{"id":"https://openalex.org/W2904884735","doi":"https://doi.org/10.1021/acsami.8b14242","title":"Elucidating Lithium Alloying-Induced Degradation Evolution in High-Capacity Electrodes","display_name":"Elucidating Lithium Alloying-Induced Degradation Evolution in High-Capacity Electrodes","publication_year":2018,"publication_date":"2018-12-18","ids":{"openalex":"https://openalex.org/W2904884735","doi":"https://doi.org/10.1021/acsami.8b14242","mag":"2904884735","pmid":"https://pubmed.ncbi.nlm.nih.gov/30561180"},"language":"en","primary_location":{"id":"doi:10.1021/acsami.8b14242","doi":"https://doi.org/10.1021/acsami.8b14242","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsami.8b14242","pdf_url":null,"source":{"id":"https://openalex.org/S164001016","display_name":"ACS Applied Materials & Interfaces","issn_l":"1944-8244","issn":["1944-8244","1944-8252"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Applied Materials &amp; Interfaces","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5062790369","display_name":"Daniel Juarez Robles","orcid":"https://orcid.org/0000-0003-2746-5775","observed_orcids":["https://orcid.org/0000-0003-2746-5775"]},"institutions":[{"id":"https://openalex.org/I219193219","display_name":"Purdue University West Lafayette","ror":"https://ror.org/02dqehb95","country_code":"US","type":"education","lineage":["https://openalex.org/I219193219"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Daniel Juarez-Robles","raw_affiliation_strings":["School of Mechanical Engineering, Purdue University, West Lafayette, Indiana 47907, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"School of Mechanical Engineering, Purdue University, West Lafayette, Indiana 47907, United States","institution_ids":["https://openalex.org/I219193219"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5005884704","display_name":"Hernando J. Gonzalez Malabet","orcid":"https://orcid.org/0000-0003-4287-362X","observed_orcids":["https://orcid.org/0000-0003-4287-362X"]},"institutions":[{"id":"https://openalex.org/I82495205","display_name":"University of Alabama in Huntsville","ror":"https://ror.org/02zsxwr40","country_code":"US","type":"education","lineage":["https://openalex.org/I82495205"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Hernando J. Gonzalez-Malabet","raw_affiliation_strings":["Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States","institution_ids":["https://openalex.org/I82495205"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5010620214","display_name":"Matthew L\u2019Antigua","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I82495205","display_name":"University of Alabama in Huntsville","ror":"https://ror.org/02zsxwr40","country_code":"US","type":"education","lineage":["https://openalex.org/I82495205"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Matthew L\u2019Antigua","raw_affiliation_strings":["Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States","institution_ids":["https://openalex.org/I82495205"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5012460820","display_name":"Xianghui Xiao","orcid":"https://orcid.org/0000-0002-7142-3452","observed_orcids":["https://orcid.org/0000-0002-7142-3452","https://orcid.org/0009-0005-4621-8114"]},"institutions":[{"id":"https://openalex.org/I1282105669","display_name":"Argonne National Laboratory","ror":"https://ror.org/05gvnxz63","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166"]},{"id":"https://openalex.org/I4387156069","display_name":"Advanced Photon Source","ror":"https://ror.org/04qxsr837","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166","https://openalex.org/I4387156069"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Xianghui Xiao","raw_affiliation_strings":["Advanced Photon Source, Argonne National Laboratory, Lemont, Illinois 60439, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Advanced Photon Source, Argonne National Laboratory, Lemont, Illinois 60439, United States","institution_ids":["https://openalex.org/I1282105669","https://openalex.org/I4387156069"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5066219804","display_name":"George J. Nelson","orcid":"https://orcid.org/0000-0002-1170-245X","observed_orcids":["https://orcid.org/0000-0002-1170-245X"]},"institutions":[{"id":"https://openalex.org/I82495205","display_name":"University of Alabama in Huntsville","ror":"https://ror.org/02zsxwr40","country_code":"US","type":"education","lineage":["https://openalex.org/I82495205"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"George J. Nelson","raw_affiliation_strings":["Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Mechanical and Aerospace Engineering, The University of Alabama in Huntsville, Huntsville, Alabama 35899, United States","institution_ids":["https://openalex.org/I82495205"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5058780839","display_name":"Partha P. Mukherjee","orcid":"https://orcid.org/0000-0001-7900-7261","observed_orcids":["https://orcid.org/0000-0001-7900-7261"]},"institutions":[{"id":"https://openalex.org/I219193219","display_name":"Purdue University West Lafayette","ror":"https://ror.org/02dqehb95","country_code":"US","type":"education","lineage":["https://openalex.org/I219193219"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Partha P. Mukherjee","raw_affiliation_strings":["School of Mechanical Engineering, Purdue University, West Lafayette, Indiana 47907, United States"],"raw_orcid":"https://orcid.org/0000-0001-7900-7261","affiliations":[{"raw_affiliation_string":"School of Mechanical Engineering, Purdue University, West Lafayette, Indiana 47907, United States","institution_ids":["https://openalex.org/I219193219"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":4,"corresponding_author_ids":["https://openalex.org/A5058780839","https://openalex.org/A5066219804"],"corresponding_institution_ids":["https://openalex.org/I219193219","https://openalex.org/I82495205"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":0.574,"has_fulltext":false,"cited_by_count":12,"citation_normalized_percentile":{"value":0.65561903,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":89,"max":97},"biblio":{"volume":"11","issue":"1","first_page":"563","last_page":"577"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.9868000149726868,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.9868000149726868,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10663","display_name":"Advanced Battery Technologies Research","score":0.009800000116229057,"subfield":{"id":"https://openalex.org/subfields/2203","display_name":"Automotive Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":0.0003000000142492354,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/lithium-alloying","display_name":"lithium alloying","score":0.8270000219345093},{"id":"https://openalex.org/keywords/bronze","display_name":"bronze","score":0.6069999933242798},{"id":"https://openalex.org/keywords/cu6sn5","display_name":"Cu6Sn5","score":0.9549999833106995},{"id":"https://openalex.org/keywords/lithium-ion-battery-electrodes","display_name":"lithium-ion battery electrodes","score":0.7519999742507935},{"id":"https://openalex.org/keywords/capacity-fade","display_name":"capacity fade","score":0.6029999852180481},{"id":"https://openalex.org/keywords/particle-cracking","display_name":"particle cracking","score":0.5770000219345093},{"id":"https://openalex.org/keywords/volume-expansion","display_name":"volume expansion","score":0.8259999752044678},{"id":"https://openalex.org/keywords/x-ray-microtomography","display_name":"X-ray microtomography","score":0.7599999904632568},{"id":"https://openalex.org/keywords/electrode-microstructure","display_name":"electrode microstructure","score":0.6629999876022339},{"id":"https://openalex.org/keywords/cycling-stability","display_name":"cycling stability","score":0.3700000047683716}],"concepts":[{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.9114636182785034},{"id":"https://openalex.org/C17525397","wikidata":"https://www.wikidata.org/wiki/Q176140","display_name":"Electrode","level":2,"score":0.7137553691864014},{"id":"https://openalex.org/C2780026712","wikidata":"https://www.wikidata.org/wiki/Q37756","display_name":"Alloy","level":2,"score":0.6505899429321289},{"id":"https://openalex.org/C52859227","wikidata":"https://www.wikidata.org/wiki/Q7877","display_name":"Electrochemistry","level":3,"score":0.6223694682121277},{"id":"https://openalex.org/C2778541603","wikidata":"https://www.wikidata.org/wiki/Q152763","display_name":"Lithium (medication)","level":2,"score":0.5752142667770386},{"id":"https://openalex.org/C2779679103","wikidata":"https://www.wikidata.org/wiki/Q5251805","display_name":"Degradation (telecommunications)","level":2,"score":0.4852893054485321},{"id":"https://openalex.org/C7040849","wikidata":"https://www.wikidata.org/wiki/Q899580","display_name":"Dielectric spectroscopy","level":4,"score":0.4497582018375397},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.4369077980518341},{"id":"https://openalex.org/C544778455","wikidata":"https://www.wikidata.org/wiki/Q753","display_name":"Copper","level":2,"score":0.4221947193145752},{"id":"https://openalex.org/C2778517922","wikidata":"https://www.wikidata.org/wiki/Q7140482","display_name":"Particle (ecology)","level":2,"score":0.41054069995880127},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.3764382302761078},{"id":"https://openalex.org/C191897082","wikidata":"https://www.wikidata.org/wiki/Q11467","display_name":"Metallurgy","level":1,"score":0.36938905715942383},{"id":"https://openalex.org/C111368507","wikidata":"https://www.wikidata.org/wiki/Q43518","display_name":"Oceanography","level":1,"score":0.0},{"id":"https://openalex.org/C127413603","wikidata":"https://www.wikidata.org/wiki/Q11023","display_name":"Engineering","level":0,"score":0.0},{"id":"https://openalex.org/C76155785","wikidata":"https://www.wikidata.org/wiki/Q418","display_name":"Telecommunications","level":1,"score":0.0},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.0},{"id":"https://openalex.org/C41008148","wikidata":"https://www.wikidata.org/wiki/Q21198","display_name":"Computer science","level":0,"score":0.0},{"id":"https://openalex.org/C127313418","wikidata":"https://www.wikidata.org/wiki/Q1069","display_name":"Geology","level":0,"score":0.0},{"id":"https://openalex.org/C71924100","wikidata":"https://www.wikidata.org/wiki/Q11190","display_name":"Medicine","level":0,"score":0.0},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.0},{"id":"https://openalex.org/C134018914","wikidata":"https://www.wikidata.org/wiki/Q162606","display_name":"Endocrinology","level":1,"score":0.0}],"mesh":[],"locations_count":3,"locations":[{"id":"doi:10.1021/acsami.8b14242","doi":"https://doi.org/10.1021/acsami.8b14242","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acsami.8b14242","pdf_url":null,"source":{"id":"https://openalex.org/S164001016","display_name":"ACS Applied Materials & Interfaces","issn_l":"1944-8244","issn":["1944-8244","1944-8252"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-b","jufo-2","ki-jl-1","medline","norway-1","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS Applied Materials &amp; Interfaces","raw_type":"journal-article"},{"id":"pmid:30561180","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/30561180","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"ACS applied materials & interfaces","raw_type":"Journal Article"},{"id":"pmh:oai:osti.gov:1493904","doi":null,"is_oa":false,"landing_page_url":"https://www.osti.gov/biblio/1493904","pdf_url":null,"source":{"id":"https://openalex.org/S4306402487","display_name":"OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information)","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I139351228","host_organization_name":"Office of Scientific and Technical Information","host_organization_lineage":["https://openalex.org/I139351228"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"submittedVersion","is_accepted":false,"is_published":false,"raw_source_name":null,"raw_type":null}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[{"id":"https://openalex.org/G4967527041","display_name":null,"funder_award_id":"CBET-1438431","funder_id":"https://openalex.org/F4320337390","funder_display_name":"Division of Chemical, Bioengineering, Environmental, and Transport Systems"},{"id":"https://openalex.org/G7584148503","display_name":null,"funder_award_id":"CBET-1759651","funder_id":"https://openalex.org/F4320337390","funder_display_name":"Division of Chemical, Bioengineering, Environmental, and Transport Systems"},{"id":"https://openalex.org/G7696294809","display_name":null,"funder_award_id":"CBET-1438683","funder_id":"https://openalex.org/F4320337390","funder_display_name":"Division of Chemical, Bioengineering, Environmental, and Transport Systems"}],"funders":[{"id":"https://openalex.org/F4320337390","display_name":"Division of Chemical, Bioengineering, Environmental, and Transport Systems","ror":"https://ror.org/0471zv972"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":43,"referenced_works":["https://openalex.org/W1963483517","https://openalex.org/W1969767076","https://openalex.org/W1995277257","https://openalex.org/W1998062017","https://openalex.org/W2015387690","https://openalex.org/W2016203320","https://openalex.org/W2021172010","https://openalex.org/W2041378281","https://openalex.org/W2049797652","https://openalex.org/W2054073411","https://openalex.org/W2057730089","https://openalex.org/W2058295379","https://openalex.org/W2067291138","https://openalex.org/W2073588364","https://openalex.org/W2078997770","https://openalex.org/W2115169493","https://openalex.org/W2132414575","https://openalex.org/W2133427030","https://openalex.org/W2155041276","https://openalex.org/W2165160023","https://openalex.org/W2166415052","https://openalex.org/W2167279371","https://openalex.org/W2168639216","https://openalex.org/W2204677827","https://openalex.org/W2255079802","https://openalex.org/W2266888598","https://openalex.org/W2320189875","https://openalex.org/W2325818996","https://openalex.org/W2327740119","https://openalex.org/W2328954108","https://openalex.org/W2513384571","https://openalex.org/W2523292331","https://openalex.org/W2544568528","https://openalex.org/W2552065728","https://openalex.org/W2554501729","https://openalex.org/W2566344822","https://openalex.org/W2587302747","https://openalex.org/W2597724394","https://openalex.org/W2606141856","https://openalex.org/W2610728007","https://openalex.org/W2620860707","https://openalex.org/W2690661596","https://openalex.org/W2798241172"],"related_works":["https://openalex.org/W3175842110","https://openalex.org/W2382608692","https://openalex.org/W2785219487","https://openalex.org/W3045361098","https://openalex.org/W2509096556","https://openalex.org/W2949171006","https://openalex.org/W2017920784","https://openalex.org/W2352756011","https://openalex.org/W4237079982","https://openalex.org/W2008175066"],"abstract_inverted_index":{"Alloy":[0],"electrode":[1,57,99,124],"materials":[2],"offer":[3],"high":[4],"capacity":[5,109],"in":[6,15],"lithium-ion":[7],"batteries;":[8],"however,":[9,148,174],"they":[10],"exhibit":[11],"rapid":[12,108],"degradation":[13,30,118],"resulting":[14],"particle":[16,158],"disintegration":[17],"and":[18,42,65,77,79,83,88,95,142,156,160],"electrochemical":[19,41,66,184],"performance":[20,67,185],"decay.":[21,186],"In":[22],"this":[23,149],"study,":[24],"the":[25,120,123,144,171,178,182],"evolution":[26,101],"of":[27,86,119,170],"lithium":[28],"alloying-induced":[29],"due":[31],"to":[32,113,125,151,166,181],"electrochemomechanical":[33],"interactions":[34],"is":[35,51],"examined":[36,69],"based":[37],"on":[38],"a":[39,126,152,168],"multipronged":[40],"microstructural":[43,100],"analysis.":[44],"Copper\u2013tin":[45],"(Cu":[46],"6":[47],"Sn":[48],"5":[49],")":[50,137],"chosen":[52],"as":[53],"an":[54],"exemplary":[55],"alloy":[56,140,172],"material.":[58],"Electrodes":[59],"with":[60],"compositional":[61],"variations":[62],"were":[63,91],"fabricated,":[64],"was":[68,102,111,164,176],"under":[70],"varying":[71],"conditions":[72],"including":[73],"voltage":[74],"window,":[75],"C-rate,":[76],"short-":[78],"long-term":[80],"cycling.":[81],"Morphology":[82],"composition":[84],"analyses":[85],"pristine":[87],"cycled":[89],"electrodes":[90],"conducted":[92],"using":[93,104],"micrography":[94],"spectroscopy":[96],"techniques.":[97],"Alloying-induced":[98],"probed":[103],"X-ray":[105],"microtomography.":[106],"The":[107],"fading":[110],"found":[112,165],"be":[114,167],"caused":[115],"by":[116],"mechanical":[117],"electrode.":[121],"Driving":[122],"lower":[127],"potential":[128],"(":[129],"E":[130],"\u2248":[131],"0.2":[132],"V":[133],"vs":[134],"Li/Li":[135],"+":[136],"induced":[138],"Li\u2013Sn":[139],"formation":[141],"provided":[143],"characteristic":[145],"large":[146,153],"capacity;":[147],"led":[150],"volume":[154],"expansion":[155],"active":[157],"cracking":[159],"disintegration.":[161],"Copper":[162],"expulsion":[163],"consequence":[169],"formation;":[173],"it":[175],"not":[177],"primary":[179],"contributor":[180],"dramatic":[183]},"counts_by_year":[{"year":2026,"cited_by_count":1},{"year":2025,"cited_by_count":2},{"year":2024,"cited_by_count":1},{"year":2022,"cited_by_count":2},{"year":2021,"cited_by_count":2},{"year":2020,"cited_by_count":3},{"year":2019,"cited_by_count":1}],"updated_date":"2026-10-27T15:51:10.671819","created_date":"2018-12-22T00:00:00"}
