{"id":"https://openalex.org/W2332366705","doi":"https://doi.org/10.1021/ja300270w","title":"Activation of Surface Hydroxyl Groups by Modification of H-Terminated Si(111) Surfaces","display_name":"Activation of Surface Hydroxyl Groups by Modification of H-Terminated Si(111) Surfaces","publication_year":2012,"publication_date":"2012-05-03","ids":{"openalex":"https://openalex.org/W2332366705","doi":"https://doi.org/10.1021/ja300270w","mag":"2332366705","pmid":"https://pubmed.ncbi.nlm.nih.gov/22554133"},"language":"en","primary_location":{"id":"doi:10.1021/ja300270w","doi":"https://doi.org/10.1021/ja300270w","is_oa":false,"landing_page_url":"https://doi.org/10.1021/ja300270w","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5017366257","display_name":"Peter Thissen","orcid":"https://orcid.org/0000-0001-7072-4109","observed_orcids":["https://orcid.org/0000-0001-7072-4109"]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Peter Thissen","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5109290183","display_name":"Tatiana Peixoto","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Tatiana Peixoto","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5061779151","display_name":"Roberto Carlos Longo","orcid":"https://orcid.org/0000-0003-4353-841X","observed_orcids":["https://orcid.org/0000-0003-4353-841X"]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Roberto C. Longo","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5109931466","display_name":"Weina Peng","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Weina Peng","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5071311557","display_name":"W. G. Schmidt","orcid":"https://orcid.org/0000-0002-2717-5076","observed_orcids":["https://orcid.org/0000-0002-2717-5076"]},"institutions":[{"id":"https://openalex.org/I206945453","display_name":"Paderborn University","ror":"https://ror.org/058kzsd48","country_code":"DE","type":"education","lineage":["https://openalex.org/I206945453"]}],"countries":["DE"],"is_corresponding":false,"raw_author_name":"Wolf Gero Schmidt","raw_affiliation_strings":["Lehrstuhl f\u00fcr Theoretische Physik, Universit\u00e4t Paderborn, 33098 Paderborn, Germany"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Lehrstuhl f\u00fcr Theoretische Physik, Universit\u00e4t Paderborn, 33098 Paderborn, Germany","institution_ids":["https://openalex.org/I206945453"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5065656919","display_name":"K. Cho","orcid":"https://orcid.org/0000-0003-2698-7774","observed_orcids":["https://orcid.org/0000-0003-2698-7774"]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Kyeongjae Cho","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5051239060","display_name":"Yves Jean Chabal","orcid":"https://orcid.org/0000-0002-6435-0347","observed_orcids":["https://orcid.org/0000-0002-6435-0347"]},"institutions":[{"id":"https://openalex.org/I162577319","display_name":"The University of Texas at Dallas","ror":"https://ror.org/049emcs32","country_code":"US","type":"education","lineage":["https://openalex.org/I162577319"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Yves J. Chabal","raw_affiliation_strings":["Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Department of Materials Science and Engineering, University of Texas at Dallas, 800 West Campbell Road, Richardson, Texas 75080, United States","institution_ids":["https://openalex.org/I162577319"]}]}],"institutions":[],"countries_distinct_count":2,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5017366257"],"corresponding_institution_ids":["https://openalex.org/I162577319"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":5.4188,"has_fulltext":false,"cited_by_count":79,"citation_normalized_percentile":{"value":0.9705635,"is_in_top_1_percent":false,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":93,"max":99},"biblio":{"volume":"134","issue":"21","first_page":"8869","last_page":"8874"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10859","display_name":"Polymer Surface Interaction Studies","score":0.44020000100135803,"subfield":{"id":"https://openalex.org/subfields/2508","display_name":"Surfaces, Coatings and Films"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10859","display_name":"Polymer Surface Interaction Studies","score":0.44020000100135803,"subfield":{"id":"https://openalex.org/subfields/2508","display_name":"Surfaces, Coatings and Films"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T12285","display_name":"Surface Chemistry and Catalysis","score":0.1859000027179718,"subfield":{"id":"https://openalex.org/subfields/1606","display_name":"Physical and Theoretical Chemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10472","display_name":"Semiconductor materials and devices","score":0.08179999887943268,"subfield":{"id":"https://openalex.org/subfields/2208","display_name":"Electrical and Electronic Engineering"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/si-111-surface","display_name":"Si(111) surface","score":0.8169999718666077},{"id":"https://openalex.org/keywords/hydroxyl-groups","display_name":"hydroxyl groups","score":0.7269999980926514},{"id":"https://openalex.org/keywords/surface-functionalization","display_name":"surface functionalization","score":0.7419999837875366},{"id":"https://openalex.org/keywords/phosphonic-acid","display_name":"phosphonic acid","score":0.5410000085830688},{"id":"https://openalex.org/keywords/chemical-grafting","display_name":"chemical grafting","score":0.578000009059906},{"id":"https://openalex.org/keywords/aqueous-stability","display_name":"aqueous stability","score":0.8140000104904175},{"id":"https://openalex.org/keywords/siox","display_name":"silicon oxide","score":0.5239999890327454},{"id":"https://openalex.org/keywords/semiconductor-surface-chemistry","display_name":"semiconductor surface chemistry","score":0.5929999947547913}],"concepts":[{"id":"https://openalex.org/C115537861","wikidata":"https://www.wikidata.org/wiki/Q7645993","display_name":"Surface modification","level":2,"score":0.7624138593673706},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.7539359331130981},{"id":"https://openalex.org/C544956773","wikidata":"https://www.wikidata.org/wiki/Q670","display_name":"Silicon","level":2,"score":0.7348344326019287},{"id":"https://openalex.org/C2779851234","wikidata":"https://www.wikidata.org/wiki/Q50690","display_name":"Oxide","level":2,"score":0.7097086310386658},{"id":"https://openalex.org/C161790260","wikidata":"https://www.wikidata.org/wiki/Q82264","display_name":"Catalysis","level":2,"score":0.5641570687294006},{"id":"https://openalex.org/C542589376","wikidata":"https://www.wikidata.org/wiki/Q192127","display_name":"Photovoltaics","level":3,"score":0.5411388874053955},{"id":"https://openalex.org/C32909587","wikidata":"https://www.wikidata.org/wiki/Q11369","display_name":"Molecule","level":2,"score":0.5304358005523682},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.5213478803634644},{"id":"https://openalex.org/C184651966","wikidata":"https://www.wikidata.org/wiki/Q906356","display_name":"Aqueous solution","level":2,"score":0.48663386702537537},{"id":"https://openalex.org/C2779105228","wikidata":"https://www.wikidata.org/wiki/Q2286029","display_name":"Silicon oxide","level":4,"score":0.4689366817474365},{"id":"https://openalex.org/C2777855556","wikidata":"https://www.wikidata.org/wiki/Q4339544","display_name":"Annealing (glass)","level":2,"score":0.4589584469795227},{"id":"https://openalex.org/C177801218","wikidata":"https://www.wikidata.org/wiki/Q36534","display_name":"Chemical reaction","level":2,"score":0.4223945736885071},{"id":"https://openalex.org/C2776910235","wikidata":"https://www.wikidata.org/wiki/Q18574","display_name":"Reactivity (psychology)","level":3,"score":0.4124774634838104},{"id":"https://openalex.org/C42360764","wikidata":"https://www.wikidata.org/wiki/Q83588","display_name":"Chemical engineering","level":1,"score":0.3696867823600769},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.1834089756011963},{"id":"https://openalex.org/C41291067","wikidata":"https://www.wikidata.org/wiki/Q1897785","display_name":"Photovoltaic system","level":2,"score":0.1668456792831421},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.16357430815696716},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.09722021222114563},{"id":"https://openalex.org/C18903297","wikidata":"https://www.wikidata.org/wiki/Q7150","display_name":"Ecology","level":1,"score":0.0},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.0},{"id":"https://openalex.org/C71924100","wikidata":"https://www.wikidata.org/wiki/Q11190","display_name":"Medicine","level":0,"score":0.0},{"id":"https://openalex.org/C2777431650","wikidata":"https://www.wikidata.org/wiki/Q413828","display_name":"Silicon nitride","level":3,"score":0.0},{"id":"https://openalex.org/C142724271","wikidata":"https://www.wikidata.org/wiki/Q7208","display_name":"Pathology","level":1,"score":0.0},{"id":"https://openalex.org/C127413603","wikidata":"https://www.wikidata.org/wiki/Q11023","display_name":"Engineering","level":0,"score":0.0},{"id":"https://openalex.org/C204787440","wikidata":"https://www.wikidata.org/wiki/Q188504","display_name":"Alternative medicine","level":2,"score":0.0},{"id":"https://openalex.org/C86803240","wikidata":"https://www.wikidata.org/wiki/Q420","display_name":"Biology","level":0,"score":0.0}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/ja300270w","doi":"https://doi.org/10.1021/ja300270w","is_oa":false,"landing_page_url":"https://doi.org/10.1021/ja300270w","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},{"id":"pmid:22554133","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/22554133","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[],"funders":[],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":38,"referenced_works":["https://openalex.org/W1597773817","https://openalex.org/W1965242230","https://openalex.org/W1965463083","https://openalex.org/W1978093886","https://openalex.org/W1979544533","https://openalex.org/W1979926766","https://openalex.org/W1983279622","https://openalex.org/W1992742673","https://openalex.org/W2006721956","https://openalex.org/W2007395042","https://openalex.org/W2009036275","https://openalex.org/W2011488302","https://openalex.org/W2019492728","https://openalex.org/W2019738895","https://openalex.org/W2034137747","https://openalex.org/W2034760552","https://openalex.org/W2039377607","https://openalex.org/W2040794475","https://openalex.org/W2044707101","https://openalex.org/W2050768366","https://openalex.org/W2065055949","https://openalex.org/W2065908010","https://openalex.org/W2067539251","https://openalex.org/W2072463909","https://openalex.org/W2072677085","https://openalex.org/W2076327902","https://openalex.org/W2078460749","https://openalex.org/W2082026649","https://openalex.org/W2083222334","https://openalex.org/W2092685342","https://openalex.org/W2093348224","https://openalex.org/W2097900321","https://openalex.org/W2144360348","https://openalex.org/W2146837441","https://openalex.org/W2166806803","https://openalex.org/W2316293245","https://openalex.org/W2922713140","https://openalex.org/W4388166534"],"related_works":["https://openalex.org/W1998011237","https://openalex.org/W2330949260","https://openalex.org/W2606397815","https://openalex.org/W4309139074","https://openalex.org/W2952582745","https://openalex.org/W7119084140","https://openalex.org/W3135893805","https://openalex.org/W2065055949","https://openalex.org/W1994696938","https://openalex.org/W1970578346"],"abstract_inverted_index":{"Chemical":[0],"functionalization":[1],"of":[2,59,100,132],"semiconductor":[3],"surfaces,":[4],"particularly":[5],"silicon":[6,81,87,127,143],"oxide,":[7],"has":[8],"enabled":[9],"many":[10],"technologically":[11,40],"important":[12,41],"applications":[13],"(e.g.,":[14],"sensing,":[15],"photovoltaics,":[16],"and":[17,111,135,148],"catalysis).":[18],"For":[19],"such":[20,43],"processes,":[21,42],"hydroxyl":[22,77],"groups":[23,78],"terminating":[24],"the":[25,29,60],"oxide":[26],"surface":[27,45,67,136],"constitute":[28],"primary":[30],"reaction":[31],"sites.":[32],"However,":[33],"their":[34],"reactivity":[35],"is":[36,105],"often":[37],"poor,":[38],"hindering":[39],"as":[44],"phosphonation":[46],"requiring":[47],"a":[48,64,69,96],"lengthy":[49],"postprocessing":[50],"annealing":[51],"step":[52],"at":[53,108],"140":[54],"\u00b0C":[55],"with":[56],"poor":[57],"control":[58],"bonding":[61],"geometry.":[62],"Using":[63],"novel":[65],"oxide-free":[66,80],"featuring":[68],"well-defined":[70],"nanopatterned":[71],"OH":[72],"coverage,":[73],"we":[74,93],"demonstrate":[75],"that":[76,95],"on":[79,86,126],"are":[82],"more":[83],"reactive":[84],"than":[85],"oxide.":[88],"On":[89],"this":[90],"model":[91],"surface,":[92],"show":[94],"perfectly":[97],"ordered":[98],"layer":[99],"monodentate":[101],"phosphonic":[102],"acid":[103],"molecules":[104],"chemically":[106],"grafted":[107,125],"room":[109],"temperature,":[110],"explain":[112],"why":[113],"it":[114],"remains":[115],"completely":[116],"stable":[117],"in":[118,121],"aqueous":[119],"environments,":[120],"contrast":[122],"to":[123,141],"phosphonates":[124],"oxides.":[128],"This":[129],"fundamental":[130],"understanding":[131],"chemical":[133],"activity":[134],"stability":[137],"suggests":[138],"new":[139],"directions":[140],"functionalize":[142],"for":[144],"sensors,":[145],"photovoltaic":[146],"devices,":[147],"nanoelectronics.":[149]},"counts_by_year":[{"year":2026,"cited_by_count":2},{"year":2025,"cited_by_count":3},{"year":2024,"cited_by_count":2},{"year":2023,"cited_by_count":5},{"year":2022,"cited_by_count":4},{"year":2021,"cited_by_count":3},{"year":2020,"cited_by_count":8},{"year":2019,"cited_by_count":6},{"year":2018,"cited_by_count":7},{"year":2017,"cited_by_count":4},{"year":2016,"cited_by_count":6},{"year":2015,"cited_by_count":8},{"year":2014,"cited_by_count":4},{"year":2013,"cited_by_count":13},{"year":2012,"cited_by_count":3}],"updated_date":"2026-11-07T11:25:07.637180","created_date":"2016-06-24T00:00:00"}
