{"id":"https://openalex.org/W2325010659","doi":"https://doi.org/10.1021/ja3062584","title":"Photodriven Charge Separation Dynamics in CdSe/ZnS Core/Shell Quantum Dot/Cobaloxime Hybrid for Efficient Hydrogen Production","display_name":"Photodriven Charge Separation Dynamics in CdSe/ZnS Core/Shell Quantum Dot/Cobaloxime Hybrid for Efficient Hydrogen Production","publication_year":2012,"publication_date":"2012-09-18","ids":{"openalex":"https://openalex.org/W2325010659","doi":"https://doi.org/10.1021/ja3062584","mag":"2325010659","pmid":"https://pubmed.ncbi.nlm.nih.gov/22989083"},"language":"en","primary_location":{"id":"doi:10.1021/ja3062584","doi":"https://doi.org/10.1021/ja3062584","is_oa":false,"landing_page_url":"https://doi.org/10.1021/ja3062584","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},"volume":null,"type":"article","indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5038255119","display_name":"Jier Huang","orcid":"https://orcid.org/0000-0002-2885-5786","observed_orcids":["https://orcid.org/0000-0002-2885-5786"]},"institutions":[{"id":"https://openalex.org/I1282105669","display_name":"Argonne National Laboratory","ror":"https://ror.org/05gvnxz63","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Jier Huang","raw_affiliation_strings":["Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States","institution_ids":["https://openalex.org/I1282105669"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5063841332","display_name":"Karen L. Mulfort","orcid":"https://orcid.org/0000-0002-3132-1179","observed_orcids":["https://orcid.org/0000-0002-3132-1179"]},"institutions":[{"id":"https://openalex.org/I1282105669","display_name":"Argonne National Laboratory","ror":"https://ror.org/05gvnxz63","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Karen L. Mulfort","raw_affiliation_strings":["Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States","institution_ids":["https://openalex.org/I1282105669"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5043498580","display_name":"Pingwu Du","orcid":"https://orcid.org/0000-0002-2715-0979","observed_orcids":["https://orcid.org/0000-0002-2715-0979"]},"institutions":[{"id":"https://openalex.org/I1282105669","display_name":"Argonne National Laboratory","ror":"https://ror.org/05gvnxz63","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166"]}],"countries":["US"],"is_corresponding":false,"raw_author_name":"Pingwu Du","raw_affiliation_strings":["Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States","institution_ids":["https://openalex.org/I1282105669"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5014620636","display_name":"Lin X. Chen","orcid":"https://orcid.org/0000-0002-8450-6687","observed_orcids":["https://orcid.org/0000-0002-8450-6687"]},"institutions":[{"id":"https://openalex.org/I111979921","display_name":"Northwestern University","ror":"https://ror.org/000e0be47","country_code":"US","type":"education","lineage":["https://openalex.org/I111979921"]},{"id":"https://openalex.org/I1282105669","display_name":"Argonne National Laboratory","ror":"https://ror.org/05gvnxz63","country_code":"US","type":"facility","lineage":["https://openalex.org/I1282105669","https://openalex.org/I1330989302","https://openalex.org/I39565521","https://openalex.org/I40347166"]}],"countries":["US"],"is_corresponding":true,"raw_author_name":"Lin X. Chen","raw_affiliation_strings":["Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States","Department of Chemistry, Northwestern University, Evanston, Illinois 60208,\rUnited States"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"Chemical Sciences\rand Engineering\rDivision, Argonne National Laboratory,\rArgonne, Illinois 60439, United States","institution_ids":["https://openalex.org/I1282105669"]},{"raw_affiliation_string":"Department of Chemistry, Northwestern University, Evanston, Illinois 60208,\rUnited States","institution_ids":["https://openalex.org/I111979921"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":2,"corresponding_author_ids":["https://openalex.org/A5014620636","https://openalex.org/A5063841332"],"corresponding_institution_ids":["https://openalex.org/I111979921","https://openalex.org/I1282105669"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":8.0942,"has_fulltext":false,"cited_by_count":272,"citation_normalized_percentile":{"value":0.98073286,"is_in_top_1_percent":false,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":94,"max":100},"biblio":{"volume":"134","issue":"40","first_page":"16472","last_page":"16475"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.7681000232696533,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T10078","display_name":"Advanced Photocatalysis Techniques","score":0.7681000232696533,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11626","display_name":"Metalloenzymes and iron-sulfur proteins","score":0.1770000010728836,"subfield":{"id":"https://openalex.org/subfields/2105","display_name":"Renewable Energy, Sustainability and the Environment"},"field":{"id":"https://openalex.org/fields/21","display_name":"Energy"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10321","display_name":"Quantum Dots Synthesis And Properties","score":0.019500000402331352,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/cdse-zns-quantum-dots","display_name":"CdSe/ZnS quantum dots","score":0.968999981880188},{"id":"https://openalex.org/keywords/cobaloximes","display_name":"cobaloximes","score":0.878000020980835},{"id":"https://openalex.org/keywords/photocatalytic-hydrogen-production","display_name":"photocatalytic hydrogen evolution","score":0.8090000152587891},{"id":"https://openalex.org/keywords/charge-separation","display_name":"charge separation","score":0.6740000247955322},{"id":"https://openalex.org/keywords/electron-transfer-dynamics","display_name":"electron transfer dynamics","score":0.8169999718666077},{"id":"https://openalex.org/keywords/charge-recombination","display_name":"charge recombination","score":0.9810000061988831},{"id":"https://openalex.org/keywords/triethanolamine","display_name":"triethanolamine","score":0.6959999799728394},{"id":"https://openalex.org/keywords/sacrificial-electron-donor","display_name":"sacrificial electron donor","score":0.7590000033378601},{"id":"https://openalex.org/keywords/artificial-photosynthesis","display_name":"artificial photosynthesis","score":0.7519999742507935}],"concepts":[{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.9219721555709839},{"id":"https://openalex.org/C124657808","wikidata":"https://www.wikidata.org/wiki/Q1133068","display_name":"Quantum dot","level":2,"score":0.8362711668014526},{"id":"https://openalex.org/C202189072","wikidata":"https://www.wikidata.org/wiki/Q1929999","display_name":"Hydrogen production","level":3,"score":0.6541459560394287},{"id":"https://openalex.org/C188082385","wikidata":"https://www.wikidata.org/wiki/Q73792","display_name":"Charge (physics)","level":2,"score":0.6021863222122192},{"id":"https://openalex.org/C2164484","wikidata":"https://www.wikidata.org/wiki/Q5170150","display_name":"Core (optical fiber)","level":2,"score":0.5395985841751099},{"id":"https://openalex.org/C512968161","wikidata":"https://www.wikidata.org/wiki/Q556","display_name":"Hydrogen","level":2,"score":0.5371286273002625},{"id":"https://openalex.org/C2778348673","wikidata":"https://www.wikidata.org/wiki/Q739302","display_name":"Production (economics)","level":2,"score":0.472613126039505},{"id":"https://openalex.org/C159467904","wikidata":"https://www.wikidata.org/wiki/Q2001702","display_name":"Chemical physics","level":1,"score":0.4720652401447296},{"id":"https://openalex.org/C171250308","wikidata":"https://www.wikidata.org/wiki/Q11468","display_name":"Nanotechnology","level":1,"score":0.4290480613708496},{"id":"https://openalex.org/C2781052500","wikidata":"https://www.wikidata.org/wiki/Q2230313","display_name":"Shell (structure)","level":2,"score":0.4154411554336548},{"id":"https://openalex.org/C145912823","wikidata":"https://www.wikidata.org/wiki/Q113558","display_name":"Dynamics (music)","level":2,"score":0.4110977053642273},{"id":"https://openalex.org/C62520636","wikidata":"https://www.wikidata.org/wiki/Q944","display_name":"Quantum mechanics","level":1,"score":0.11128243803977966},{"id":"https://openalex.org/C121332964","wikidata":"https://www.wikidata.org/wiki/Q413","display_name":"Physics","level":0,"score":0.07735848426818848},{"id":"https://openalex.org/C120665830","wikidata":"https://www.wikidata.org/wiki/Q14620","display_name":"Optics","level":1,"score":0.049779146909713745},{"id":"https://openalex.org/C162324750","wikidata":"https://www.wikidata.org/wiki/Q8134","display_name":"Economics","level":0,"score":0.0},{"id":"https://openalex.org/C159985019","wikidata":"https://www.wikidata.org/wiki/Q181790","display_name":"Composite material","level":1,"score":0.0},{"id":"https://openalex.org/C192562407","wikidata":"https://www.wikidata.org/wiki/Q228736","display_name":"Materials science","level":0,"score":0.0},{"id":"https://openalex.org/C139719470","wikidata":"https://www.wikidata.org/wiki/Q39680","display_name":"Macroeconomics","level":1,"score":0.0},{"id":"https://openalex.org/C178790620","wikidata":"https://www.wikidata.org/wiki/Q11351","display_name":"Organic chemistry","level":1,"score":0.0},{"id":"https://openalex.org/C24890656","wikidata":"https://www.wikidata.org/wiki/Q82811","display_name":"Acoustics","level":1,"score":0.0}],"mesh":[],"locations_count":2,"locations":[{"id":"doi:10.1021/ja3062584","doi":"https://doi.org/10.1021/ja3062584","is_oa":false,"landing_page_url":"https://doi.org/10.1021/ja3062584","pdf_url":null,"source":{"id":"https://openalex.org/S111155417","display_name":"Journal of the American Chemical Society","issn_l":"0002-7863","issn":["0002-7863","1520-5126","1943-2984"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["cwts-core","dongbi-a","jufo-3","ki-jl-3","medline","norway-2","poland-200","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"journal-article"},{"id":"pmid:22989083","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/22989083","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Journal of the American Chemical Society","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[{"display_name":"Affordable and clean energy","score":0.75,"id":"https://metadata.un.org/sdg/7"}],"study_designs":[],"awards":[],"funders":[],"has_content":{"grobid_xml":false,"pdf":false},"content_urls":null,"referenced_works_count":36,"referenced_works":["https://openalex.org/W221088158","https://openalex.org/W1560627658","https://openalex.org/W1896289247","https://openalex.org/W1986829915","https://openalex.org/W1990770447","https://openalex.org/W1990986472","https://openalex.org/W1996533547","https://openalex.org/W2002267607","https://openalex.org/W2004567430","https://openalex.org/W2010436521","https://openalex.org/W2011399034","https://openalex.org/W2012496309","https://openalex.org/W2017121843","https://openalex.org/W2030448178","https://openalex.org/W2034958507","https://openalex.org/W2036095406","https://openalex.org/W2037187406","https://openalex.org/W2038980827","https://openalex.org/W2044543075","https://openalex.org/W2052989605","https://openalex.org/W2055264889","https://openalex.org/W2065706045","https://openalex.org/W2065843750","https://openalex.org/W2075539838","https://openalex.org/W2077472794","https://openalex.org/W2078833116","https://openalex.org/W2084429162","https://openalex.org/W2085666906","https://openalex.org/W2099297906","https://openalex.org/W2102128050","https://openalex.org/W2112953889","https://openalex.org/W2151706384","https://openalex.org/W2151853961","https://openalex.org/W2316616988","https://openalex.org/W2326153055","https://openalex.org/W2330532819"],"related_works":["https://openalex.org/W2148189623","https://openalex.org/W2988280305","https://openalex.org/W1990770447","https://openalex.org/W4412753387","https://openalex.org/W2919051270","https://openalex.org/W2908978643","https://openalex.org/W2809082834","https://openalex.org/W4412478877","https://openalex.org/W2269050384","https://openalex.org/W4232367193"],"abstract_inverted_index":{"Photodriven":[0],"charge-transfer":[1],"dynamics":[2],"and":[3,19,108],"catalytic":[4,106],"properties":[5],"have":[6,112],"been":[7],"investigated":[8],"for":[9,120],"a":[10,49,56,88],"hybrid":[11,73],"system":[12],"containing":[13],"CdSe/ZnS":[14],"core/shell":[15],"quantum":[16],"dots":[17],"(QDs)":[18],"surface-bound":[20],"molecular":[21],"cobaloxime":[22],"catalysts.":[23],"The":[24],"electron":[25,90],"transfer":[26],"from":[27,123],"light-excited":[28],"QDs":[29],"to":[30],"cobaloxime,":[31],"revealed":[32],"by":[33,70],"optical":[34],"transient":[35],"absorption":[36],"spectroscopy,":[37],"takes":[38],"place":[39],"with":[40,55,75,103],"an":[41],"average":[42],"time":[43,57],"constant":[44,58],"of":[45,59,78],"105":[46],"ps,":[47],"followed":[48],"much":[50],"slower":[51],"charge":[52],"recombination":[53],"process":[54],"\u226b3":[60],"ns.":[61],"More":[62],"interestingly,":[63],"we":[64],"also":[65],"observed":[66],"photocatalytic":[67],"hydrogen":[68],"generation":[69,122],"this":[71],"QD/cobaloxime":[72,96],"system,":[74],">10,000":[76],"turnovers":[77],"H(2)":[79],"per":[80],"QD":[81],"in":[82,99,115],"10":[83],"h,":[84],"using":[85],"triethanolamine":[86],"as":[87],"sacrificial":[89],"donor.":[91],"These":[92],"results":[93],"suggest":[94],"that":[95],"hybrids":[97],"succeed":[98],"coupling":[100],"single-photon":[101],"events":[102],"multielectron":[104],"redox":[105],"reactions,":[107],"such":[109],"systems":[110],"could":[111],"potential":[113],"applications":[114],"long-lived":[116],"artificial":[117],"photosynthetic":[118],"devices":[119],"fuel":[121],"sunlight.":[124]},"counts_by_year":[{"year":2026,"cited_by_count":4},{"year":2025,"cited_by_count":9},{"year":2024,"cited_by_count":10},{"year":2023,"cited_by_count":9},{"year":2022,"cited_by_count":12},{"year":2021,"cited_by_count":25},{"year":2020,"cited_by_count":20},{"year":2019,"cited_by_count":23},{"year":2018,"cited_by_count":24},{"year":2017,"cited_by_count":23},{"year":2016,"cited_by_count":43},{"year":2015,"cited_by_count":21},{"year":2014,"cited_by_count":30},{"year":2013,"cited_by_count":17},{"year":2012,"cited_by_count":2}],"updated_date":"2026-11-04T10:54:05.112534","created_date":"2016-06-24T00:00:00"}
