{"id":"https://openalex.org/W1985648548","doi":"https://doi.org/10.1021/es070832y","title":"Radiation Induced Spent Nuclear Fuel Dissolution under Deep Repository Conditions","display_name":"Radiation Induced Spent Nuclear Fuel Dissolution under Deep Repository Conditions","publication_year":2007,"publication_date":"2007-09-07","ids":{"openalex":"https://openalex.org/W1985648548","doi":"https://doi.org/10.1021/es070832y","mag":"1985648548","pmid":"https://pubmed.ncbi.nlm.nih.gov/17993152"},"language":"en","primary_location":{"id":"doi:10.1021/es070832y","doi":"https://doi.org/10.1021/es070832y","is_oa":false,"landing_page_url":"https://doi.org/10.1021/es070832y","pdf_url":null,"source":{"id":"https://openalex.org/S13479253","display_name":"Environmental Science & Technology","issn_l":"0013-936X","issn":["0013-936X","1520-5851"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["anvur-class-a","anvur-scientific","cwts-core","dongbi-a","fnege-4","jufo-2","ki-jl-2","medline","norway-2","poland-140","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Environmental Science & Technology","raw_type":"journal-article"},"volume":null,"type":"article","is_traditional":true,"indexed_in":["crossref","pubmed"],"open_access":{"is_oa":false,"oa_status":"closed","oa_url":null,"any_repository_has_fulltext":false},"authorships":[{"author_position":"first","author":{"id":"https://openalex.org/A5114259957","display_name":"Mats J\u00f6nsson","orcid":"https://orcid.org/0000-0003-0663-0751","observed_orcids":["https://orcid.org/0000-0003-0663-0751"]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Mats Jonsson","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]},{"author_position":"middle","author":{"id":null,"display_name":"Fredrik Nielsen","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Fredrik Nielsen","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5010608481","display_name":"Olivia Roth","orcid":"https://orcid.org/0000-0003-0582-1011","observed_orcids":["https://orcid.org/0000-0003-0582-1011","https://orcid.org/0009-0006-0131-2956"]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Olivia Roth","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5034454762","display_name":"Ella Ekeroth","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Ella Ekeroth","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]},{"author_position":"middle","author":{"id":"https://openalex.org/A5074465343","display_name":"Sara Nilsson","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Sara Nilsson","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]},{"author_position":"last","author":{"id":"https://openalex.org/A5023190416","display_name":"Mohammad Mohsin Hossain","orcid":null,"observed_orcids":[]},"institutions":[{"id":"https://openalex.org/I86987016","display_name":"KTH Royal Institute of Technology","ror":"https://ror.org/026vcq606","country_code":"SE","type":"education","lineage":["https://openalex.org/I86987016"]}],"countries":["SE"],"is_corresponding":false,"raw_author_name":"Mohammad Mohsin Hossain","raw_affiliation_strings":["KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden"],"raw_orcid":null,"affiliations":[{"raw_affiliation_string":"KTH Chemical Science and Engineering, Nuclear Chemistry, Royal Institute of Technology, SE \u2212 100 44 Stockholm, Sweden","institution_ids":["https://openalex.org/I86987016"]}]}],"institutions":[],"countries_distinct_count":1,"institutions_distinct_count":1,"corresponding_author_ids":[],"corresponding_institution_ids":["https://openalex.org/I86987016"],"apc_list":{"value":4500,"currency":"USD","value_usd":4500},"apc_paid":null,"fwci":22.0723,"has_fulltext":false,"cited_by_count":88,"citation_normalized_percentile":{"value":0.99403697,"is_in_top_1_percent":true,"is_in_top_10_percent":true},"cited_by_percentile_year":{"min":93,"max":99},"biblio":{"volume":"41","issue":"20","first_page":"7087","last_page":"7093"},"is_retracted":false,"is_paratext":false,"is_xpac":false,"primary_topic":{"id":"https://openalex.org/T13923","display_name":"Nuclear and radioactivity studies","score":0.5717999935150146,"subfield":{"id":"https://openalex.org/subfields/2213","display_name":"Safety, Risk, Reliability and Quality"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},"topics":[{"id":"https://openalex.org/T13923","display_name":"Nuclear and radioactivity studies","score":0.5717999935150146,"subfield":{"id":"https://openalex.org/subfields/2213","display_name":"Safety, Risk, Reliability and Quality"},"field":{"id":"https://openalex.org/fields/22","display_name":"Engineering"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T10973","display_name":"Radioactive element chemistry and processing","score":0.3610999882221222,"subfield":{"id":"https://openalex.org/subfields/1604","display_name":"Inorganic Chemistry"},"field":{"id":"https://openalex.org/fields/16","display_name":"Chemistry"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}},{"id":"https://openalex.org/T11242","display_name":"Nuclear Materials and Properties","score":0.04280000180006027,"subfield":{"id":"https://openalex.org/subfields/2505","display_name":"Materials Chemistry"},"field":{"id":"https://openalex.org/fields/25","display_name":"Materials Science"},"domain":{"id":"https://openalex.org/domains/3","display_name":"Physical Sciences"}}],"keywords":[{"id":"https://openalex.org/keywords/spent-nuclear-fuel-dissolution","display_name":"spent nuclear fuel dissolution","score":0.9829999804496765},{"id":"https://openalex.org/keywords/deep-geological-repository","display_name":"deep geological repository","score":0.9430000185966492},{"id":"https://openalex.org/keywords/high-level-radioactive-waste","display_name":"high-level radioactive waste","score":0.7549999952316284},{"id":"https://openalex.org/keywords/noble-metal-nanoparticles","display_name":"noble metal nanoparticles","score":0.8560000061988831},{"id":"https://openalex.org/keywords/hydrogen-production","display_name":"hydrogen production","score":0.574999988079071},{"id":"https://openalex.org/keywords/hydrogen-peroxide","display_name":"hydrogen peroxide","score":0.7599999904632568},{"id":"https://openalex.org/keywords/groundwater-hydrochemistry","display_name":"hydrogeochemistry","score":0.5199999809265137},{"id":"https://openalex.org/keywords/fuel-burnup","display_name":"fuel burnup","score":0.6039999723434448},{"id":"https://openalex.org/keywords/fuel-age","display_name":"fuel age","score":0.8259999752044678},{"id":"https://openalex.org/keywords/radiolysis","display_name":"radiolysis","score":0.718999981880188}],"concepts":[{"id":"https://openalex.org/C7083945","wikidata":"https://www.wikidata.org/wiki/Q2623868","display_name":"Spent nuclear fuel","level":2,"score":0.9142682552337646},{"id":"https://openalex.org/C88380143","wikidata":"https://www.wikidata.org/wiki/Q416674","display_name":"Dissolution","level":2,"score":0.8698698878288269},{"id":"https://openalex.org/C89690796","wikidata":"https://www.wikidata.org/wiki/Q185252","display_name":"Radioactive waste","level":2,"score":0.6300091743469238},{"id":"https://openalex.org/C2779819667","wikidata":"https://www.wikidata.org/wiki/Q194523","display_name":"Nuclear fuel","level":2,"score":0.6195537447929382},{"id":"https://openalex.org/C39432304","wikidata":"https://www.wikidata.org/wiki/Q188847","display_name":"Environmental science","level":0,"score":0.5657742023468018},{"id":"https://openalex.org/C76177295","wikidata":"https://www.wikidata.org/wiki/Q161598","display_name":"Groundwater","level":2,"score":0.5191930532455444},{"id":"https://openalex.org/C21553396","wikidata":"https://www.wikidata.org/wiki/Q3042614","display_name":"High-level waste","level":3,"score":0.48066794872283936},{"id":"https://openalex.org/C548081761","wikidata":"https://www.wikidata.org/wiki/Q180388","display_name":"Waste management","level":1,"score":0.4551652669906616},{"id":"https://openalex.org/C177322064","wikidata":"https://www.wikidata.org/wiki/Q750955","display_name":"Radiochemistry","level":1,"score":0.4260895252227783},{"id":"https://openalex.org/C185592680","wikidata":"https://www.wikidata.org/wiki/Q2329","display_name":"Chemistry","level":0,"score":0.4120187759399414},{"id":"https://openalex.org/C107872376","wikidata":"https://www.wikidata.org/wiki/Q321355","display_name":"Environmental chemistry","level":1,"score":0.3333868682384491},{"id":"https://openalex.org/C13965031","wikidata":"https://www.wikidata.org/wiki/Q243545","display_name":"Nuclear chemistry","level":1,"score":0.2963755428791046},{"id":"https://openalex.org/C127313418","wikidata":"https://www.wikidata.org/wiki/Q1069","display_name":"Geology","level":0,"score":0.21001726388931274},{"id":"https://openalex.org/C127413603","wikidata":"https://www.wikidata.org/wiki/Q11023","display_name":"Engineering","level":0,"score":0.11858034133911133},{"id":"https://openalex.org/C187320778","wikidata":"https://www.wikidata.org/wiki/Q1349130","display_name":"Geotechnical engineering","level":1,"score":0.08601734042167664},{"id":"https://openalex.org/C147789679","wikidata":"https://www.wikidata.org/wiki/Q11372","display_name":"Physical chemistry","level":1,"score":0.0}],"mesh":[{"descriptor_ui":"D007700","descriptor_name":"Kinetics","qualifier_ui":null,"qualifier_name":null,"is_major_topic":false},{"descriptor_ui":"D010084","descriptor_name":"Oxidation-Reduction","qualifier_ui":null,"qualifier_name":null,"is_major_topic":false},{"descriptor_ui":"D011850","descriptor_name":"Radioactive Waste","qualifier_ui":null,"qualifier_name":null,"is_major_topic":true},{"descriptor_ui":"D012995","descriptor_name":"Solubility","qualifier_ui":null,"qualifier_name":null,"is_major_topic":false},{"descriptor_ui":"D018505","descriptor_name":"Waste Management","qualifier_ui":null,"qualifier_name":null,"is_major_topic":true}],"locations_count":2,"locations":[{"id":"doi:10.1021/es070832y","doi":"https://doi.org/10.1021/es070832y","is_oa":false,"landing_page_url":"https://doi.org/10.1021/es070832y","pdf_url":null,"source":{"id":"https://openalex.org/S13479253","display_name":"Environmental Science & Technology","issn_l":"0013-936X","issn":["0013-936X","1520-5851"],"is_oa":false,"is_in_doaj":false,"is_core":true,"listed_in":["anvur-class-a","anvur-scientific","cwts-core","dongbi-a","fnege-4","jufo-2","ki-jl-2","medline","norway-2","poland-140","russia-white-list-1","vabb-shw"],"host_organization":"https://openalex.org/P4310320006","host_organization_name":"American Chemical Society","host_organization_lineage":["https://openalex.org/P4310320006"],"host_organization_lineage_names":["American Chemical Society"],"type":"journal"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Environmental Science & Technology","raw_type":"journal-article"},{"id":"pmid:17993152","doi":null,"is_oa":false,"landing_page_url":"https://pubmed.ncbi.nlm.nih.gov/17993152","pdf_url":null,"source":{"id":"https://openalex.org/S4306525036","display_name":"PubMed","issn_l":null,"issn":null,"is_oa":false,"is_in_doaj":false,"is_core":false,"listed_in":[],"host_organization":"https://openalex.org/I1299303238","host_organization_name":"National Institutes of Health","host_organization_lineage":["https://openalex.org/I1299303238"],"host_organization_lineage_names":[],"type":"repository"},"license":null,"license_id":null,"version":"publishedVersion","is_accepted":true,"is_published":true,"raw_source_name":"Environmental science & technology","raw_type":"Journal Article"}],"best_oa_location":null,"sustainable_development_goals":[],"study_designs":[],"awards":[],"funders":[],"has_content":{"pdf":false,"grobid_xml":false},"content_urls":null,"referenced_works_count":19,"referenced_works":["https://openalex.org/W25745213","https://openalex.org/W631299280","https://openalex.org/W858343709","https://openalex.org/W1964914273","https://openalex.org/W1985144076","https://openalex.org/W1991707633","https://openalex.org/W2009280313","https://openalex.org/W2010948145","https://openalex.org/W2014898433","https://openalex.org/W2021523869","https://openalex.org/W2024876366","https://openalex.org/W2025143610","https://openalex.org/W2030597363","https://openalex.org/W2038499887","https://openalex.org/W2039063132","https://openalex.org/W2070392217","https://openalex.org/W2070664952","https://openalex.org/W2073345848","https://openalex.org/W2319770624"],"related_works":["https://openalex.org/W2011951394","https://openalex.org/W2994174474","https://openalex.org/W4386479248","https://openalex.org/W2052320298","https://openalex.org/W2319244976","https://openalex.org/W1600961854","https://openalex.org/W4412609417","https://openalex.org/W2319879671","https://openalex.org/W2105569324","https://openalex.org/W7116048079"],"abstract_inverted_index":{"The":[0,93],"dynamics":[1],"of":[2,13,17,43,59,74,104,116,142,155],"spent":[3,44,60,117,143,167],"nuclear":[4,25,45,61,118,144,168],"fuel":[5,62,75,119,145,169],"dissolution":[6,42,63,164],"in":[7,38,129],"groundwater":[8,156],"is":[9],"an":[10],"important":[11,32],"part":[12],"the":[14,72,114,124,134,139,163],"safety":[15],"assessment":[16],"a":[18,54],"deep":[19,65],"geological":[20],"repository":[21,66,127],"for":[22,57,71,166],"high":[23],"level":[24],"waste.":[26],"In":[27],"this":[28],"paperwe":[29],"discussthe":[30],"most":[31],"elementary":[33],"processes":[34],"and":[35,85,90,101,108],"parameters":[36],"involved":[37],"radiation":[39],"induced":[40],"oxidative":[41],"fuel.":[46],"Based":[47],"on":[48,113],"these":[49],"processes,":[50],"we":[51,131],"also":[52],"present":[53],"new":[55,135],"approach":[56,69,136],"simulation":[58],"under":[64],"conditions.":[67],"This":[68,147],"accounts":[70],"effects":[73,103],"age,":[76],"burn":[77],"up,":[78],"noble":[79,105],"metal":[80,106],"nanoparticle":[81],"contents,":[82],"aqueous":[83],"H2":[84,109,151],"HCO3-":[86],"concentration,":[87],"water":[88],"chemistry,":[89],"combinations":[91],"thereof.":[92],"results":[94],"clearly":[95],"indicate":[96],"that":[97,150],"solutes":[98],"consuming":[99],"H202":[100],"combined":[102],"nanoparticles":[107],"have":[110,132],"significant":[111],"impact":[112],"rate":[115,141],"dissolution.":[120,146],"Using":[121],"data":[122],"from":[123,153],"two":[125],"possible":[126],"sites":[128],"Sweden,":[130],"employed":[133],"to":[137,161],"estimate":[138,148],"maximum":[140],"indicates":[149],"produced":[152],"radiolysis":[154],"alone":[157],"will":[158],"be":[159],"sufficient":[160],"inhibit":[162],"completely":[165],"older":[170],"than":[171],"100":[172],"years.":[173]},"counts_by_year":[{"year":2026,"cited_by_count":4},{"year":2025,"cited_by_count":3},{"year":2024,"cited_by_count":5},{"year":2023,"cited_by_count":3},{"year":2022,"cited_by_count":3},{"year":2021,"cited_by_count":3},{"year":2020,"cited_by_count":6},{"year":2019,"cited_by_count":7},{"year":2018,"cited_by_count":2},{"year":2017,"cited_by_count":3},{"year":2016,"cited_by_count":4},{"year":2015,"cited_by_count":5},{"year":2014,"cited_by_count":6},{"year":2013,"cited_by_count":3},{"year":2012,"cited_by_count":4}],"updated_date":"2026-11-04T10:54:05.112534","created_date":"2016-06-24T00:00:00"}