidata":"https://www.wikidata.org/wiki/Q1133068","display_name":"Quantum dot","level":2,"score":0.578934371471405},{"id":"https://openalex.org/C173523689","wikidata":"https://www.wikidata.org/wiki/Q215589","display_name":"Dipole","level":2,"score":0.5408706068992615},{"id":"https://openalex.org/C152365726","wikidata":"https://www.wikidata.org/wiki/Q1048589","display_name":"Density functional theory","level":2,"score":0.5383352637290955},{"id":"https://openalex.org/C49874194","wikidata":"https://www.wikidata.org/wiki/Q5282045","display_name":"Discrete dipole approximation","level":3,"score":0.5272796750068665},{"id":"https://openalex.org/C181500209","wikidata":"https://www.wikidata.org/wiki/Q215328","display_name":"Excited state","level":2,"score":0.509023904800415},{"id":"https://openalex.org/C2777742735","wikidata":"https://www.wikidata.org/wiki/Q7187921","display_name":"Photothermal effect","level":3,"score":0.47634389996528625},{"id":"https://openalex.org/C125287762","wikidata":"https://www.wikidata.org/wiki/Q1758948","display_name":"Absorption (acoustics)","level":2,"score":0.45991483330726624},{"id":"https://openalex.org/C198990423","wikidata":"https://www.wikidata.org/wiki/Q331882","display_name":"Transition dipole moment","level":3,"score":0.4353374242782593},{"id":"https://openalex.org/C49040817","wikidata":"https://www.wikidata.org/wiki/Q193091","display_name":"Optoelectronics","level":1,"score":0.4065529406070709},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.374406635761261},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.36164432764053345},{"id":"https://openalex.org/C75473681","wikidata":"https://www.wikidata.org/wiki/Q188651","display_name":"Photochemistry","level":1,"score":0.33472198247909546},{"id":"https://openalex.org/C184779094","wikidata":"https://www.wikidata.org/wiki/Q26383","display_name":"Atomic physics","level":1,"score":0.2404029369354248},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.1796908676624298},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.1471557915210724},{"id":"https://openalex.org/C147597530","wikidata":"https://www.wikidata.org/wiki/Q369472","display_name":"Computational chemistry","level":1,"score":0.11926567554473877},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.0},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.0}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/acsami.9b02771","doi":"https://doi.org/10.1021/acsami.9b02771","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsami.9b02771","pdf_url":null,"source":{"id":"https://openalex.org/S164001016","display_name":"ACS Applied Materials & Interfaces","issn_l":"1944-8244","issn":["1944-8244","1944-8252"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Applied Materials & Interfaces","raw_type":"journal-article"},{"id":"pmid:31025563","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/31025563","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS applied materials & interfaces","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G5759921365","display_name":null,"funder_award_id":"NY219025","funder_id":"https://openalex.org/F4320323268","funder_display_name":"Nanjing University of Posts and Telecommunications"},{"id":"https://openalex.org/G6455872407","display_name":null,"funder_award_id":"2017YFA0204800","funder_id":"https://openalex.org/F4320321540","funder_display_name":"Ministry of Science and Technology of the People's Republic of China"},{"id":"https://openalex.org/G75599597","display_name":null,"funder_award_id":"21803032","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G7586777975","display_name":null,"funder_award_id":"21525311","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G7854832200","display_name":null,"funder_award_id":"21703032","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"},{"id":"https://openalex.org/G78644477","display_name":null,"funder_award_id":"BRA2016353","funder_id":"https://openalex.org/F4320321605","funder_display_name":"Government of Jiangsu Province"},{"id":"https://openalex.org/G8724205382","display_name":null,"funder_award_id":"BK20180735","funder_id":"https://openalex.org/F4320322769","funder_display_name":"Natural Science Foundation of Jiangsu Province"},{"id":"https://openalex.org/G8903996205","display_name":null,"funder_award_id":"21773027","funder_id":"https://openalex.org/F4320321001","funder_display_name":"National Natural Science Foundation of China"}],"funders":[{"id":"https://openalex.org/F4320321001","display_name":"National Natural Science Foundation of China","ror":"https://ror.org/01h0zpd94"},{"id":"https://openalex.org/F4320321540","display_name":"Ministry of Science and Technology of the People's Republic of China","ror":"https://ror.org/027s68j25"},{"id":"https://openalex.org/F4320321605","display_name":"Government of Jiangsu Province","ror":"https://ror.org/004svx814"},{"id":"https://openalex.org/F4320322769","display_name":"Natural Science Foundation of Jiangsu Province","ror":"https://ror.org/01h0zpd94"},{"id":"https://openalex.org/F4320323268","display_name":"Nanjing University of Posts and Telecommunications","ror":"https://ror.org/043bpky34"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":60,"referenced_works":["https://openalex.org/W1980107343","https://openalex.org/W1981368803","https://openalex.org/W1989306682","https://openalex.org/W1995734581","https://openalex.org/W1996294190","https://openalex.org/W2003133084","https://openalex.org/W2007395042","https://openalex.org/W2039774902","https://openalex.org/W2049397384","https://openalex.org/W2056612033","https://openalex.org/W2079753334","https://openalex.org/W2083222334","https://openalex.org/W2116373706","https://openalex.org/W2130567521","https://openalex.org/W2139622469","https://openalex.org/W2150345533","https://openalex.org/W2174451920","https://openalex.org/W2221415887","https://openalex.org/W2256619573","https://openalex.org/W2318724650","https://openalex.org/W2320589001","https://openalex.org/W2347099738","https://openalex.org/W2412158561","https://openalex.org/W2419191518","https://openalex.org/W2420753931","https://openalex.org/W2469788238","https://openalex.org/W2489951001","https://openalex.org/W2515369844","https://openalex.org/W2550660184","https://openalex.org/W2565535936","https://openalex.org/W2571894720","https://openalex.org/W2577934459","https://openalex.org/W2586121265","https://openalex.org/W2610217321","https://openalex.org/W2705497096","https://openalex.org/W2726462748","https://openalex.org/W2755286441","https://openalex.org/W2762935046","https://openalex.org/W2765225492","https://openalex.org/W2766321195","https://openalex.org/W2775062543","https://openalex.org/W2782504069","https://openalex.org/W2784246232","https://openalex.org/W2784945413","https://openalex.org/W2786058894","https://openalex.org/W2787832795","https://openalex.org/W2792597292","https://openalex.org/W2794058099","https://openalex.org/W2804959518","https://openalex.org/W2806648530","https://openalex.org/W2884534758","https://openalex.org/W2886785802","https://openalex.org/W2892182027","https://openalex.org/W2896904357","https://openalex.org/W2908340776","https://openalex.org/W2909391978","https://openalex.org/W2912455634","https://openalex.org/W2912863438","https://openalex.org/W4241885018","https://openalex.org/W4249297537"],"related_works":["https://openalex.org/W2705497096","https://openalex.org/W2754805959","https://openalex.org/W2754248634","https://openalex.org/W3033085934","https://openalex.org/W4392196572","https://openalex.org/W4213280254","https://openalex.org/W7129602479","https://openalex.org/W3119744641","https://openalex.org/W4200029675","https://openalex.org/W2999893287"],"abstract_inverted_index":{"Two-dimensional":[0],"quantum":[1],"dots":[2],"(2DQDs),":[3],"as":[4],"promising":[5],"photothermal":[6,10,26,76,142],"agents":[7],"(PTAs)":[8],"in":[9,162],"therapy":[11],"(PTT)":[12],"to":[13,71],"malignant":[14],"tumors,":[15],"have":[16],"been":[17],"widely":[18],"studied":[19],"experimentally,":[20],"whereas":[21],"the":[22,36,42,88,104,111,117,120,126,133,141],"superior":[23,80],"photoabsorption":[24,73],"and":[25,55,74,139,155],"conversion":[27,77,143],"mechanisms":[28],"remain":[29],"unclear.":[30],"In":[31],"this":[32],"work,":[33],"we":[34],"present":[35],"first":[37],"excited-state":[38],"dynamics":[39,60],"study":[40],"on":[41],"PTT":[43,81],"of":[44,83,135,152,160],"2D":[45],"antimonene":[46],"(AM)":[47],"QDs":[48],"by":[49],"employing":[50],"time-dependent":[51],"density":[52],"functional":[53],"theory":[54],"ab":[56],"initio":[57],"nonadiabatic":[58],"molecular":[59],"calculations.":[61],"Surprisingly,":[62],"pristine":[63],"AMQDs":[64,84],"themselves":[65],"are":[66],"not":[67,101],"good":[68],"PTAs":[69],"due":[70],"weak":[72],"low":[75],"performance.":[78],"The":[79,92,145],"capacity":[82],"actually":[85],"derives":[86],"from":[87,125],"spontaneously":[89],"partial":[90,93],"oxidation.":[91],"oxidation":[94,118],"introduces":[95],"additional":[96],"band":[97],"edge":[98],"states,":[99],"which":[100,130],"only":[102],"broaden":[103],"optical":[105],"absorption":[106],"range":[107],"but":[108],"also":[109],"strengthen":[110],"transition":[112,122],"dipole":[113],"moment.":[114],"More":[115],"importantly,":[116],"doubles":[119],"nonradiative":[121,128],"rate":[123],"arising":[124],"increased":[127],"coupling,":[129],"greatly":[131],"promotes":[132],"release":[134],"photogenerated":[136],"electron":[137],"energy":[138],"accelerates":[140],"efficiency.":[144],"in-depth":[146],"insight":[147],"unveiled":[148],"here":[149],"should":[150],"be":[151],"fundamental":[153],"importance":[154],"benefit":[156],"for":[157],"efficient":[158],"utilization":[159],"2DQDs":[161],"biomedical":[163],"field.":[164]},"counts_by_year":[{"year":2026,"cited_by_count":2},{"year":2025,"cited_by_count":3},{"year":2024,"cited_by_count":2},{"year":2023,"cited_by_count":6},{"year":2022,"cited_by_count":4},{"year":2021,"cited_by_count":5},{"year":2020,"cited_by_count":14}],"updated_date":"2026-11-04T10:54:05.112534","created_date":"2019-05-03T00:00:00"}