{"id":"https://openalex.org/W2601651270","doi":"https://doi.org/10.1021/acs.estlett.7b00068","title":"Direct Visualization of Aggregate Morphology and Dynamics in a Model Soil Organic\u2013Mineral System","display_name":"Direct Visualization of Aggregate Morphology and Dynamics in a Model Soil Organic\u2013Mineral System","publication_year":2017,"publication_date":"2017-03-30","ids":{"openalex":"https://openalex.org/W2601651270","doi":"https://doi.org/10.1021/acs.estlett.7b00068","mag":"2601651270"},"language":"en","primary_location":{"id":"doi:10.1021/acs.estlett.7b00068","doi":"https://doi.org/10.1021/acs.estlett.7b00068","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.estlett.7b00068","pdf_url":null,"source":{"id":"https://openalex.org/S2764476807","display_name":"Environmental Science & Technology Letters","issn_l":"2328-8930","issn":["2328-8930"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-1","ki-jl-1","norway-1","poland-140","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Environmental Science &amp; Technology Letters","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5049059156","display_name":"Ryan Hufschmid","orcid":"https://orcid.org/0000-0003-4557-8060","observed_orcids":["https://orcid.org/0000-0003-4557-8060"]},"institutions":[{"id":"https://openalex.org/I201448701","display_name":"University of Washington","ror":"https://ror.org/00cvxb145","country_code":"US","type":"education","lineage":["https://openalex.org/I201448701"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Ryan Hufschmid","raw_affiliation_strings":["Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States"],"raw_orcid":"https://orcid.org/0000-0003-4557-8060","affiliations":[{"raw_affiliation_string":"Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States","institution_ids":["https://openalex.org/I201448701"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5049837267","display_name":"Christina J. Newcomb","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Christina J. Newcomb","raw_affiliation_strings":["Pacific Northwest National Laboratory, Richland, Washington 99352, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Pacific Northwest National Laboratory, Richland, Washington 99352, United States","institution_ids":["https://openalex.org/I142606810"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5087963967","display_name":"Jay W. Grate","orcid":"https://orcid.org/0000-0002-2163-8383","observed_orcids":["https://orcid.org/0000-0002-2163-8383"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Jay W. Grate","raw_affiliation_strings":["Pacific Northwest National Laboratory, Richland, Washington 99352, United States"],"raw_orcid":"https://orcid.org/0000-0002-2163-8383","affiliations":[{"raw_affiliation_string":"Pacific Northwest National Laboratory, Richland, Washington 99352, United States","institution_ids":["https://openalex.org/I142606810"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5110346792","display_name":"James J. De Yoreo","orcid":"https://orcid.org/0000-0002-9194-6699","observed_orcids":["https://orcid.org/0000-0002-9194-6699","https://orcid.org/0000-0002-9541-733X"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I201448701","display_name":"University of Washington","ror":"https://ror.org/00cvxb145","country_code":"US","type":"education","lineage":["https://openalex.org/I201448701"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"James J. De Yoreo","raw_affiliation_strings":["Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States","Pacific Northwest National Laboratory, Richland, Washington 99352, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States","institution_ids":["https://openalex.org/I201448701"]},{"raw_affiliation_string":"Pacific Northwest National Laboratory, Richland, Washington 99352, United States","institution_ids":["https://openalex.org/I142606810"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5077792493","display_name":"Nigel D. Browning","orcid":"https://orcid.org/0000-0003-0491-251X","observed_orcids":["https://orcid.org/0000-0003-0491-251X"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]},{"id":"https://openalex.org/I201448701","display_name":"University of Washington","ror":"https://ror.org/00cvxb145","country_code":"US","type":"education","lineage":["https://openalex.org/I201448701"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Nigel D. Browning","raw_affiliation_strings":["Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States","Pacific Northwest National Laboratory, Richland, Washington 99352, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department\rof Materials Science and Engineering, University of Washington, Seattle, Washington 98195-2120, United States","institution_ids":["https://openalex.org/I201448701"]},{"raw_affiliation_string":"Pacific Northwest National Laboratory, Richland, Washington 99352, United States","institution_ids":["https://openalex.org/I142606810"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5071457298","display_name":"Nikolla  P. Qafoku","orcid":"https://orcid.org/0000-0002-3258-5379","observed_orcids":["https://orcid.org/0000-0002-3258-5379"]},"institutions":[{"id":"https://openalex.org/I142606810","display_name":"Pacific Northwest National Laboratory","ror":"https://ror.org/05h992307","country_code":"US","type":"facility","lineage":["https://openalex.org/I1325736334","https://openalex.org/I1330989302","https://openalex.org/I142606810","https://openalex.org/I39565521"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Nikolla P. Qafoku","raw_affiliation_strings":["Pacific Northwest National Laboratory, Richland, Washington 99352, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Pacific Northwest National Laboratory, Richland, Washington 99352, United States","institution_ids":["https://openalex.org/I142606810"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5071457298"],"corresponding_institution_ids":["https://openalex.org/I142606810"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":1.3884,"has_fulltext":false,"cited_by_count":21,"citation_normalized_percentile":{"value":0.78657074,"is_in_top_1_percent":false,"is_in_top_10_percent":false},"cited_by_percentile_year":{"min":88,"max":98},"biblio":{"volume":"4","issue":"5","first_page":"186","last_page":"191"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T11877","display_name":"Iron oxide chemistry and applications","score":0.2134000062942505,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T11877","display_name":"Iron oxide chemistry and applications","score":0.2134000062942505,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11852","display_name":"Clay minerals and soil interactions","score":0.20100000500679016,"subfield":{"id":"https://openalex.org/subfields/1906","display_name":"Geochemistry and Petrology"},"field":{"id":"https://openalex.org/fields/19","display_name":"Earth and Planetary Sciences"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10004","display_name":"Soil Carbon and Nitrogen Dynamics","score":0.13770000636577606,"subfield":{"id":"https://openalex.org/subfields/1111","display_name":"Soil Science"},"field":{"id":"https://openalex.org/fields/11","display_name":"Agricultural and Biological Sciences"},"domain":{"id":"https://openalex.org/domains/1","display_name":"Life Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/organo-mineral-interactions","display_name":"organo-mineral interactions","score":0.9070000052452087},{"id":"https://openalex.org/keywords/soil-organic-matter","display_name":"soil organic matter","score":0.9259999990463257},{"id":"https://openalex.org/keywords/goethite-nanoparticles","display_name":"goethite nanoparticles","score":0.8410000205039978},{"id":"https://openalex.org/keywords/aggregate-morphology","display_name":"aggregate morphology","score":0.8169999718666077},{"id":"https://openalex.org/keywords/aggregation-dynamics","display_name":"aggregation dynamics","score":0.6819999814033508},{"id":"https://openalex.org/keywords/cryo-tem","display_name":"cryo-TEM","score":0.703000009059906},{"id":"https://openalex.org/keywords/in-situ-liquid-cell-tem","display_name":"in situ liquid cell TEM","score":0.9559999704360962}],"concepts":[{"id":"https://openalex.org/C48743137","wikidata":"https://www.wikidata.org/wiki/Q1783121","display_name":"Organic matter","level":2,"score":0.6673098802566528},{"id":"https://openalex.org/C77066764","wikidata":"https://www.wikidata.org/wiki/Q178674","display_name":"Nanometre","level":2,"score":0.5670321583747864},{"id":"https://openalex.org/C2776432453","wikidata":"https://www.wikidata.org/wiki/Q7946","display_name":"Mineral","level":2,"score":0.5591797828674316},{"id":"https://openalex.org/C146088050","wikidata":"https://www.wikidata.org/wiki/Q744818","display_name":"Transmission electron microscopy","level":2,"score":0.48022347688674927},{"id":"https://openalex.org/C45206210","wikidata":"https://www.wikidata.org/wiki/Q2415817","display_name":"Nanoscopic scale","level":2,"score":0.4798121452331543},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.44796374440193176},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.4250122308731079},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.4166065752506256},{"id":"https://openalex.org/C40212044","wikidata":"https://www.wikidata.org/wiki/Q1799034","display_name":"Clay minerals","level":2,"score":0.41344523429870605},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.41225725412368774},{"id":"https://openalex.org/C199289684","wikidata":"https://www.wikidata.org/wiki/Q83353","display_name":"Mineralogy","level":1,"score":0.37744206190109253},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.14101925492286682},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.07712447643280029},{"id":"https://openalex.org/C127413603","wikidata":"https://www.wikidata.org/wiki/Q11023","display_name":"Engineering","level":0,"score":0.0}],"mesh":[],"locations_count":1,"locations":[{"id":"doi:10.1021/acs.estlett.7b00068","doi":"https://doi.org/10.1021/acs.estlett.7b00068","is_oa":false,"landing_page_url":"https://doi.org/10.1021/acs.estlett.7b00068","pdf_url":null,"source":{"id":"https://openalex.org/S2764476807","display_name":"Environmental Science & Technology Letters","issn_l":"2328-8930","issn":["2328-8930"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-1","ki-jl-1","norway-1","poland-140","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Environmental Science &amp; Technology Letters","raw_type":"journal-article"}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[],"funders":[{"id":"https://openalex.org/F4320337547","display_name":"Laboratory Directed Research and Development","ror":"https://ror.org/01e41cf67"}],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":33,"referenced_works":["https://openalex.org/W72751723","https://openalex.org/W249666353","https://openalex.org/W1519631808","https://openalex.org/W1606015344","https://openalex.org/W1839550574","https://openalex.org/W1999783956","https://openalex.org/W2008962657","https://openalex.org/W2023417433","https://openalex.org/W2031004957","https://openalex.org/W2036122636","https://openalex.org/W2045622390","https://openalex.org/W2046722134","https://openalex.org/W2046940222","https://openalex.org/W2066459710","https://openalex.org/W2080461935","https://openalex.org/W2099049147","https://openalex.org/W2099540110","https://openalex.org/W2110406941","https://openalex.org/W2117348990","https://openalex.org/W2132484323","https://openalex.org/W2139405554","https://openalex.org/W2155659696","https://openalex.org/W2161839642","https://openalex.org/W2276485526","https://openalex.org/W2321774739","https://openalex.org/W2325382080","https://openalex.org/W2326211450","https://openalex.org/W2344180436","https://openalex.org/W2344411363","https://openalex.org/W2344442458","https://openalex.org/W2438516979","https://openalex.org/W2462218518","https://openalex.org/W2514518356"],"related_works":["https://openalex.org/W2761675005","https://openalex.org/W3042647629","https://openalex.org/W2531154650","https://openalex.org/W2897673401","https://openalex.org/W2509557551","https://openalex.org/W3143682559","https://openalex.org/W4415509771","https://openalex.org/W2116115127","https://openalex.org/W3042580107","https://openalex.org/W2750437866"],"abstract_inverted_index":{"Interactions":[0],"between":[1],"mineral":[2,164],"surfaces":[3],"and":[4,11,17,36,54,65,82,101,130,168,176,181],"organic":[5,26,127,142],"matter":[6,27],"are":[7,73],"ubiquitous":[8],"in":[9,92,102,115,145],"soils":[10],"the":[12,40,116,138,141,156],"environment.":[13],"Through":[14],"both":[15],"physical":[16],"chemical":[18],"mechanisms,":[19],"organic\u2013mineral":[20,43,80,180],"assemblages":[21,165],"prevent":[22],"decomposition":[23],"of":[24,34,119,124,137,140,155,163],"soil":[25],"by":[28],"limiting":[29],"accessibility":[30],"or":[31],"reducing":[32],"efficacy":[33],"enzymes":[35],"microbes.":[37],"To":[38],"understand":[39],"mechanisms":[41],"underlying":[42],"interactions,":[44],"researchers":[45,67],"have":[46],"begun":[47],"to":[48,68,160],"interrogate":[49],"these":[50],"systems":[51],"at":[52],"micro-":[53],"nanometer":[55,70],"length":[56,71],"scales.":[57],"Current":[58],"techniques":[59,86],"that":[60,87],"maintain":[61],"a":[62,78,112,125,131,152],"hydrated":[63],"state":[64],"allow":[66],"characterize":[69],"scales":[72],"limited.":[74],"Here":[75],"we":[76],"chose":[77],"model":[79,126],"system":[81],"performed":[83],"complementary":[84],"imaging":[85],"allowed":[88],"direct":[89],"nanoscale":[90],"observations":[91],"environmentally":[93],"relevant":[94],"conditions:":[95],"cryogenic":[96],"transmission":[97,106],"electron":[98,107],"microscopy":[99,108],"(cryo-TEM)":[100],"situ":[103,146],"liquid":[104,147],"cell":[105,148],"(TEM).":[109],"We":[110],"observed":[111],"3-fold":[113],"increase":[114],"aggregate":[117],"size":[118],"goethite":[120],"nanoparticles":[121],"upon":[122],"addition":[123,139],"phosphate":[128],"ligand":[129],"preference":[132],"for":[133,179],"side-to-side":[134],"interactions":[135,157],"independent":[136],"ligand.":[143],"Additionally,":[144],"TEM":[149],"experiments":[150],"provided":[151],"dynamic":[153],"view":[154],"allowing":[158],"us":[159],"report":[161],"velocities":[162],"during":[166],"aggregation":[167],"disaggregation,":[169],"which":[170],"could":[171],"potentially":[172],"provide":[173],"binding":[174],"energetics":[175],"kinetic":[177],"parameters":[178],"mineral\u2013mineral":[182],"systems.":[183]},"counts_by_year":[{"year":2025,"cited_by_count":3},{"year":2024,"cited_by_count":1},{"year":2022,"cited_by_count":3},{"year":2021,"cited_by_count":1},{"year":2020,"cited_by_count":3},{"year":2019,"cited_by_count":6},{"year":2018,"cited_by_count":2},{"year":2017,"cited_by_count":2}],"updated_date":"2026-09-25T08:18:29.962427","created_date":"2017-04-07T00:00:00"}
