{"id":"https://openalex.org/W2613136397","doi":"https://doi.org/10.1021/acs.nanolett.7b01546","title":"Atomic Resolution Structural and Chemical Imaging Revealing the Sequential Migration of Ni, Co, and Mn upon the Battery Cycling of Layered Cathode","display_name":"Atomic Resolution Structural and Chemical Imaging Revealing the Sequential Migration of Ni, Co, and Mn upon the Battery Cycling of Layered Cathode","publication_year":2017,"publication_date":"2017-05-09","ids":{"openalex":"https://openalex.org/W2613136397","doi":"https://doi.org/10.1021/acs.nanolett.7b01546","mag":"2613136397","pmid":"https://pubmed.ncbi.nlm.nih.gov/28485969"},"language":"en","primary_location":{"id":"doi:10.1021/acs.nanolett.7b01546","doi":"https://doi.org/10.1021/acs.nanolett.7b01546","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.nanolett.7b01546","pdf_url":null,"source":{"id":"https://openalex.org/S143846845","display_name":"Nano Letters","issn_l":"1530-6984","issn":["1530-6984","1530-6992"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-2","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano Letters","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5086670941","display_name":"Pengfei Yan","orcid":"https://orcid.org/0000-0001-6387-7502","observed_orcids":["https://orcid.org/0000-0001-6387-7502","https://orcid.org/0009-0007-4503-2945"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I2801280572","display_name":"Environmental Molecular Sciences Laboratory","ror":"https://ror.org/04rc0xn13","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I2801280572","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Pengfei Yan","raw_affiliation_strings":["Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States","institution_ids":["https://openalex.org/I142606810","https://openalex.org/I2801280572"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5023144456","display_name":"Jianming Zheng","orcid":"https://orcid.org/0000-0002-4928-8194","observed_orcids":["https://orcid.org/0000-0002-4928-8194"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I2801280572","display_name":"Environmental Molecular Sciences Laboratory","ror":"https://ror.org/04rc0xn13","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I2801280572","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Jianming Zheng","raw_affiliation_strings":["Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States","institution_ids":["https://openalex.org/I142606810","https://openalex.org/I2801280572"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5032583158","display_name":"Ji\u2010Guang Zhang","orcid":"https://orcid.org/0000-0001-7343-4609","observed_orcids":["https://orcid.org/0000-0001-7343-4609"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I2801280572","display_name":"Environmental Molecular Sciences Laboratory","ror":"https://ror.org/04rc0xn13","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I2801280572","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Ji-Guang Zhang","raw_affiliation_strings":["Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States"],"raw_orcid":"https://orcid.org/0000-0001-7343-4609","affiliations":[{"raw_affiliation_string":"Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States","institution_ids":["https://openalex.org/I142606810","https://openalex.org/I2801280572"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5100622274","display_name":"Chongmin Wang","orcid":"https://orcid.org/0000-0003-3327-0958","observed_orcids":["https://orcid.org/0000-0003-3327-0958"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I2801280572","display_name":"Environmental Molecular Sciences Laboratory","ror":"https://ror.org/04rc0xn13","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I2801280572","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Chongmin Wang","raw_affiliation_strings":["Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States"],"raw_orcid":"https://orcid.org/0000-0003-3327-0958","affiliations":[{"raw_affiliation_string":"Environmental\rMolecular Sciences Laboratory, \u2021Energy and Environment Directorate, Pacific Northwest National Laboratory, 902 Battelle Boulevard, Richland, Washington 99354, United States","institution_ids":["https://openalex.org/I142606810","https://openalex.org/I2801280572"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5100622274"],"corresponding_institution_ids":["https://openalex.org/I142606810","https://openalex.org/I2801280572"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":9.174,"has_fulltext":false,"cited_by_count":172,"citation_normalized_percentile":{"value":0.98502242,"is_in_top_1_percent":false,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":96,"max":100},"biblio":{"volume":"17","issue":"6","first_page":"3946","last_page":"3951"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.9937000274658203,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10018","display_name":"Advancements in Battery Materials","score":0.9937000274658203,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10663","display_name":"Advanced Battery Technologies Research","score":0.0017999999690800905,"subfield":{"id":"https://openalex.org/subfields/2203","display_name":"Automotive Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10281","display_name":"Advanced Battery Materials and Technologies","score":0.001500000013038516,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/layered-lithium-transition-metal-oxide","display_name":"layered lithium transition metal oxide","score":0.8230000138282776},{"id":"https://openalex.org/keywords/lini1-3co1-3mn1-3o2","display_name":"LiNi1/3Co1/3Mn1/3O2","score":0.9309999942779541},{"id":"https://openalex.org/keywords/layered-oxide-cathodes","display_name":"layered oxide cathodes","score":0.5879999995231628},{"id":"https://openalex.org/keywords/lattice-disordering","display_name":"lattice disordering","score":0.8349999785423279},{"id":"https://openalex.org/keywords/solid-electrolyte-interphase","display_name":"solid electrolyte interphase","score":0.640999972820282},{"id":"https://openalex.org/keywords/oxygen-vacancies","display_name":"oxygen vacancies","score":0.7289999723434448},{"id":"https://openalex.org/keywords/capacity-fade","display_name":"capacity fade","score":0.46799999475479126},{"id":"https://openalex.org/keywords/voltage-fade","display_name":"voltage fade","score":0.7429999709129333}],"concepts":[{"id":"https://openalex.org/C49110097","wikidata":"https://www.wikidata.org/wiki/Q175233","display_name":"Cathode","level":2,"score":0.7527451515197754},{"id":"https://openalex.org/C145148216","wikidata":"https://www.wikidata.org/wiki/Q36496","display_name":"Ion","level":2,"score":0.5768799781799316},{"id":"https://openalex.org/C66823137","wikidata":"https://www.wikidata.org/wiki/Q757568","display_name":"Atomic units","level":2,"score":0.5399588942527771},{"id":"https://openalex.org/C68801617","wikidata":"https://www.wikidata.org/wiki/Q162908","display_name":"Electrolyte","level":3,"score":0.5353342294692993},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.5322791337966919},{"id":"https://openalex.org/C178187954","wikidata":"https://www.wikidata.org/wiki/Q902328","display_name":"Electron energy loss spectroscopy","level":3,"score":0.4881513714790344},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.47762173414230347},{"id":"https://openalex.org/C555008776","wikidata":"https://www.wikidata.org/wiki/Q267298","display_name":"Battery (electricity)","level":3,"score":0.4654363691806793},{"id":"https://openalex.org/C106773901","wikidata":"https://www.wikidata.org/wiki/Q19588","display_name":"Transition metal","level":3,"score":0.42832377552986145},{"id":"https://openalex.org/C155673373","wikidata":"https://www.wikidata.org/wiki/Q1648886","display_name":"Structural stability","level":2,"score":0.41525959968566895},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.3312099575996399},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.2880939841270447},{"id":"https://openalex.org/C17525397","wikidata":"https://www.wikidata.org/wiki/Q176140","display_name":"Electrode","level":2,"score":0.19054949283599854},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.13573315739631653},{"id":"https://openalex.org/C146088050","wikidata":"https://www.wikidata.org/wiki/Q744818","display_name":"Transmission electron microscopy","level":2,"score":0.0},{"id":"https://openalex.org/C127413603","wikidata":"https://www.wikidata.org/wiki/Q11023","display_name":"Engineering","level":0,"score":0.0},{"id":"https://openalex.org/C66938386","wikidata":"https://www.wikidata.org/wiki/Q633538","display_name":"Structural engineering","level":1,"score":0.0},{"id":"https://openalex.org/C55493867","wikidata":"https://www.wikidata.org/wiki/Q7094","display_name":"Biochemistry","level":1,"score":0.0},{"id":"https://openalex.org/C163258240","wikidata":"https://www.wikidata.org/wiki/Q25342","display_name":"Power (physics)","level":2,"score":0.0},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.0},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.0},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.0},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.0}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/acs.nanolett.7b01546","doi":"https://doi.org/10.1021/acs.nanolett.7b01546","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.nanolett.7b01546","pdf_url":null,"source":{"id":"https://openalex.org/S143846845","display_name":"Nano Letters","issn_l":"1530-6984","issn":["1530-6984","1530-6992"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-2","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano Letters","raw_type":"journal-article"},{"id":"pmid:28485969","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/28485969","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Nano letters","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[{"score":0.75,"display_name":"Affordable and clean energy","id":"https://metadata.un.org/sdg/7"}],"sustainable_development_goals_aurora":[{"score":0.6000000238418579,"display_name":"Affordable and clean energy","id":"https://metadata.un.org/sdg/7"}],"study_designs":[],"awards":[{"id":"https://openalex.org/G343155448","display_name":null,"funder_award_id":"DE-AC02-05CH 11231","funder_id":"https://openalex.org/F4320336521","funder_display_name":"Vehicle Technologies Program"}],"funders":[{"id":"https://openalex.org/F4320336521","display_name":"Vehicle Technologies Program","ror":"https://ror.org/00f93gc02"}],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":30,"referenced_works":["https://openalex.org/W1854827278","https://openalex.org/W1946860194","https://openalex.org/W1991730311","https://openalex.org/W1994508715","https://openalex.org/W2009632951","https://openalex.org/W2026001144","https://openalex.org/W2094580245","https://openalex.org/W2127194196","https://openalex.org/W2142745319","https://openalex.org/W2145636836","https://openalex.org/W2154358568","https://openalex.org/W2159519319","https://openalex.org/W2161747741","https://openalex.org/W2169509465","https://openalex.org/W2289922254","https://openalex.org/W2300083770","https://openalex.org/W2312439657","https://openalex.org/W2317163358","https://openalex.org/W2317541435","https://openalex.org/W2319146961","https://openalex.org/W2322657253","https://openalex.org/W2324493659","https://openalex.org/W2329754800","https://openalex.org/W2337948669","https://openalex.org/W2344355699","https://openalex.org/W2345247467","https://openalex.org/W2466722978","https://openalex.org/W2514470665","https://openalex.org/W2574644588","https://openalex.org/W2576928823"],"related_works":["https://openalex.org/W2316243321","https://openalex.org/W2009884537","https://openalex.org/W1996871648","https://openalex.org/W1968833643","https://openalex.org/W2170495660","https://openalex.org/W3012237635","https://openalex.org/W2914727333","https://openalex.org/W2378325450","https://openalex.org/W2599519345","https://openalex.org/W4396610267"],"abstract_inverted_index":{"Layered":[0],"lithium":[1,15],"transition":[2,57],"metal":[3,58],"oxides":[4],"(LTMO)":[5],"are":[6,187,202],"promising":[7],"candidate":[8],"cathode":[9,25,237],"materials":[10],"for":[11,20,95,234],"next-generation":[12],"high-energy":[13],"density":[14],"ion":[16],"battery.":[17],"The":[18],"challenge":[19],"using":[21],"this":[22,83],"category":[23],"of":[24,71,105,135,146,157,167,222,225,236],"is":[26,33,46,77],"the":[27,39,49,66,96,102,132,144,150,163,168,180,199,223,229],"capacity":[28],"and":[29,54,61,108,153,160,209,211,242],"voltage":[30],"fading,":[31],"which":[32],"believed":[34],"to":[35,189,191,216],"be":[36],"associated":[37],"with":[38,125,140,207,238],"layered":[40,74,121,169,218],"structure":[41,75],"disordering,":[42,142],"a":[43,73,111,154,244],"process":[44],"that":[45,174],"initiated":[47],"from":[48],"surface":[50],"or":[51],"solid-electrolyte":[52],"interface":[53],"facilitated":[55],"by":[56],"(TM)":[59],"reduction":[60],"oxygen":[62],"vacancy":[63],"formation.":[64],"However,":[65],"atomic":[67,86,100,126],"level":[68,127],"dynamic":[69],"mechanism":[70],"such":[72],"disordering":[76,166,194],"still":[78],"not":[79],"fully":[80],"clear.":[81],"In":[82,123],"work,":[84],"utilizing":[85],"resolution":[87],"electron":[88],"energy":[89],"loss":[90],"spectroscopy":[91],"(EELS),":[92],"we":[93,130],"map,":[94],"first":[97],"time":[98],"at":[99],"scale,":[101],"spatial":[103],"evolution":[104],"Ni,":[106,158],"Co":[107,117,210],"Mn":[109,115,161,200],"in":[110,149,184],"cycled":[112],"LiNi":[113],"1/3":[114,116,118],"O":[119],"2":[120],"cathode.":[122],"combination":[124],"structural":[128,240],"imaging,":[129],"discovered":[131],"direct":[133],"correlation":[134],"TM":[136,147,226],"ions":[137,148,201,227],"migration":[138,156],"behavior":[139,224],"lattice":[141,165,193],"featuring":[143],"residing":[145],"tetrahedral":[151],"site":[152],"sequential":[155],"Co,":[159],"upon":[162,195],"increased":[164],"structure.":[170,219],"This":[171],"work":[172],"highlights":[173],"Ni":[175,208],"ions,":[176],"though":[177],"acting":[178],"as":[179,205,214],"dominant":[181],"redox":[182],"species":[183],"many":[185],"LTMO,":[186],"labile":[188],"migrate":[190],"cause":[192],"battery":[196,230],"cycling,":[197],"while":[198],"more":[203],"stable":[204],"compared":[206],"can":[212],"act":[213],"pillar":[215],"stabilize":[217],"Direct":[220],"visualization":[221],"during":[228],"cycling":[231],"provides":[232],"insight":[233],"designing":[235],"high":[239],"stability":[241],"correspondingly":[243],"superior":[245],"performance.":[246]},"counts_by_year":[{"year":2026,"cited_by_count":5},{"year":2025,"cited_by_count":17},{"year":2024,"cited_by_count":12},{"year":2023,"cited_by_count":15},{"year":2022,"cited_by_count":16},{"year":2021,"cited_by_count":25},{"year":2020,"cited_by_count":32},{"year":2019,"cited_by_count":30},{"year":2018,"cited_by_count":17},{"year":2017,"cited_by_count":3}],"updated_date":"2026-10-12T09:40:04.860316","created_date":"2025-10-10T00:00:00"}
